Evolution of Threshold Displacement Energy in Irradiated Graphite

Molecular-dynamics simulations are used to compute the threshold displacement energy (Ed) in a series of progressively damaged graphite structures. The Ed values are obtained by a statistically robust probabilistic method using a large number of primary-knock-on-atom events at energies up to 100 eV....

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Main Authors: Vukovic, F., Leyssale, J., Aurel, P., Marks, Nigel
Format: Journal Article
Published: 2018
Online Access:http://hdl.handle.net/20.500.11937/74332
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author Vukovic, F.
Leyssale, J.
Aurel, P.
Marks, Nigel
author_facet Vukovic, F.
Leyssale, J.
Aurel, P.
Marks, Nigel
author_sort Vukovic, F.
building Curtin Institutional Repository
collection Online Access
description Molecular-dynamics simulations are used to compute the threshold displacement energy (Ed) in a series of progressively damaged graphite structures. The Ed values are obtained by a statistically robust probabilistic method using a large number of primary-knock-on-atom events at energies up to 100 eV. No sharp threshold for Ed is observed, and a number of possible definitions are considered. For pristine graphite, the best estimate of Ed is 24 eV. Ed decreases with increasing irradiation damage, dropping by nearly a factor of 2 at a dose of one displacement per atom. For a fully disordered amorphous-carbon structure, Ed is around 5 eV. This evolution of Ed is an important missing ingredient in current estimates of radiation doses in nuclear reactors, which assume Ed is constant over the reactor lifetime, despite substantial structural evolution.
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spelling curtin-20.500.11937-743322019-08-22T05:42:41Z Evolution of Threshold Displacement Energy in Irradiated Graphite Vukovic, F. Leyssale, J. Aurel, P. Marks, Nigel Molecular-dynamics simulations are used to compute the threshold displacement energy (Ed) in a series of progressively damaged graphite structures. The Ed values are obtained by a statistically robust probabilistic method using a large number of primary-knock-on-atom events at energies up to 100 eV. No sharp threshold for Ed is observed, and a number of possible definitions are considered. For pristine graphite, the best estimate of Ed is 24 eV. Ed decreases with increasing irradiation damage, dropping by nearly a factor of 2 at a dose of one displacement per atom. For a fully disordered amorphous-carbon structure, Ed is around 5 eV. This evolution of Ed is an important missing ingredient in current estimates of radiation doses in nuclear reactors, which assume Ed is constant over the reactor lifetime, despite substantial structural evolution. 2018 Journal Article http://hdl.handle.net/20.500.11937/74332 10.1103/PhysRevApplied.10.064040 restricted
spellingShingle Vukovic, F.
Leyssale, J.
Aurel, P.
Marks, Nigel
Evolution of Threshold Displacement Energy in Irradiated Graphite
title Evolution of Threshold Displacement Energy in Irradiated Graphite
title_full Evolution of Threshold Displacement Energy in Irradiated Graphite
title_fullStr Evolution of Threshold Displacement Energy in Irradiated Graphite
title_full_unstemmed Evolution of Threshold Displacement Energy in Irradiated Graphite
title_short Evolution of Threshold Displacement Energy in Irradiated Graphite
title_sort evolution of threshold displacement energy in irradiated graphite
url http://hdl.handle.net/20.500.11937/74332