Photo-degradation of high efficiency fullerene-free polymer solar cells

Polymer solar cells are a promising technology for the commercialization of low cost, large scale organic solar cells. With the evolution of high efficiency (>13%) non-fullerene polymer solar cells, the stability of the cells has become a crucial parameter to be considered. Among the several degr...

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Main Authors: Upama, M., Wright, M., Mahmud, M., Elumalai, Naveen Kumar, Soufiani, A., Wang, D., Xu, C., Uddin, A.
Format: Journal Article
Published: R S C Publications 2017
Online Access:http://hdl.handle.net/20.500.11937/73978
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author Upama, M.
Wright, M.
Mahmud, M.
Elumalai, Naveen Kumar
Soufiani, A.
Wang, D.
Xu, C.
Uddin, A.
author_facet Upama, M.
Wright, M.
Mahmud, M.
Elumalai, Naveen Kumar
Soufiani, A.
Wang, D.
Xu, C.
Uddin, A.
author_sort Upama, M.
building Curtin Institutional Repository
collection Online Access
description Polymer solar cells are a promising technology for the commercialization of low cost, large scale organic solar cells. With the evolution of high efficiency (>13%) non-fullerene polymer solar cells, the stability of the cells has become a crucial parameter to be considered. Among the several degradation mechanisms of polymer solar cells, burn-in photo-degradation is relatively less studied. Herein, we present the first systematic study of photo-degradation of novel PBDB-T:ITIC fullerene-free polymer solar cells. The thermally treated and as-prepared PBDB-T:ITIC solar cells were exposed to continuous 1 sun illumination for 5 hours. The aged devices exhibited rapid losses in the short-circuit current density and fill factor. The severe short-circuit current and fill factor burn in losses were attributed to trap mediated charge recombination, as evidenced by an increase in Urbach energy for aged devices.
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institution Curtin University Malaysia
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last_indexed 2025-11-14T10:58:51Z
publishDate 2017
publisher R S C Publications
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spelling curtin-20.500.11937-739782019-06-26T08:02:22Z Photo-degradation of high efficiency fullerene-free polymer solar cells Upama, M. Wright, M. Mahmud, M. Elumalai, Naveen Kumar Soufiani, A. Wang, D. Xu, C. Uddin, A. Polymer solar cells are a promising technology for the commercialization of low cost, large scale organic solar cells. With the evolution of high efficiency (>13%) non-fullerene polymer solar cells, the stability of the cells has become a crucial parameter to be considered. Among the several degradation mechanisms of polymer solar cells, burn-in photo-degradation is relatively less studied. Herein, we present the first systematic study of photo-degradation of novel PBDB-T:ITIC fullerene-free polymer solar cells. The thermally treated and as-prepared PBDB-T:ITIC solar cells were exposed to continuous 1 sun illumination for 5 hours. The aged devices exhibited rapid losses in the short-circuit current density and fill factor. The severe short-circuit current and fill factor burn in losses were attributed to trap mediated charge recombination, as evidenced by an increase in Urbach energy for aged devices. 2017 Journal Article http://hdl.handle.net/20.500.11937/73978 10.1039/C7NR06151J R S C Publications restricted
spellingShingle Upama, M.
Wright, M.
Mahmud, M.
Elumalai, Naveen Kumar
Soufiani, A.
Wang, D.
Xu, C.
Uddin, A.
Photo-degradation of high efficiency fullerene-free polymer solar cells
title Photo-degradation of high efficiency fullerene-free polymer solar cells
title_full Photo-degradation of high efficiency fullerene-free polymer solar cells
title_fullStr Photo-degradation of high efficiency fullerene-free polymer solar cells
title_full_unstemmed Photo-degradation of high efficiency fullerene-free polymer solar cells
title_short Photo-degradation of high efficiency fullerene-free polymer solar cells
title_sort photo-degradation of high efficiency fullerene-free polymer solar cells
url http://hdl.handle.net/20.500.11937/73978