Preparation of N-Graphdiyne Nanosheets at Liquid/Liquid Interface for Photocatalytic NADH Regeneration

Two-dimensional (2D) N-graphdiyne (N-GDY) nanosheets containing different number of N were synthesized by polymerization of triazine, pyrazine, and pyridine-based monomers at liquid/liquid interface. The configurations and nanostructures of N-GDY were well-characterized. The wettability changed to m...

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Main Authors: Pan, Q., Liu, H., Zhao, Y., Chen, S., Xue, B., Kan, X., Huang, X., Liu, Jian, Li, Z.
Format: Journal Article
Published: American Chemical Society 2019
Online Access:http://hdl.handle.net/20.500.11937/73941
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author Pan, Q.
Liu, H.
Zhao, Y.
Chen, S.
Xue, B.
Kan, X.
Huang, X.
Liu, Jian
Li, Z.
author_facet Pan, Q.
Liu, H.
Zhao, Y.
Chen, S.
Xue, B.
Kan, X.
Huang, X.
Liu, Jian
Li, Z.
author_sort Pan, Q.
building Curtin Institutional Repository
collection Online Access
description Two-dimensional (2D) N-graphdiyne (N-GDY) nanosheets containing different number of N were synthesized by polymerization of triazine, pyrazine, and pyridine-based monomers at liquid/liquid interface. The configurations and nanostructures of N-GDY were well-characterized. The wettability changed to more hydrophilic as the N contents increased. The collected N-GDY was further employed as metal-free photocatalyst for NADH regeneration. The catalytic performance was related with the N content in the graphdiyne. The N3-GDY demonstrated the best activity. This strategy provided a new promising platform of designing unique 2D N-GDY with tunable performance in biorelated catalysis.
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institution Curtin University Malaysia
institution_category Local University
last_indexed 2025-11-14T10:58:41Z
publishDate 2019
publisher American Chemical Society
recordtype eprints
repository_type Digital Repository
spelling curtin-20.500.11937-739412019-03-25T04:50:50Z Preparation of N-Graphdiyne Nanosheets at Liquid/Liquid Interface for Photocatalytic NADH Regeneration Pan, Q. Liu, H. Zhao, Y. Chen, S. Xue, B. Kan, X. Huang, X. Liu, Jian Li, Z. Two-dimensional (2D) N-graphdiyne (N-GDY) nanosheets containing different number of N were synthesized by polymerization of triazine, pyrazine, and pyridine-based monomers at liquid/liquid interface. The configurations and nanostructures of N-GDY were well-characterized. The wettability changed to more hydrophilic as the N contents increased. The collected N-GDY was further employed as metal-free photocatalyst for NADH regeneration. The catalytic performance was related with the N content in the graphdiyne. The N3-GDY demonstrated the best activity. This strategy provided a new promising platform of designing unique 2D N-GDY with tunable performance in biorelated catalysis. 2019 Journal Article http://hdl.handle.net/20.500.11937/73941 10.1021/acsami.8b03311 American Chemical Society restricted
spellingShingle Pan, Q.
Liu, H.
Zhao, Y.
Chen, S.
Xue, B.
Kan, X.
Huang, X.
Liu, Jian
Li, Z.
Preparation of N-Graphdiyne Nanosheets at Liquid/Liquid Interface for Photocatalytic NADH Regeneration
title Preparation of N-Graphdiyne Nanosheets at Liquid/Liquid Interface for Photocatalytic NADH Regeneration
title_full Preparation of N-Graphdiyne Nanosheets at Liquid/Liquid Interface for Photocatalytic NADH Regeneration
title_fullStr Preparation of N-Graphdiyne Nanosheets at Liquid/Liquid Interface for Photocatalytic NADH Regeneration
title_full_unstemmed Preparation of N-Graphdiyne Nanosheets at Liquid/Liquid Interface for Photocatalytic NADH Regeneration
title_short Preparation of N-Graphdiyne Nanosheets at Liquid/Liquid Interface for Photocatalytic NADH Regeneration
title_sort preparation of n-graphdiyne nanosheets at liquid/liquid interface for photocatalytic nadh regeneration
url http://hdl.handle.net/20.500.11937/73941