Spatio-temporal distribution and sources of Pb identified by stable isotopic ratios in sediments from the Yangtze River Estuary and adjacent areas

© 2016 To understand the spatio-temporal distribution and sources of Pb in the sediments of the Yangtze River Estuary and its adjacent areas, 25 surface sediments and 1 sediment core were collected from the study areas. The concentrations of Al and Pb of these sediments exhibit a decreasing trend fr...

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Main Authors: Chen, B., Liu, Jian, Hu, L., Liu, M., Wang, L., Zhang, X., Fan, D.
Format: Journal Article
Published: Elsevier 2017
Online Access:http://hdl.handle.net/20.500.11937/72872
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author Chen, B.
Liu, Jian
Hu, L.
Liu, M.
Wang, L.
Zhang, X.
Fan, D.
author_facet Chen, B.
Liu, Jian
Hu, L.
Liu, M.
Wang, L.
Zhang, X.
Fan, D.
author_sort Chen, B.
building Curtin Institutional Repository
collection Online Access
description © 2016 To understand the spatio-temporal distribution and sources of Pb in the sediments of the Yangtze River Estuary and its adjacent areas, 25 surface sediments and 1 sediment core were collected from the study areas. The concentrations of Al and Pb of these sediments exhibit a decreasing trend from the nearshore towards the offshore, with higher concentrations in the coastal areas of the East China Sea (ECS) and southwest of Jeju Island. According to the stable isotopic ratios of Pb, in combination with the elemental ratios and clay mineral data, it is inferred that sedimentary Pb in the surface sediments of the coastal areas of the ECS may come primarily from the Yangtze River, while the Pb southwest of Jeju Island is probably derived from both the Yangtze and Yellow Rivers. The particulate Pb derived from the Yangtze River was possibly dispersed along two paths: the path southward along the coastline of the ECS and the path eastward associated with the Changjiang Diluted Water (CDW), which crosses the shelf of the ECS towards the area southeast of Jeju Island. Although the Yangtze River Basin witnessed rapid economic development during the period from the late 1970s to the middle 1990s, the influence of human activity on Pb concentration remained weak in the Yangtze River Estuary. Since the early 2000s, however, sedimentary Pb has been significantly increasing in the coastal mud areas of the ECS due to the increasing influence of human activity, such as the increase in atmospheric emission of anthropogenic Pb in China, construction of the Three Gorges Dam (TGD), and the construction of smaller dams in the upper reaches of the Yangtze River. Coal combustion and the smelting of non-ferrous metals are possible anthropogenic sources for the sedimentary Pb in the Yangtze River Estuary.
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institution Curtin University Malaysia
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publishDate 2017
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spelling curtin-20.500.11937-728722018-12-13T09:33:39Z Spatio-temporal distribution and sources of Pb identified by stable isotopic ratios in sediments from the Yangtze River Estuary and adjacent areas Chen, B. Liu, Jian Hu, L. Liu, M. Wang, L. Zhang, X. Fan, D. © 2016 To understand the spatio-temporal distribution and sources of Pb in the sediments of the Yangtze River Estuary and its adjacent areas, 25 surface sediments and 1 sediment core were collected from the study areas. The concentrations of Al and Pb of these sediments exhibit a decreasing trend from the nearshore towards the offshore, with higher concentrations in the coastal areas of the East China Sea (ECS) and southwest of Jeju Island. According to the stable isotopic ratios of Pb, in combination with the elemental ratios and clay mineral data, it is inferred that sedimentary Pb in the surface sediments of the coastal areas of the ECS may come primarily from the Yangtze River, while the Pb southwest of Jeju Island is probably derived from both the Yangtze and Yellow Rivers. The particulate Pb derived from the Yangtze River was possibly dispersed along two paths: the path southward along the coastline of the ECS and the path eastward associated with the Changjiang Diluted Water (CDW), which crosses the shelf of the ECS towards the area southeast of Jeju Island. Although the Yangtze River Basin witnessed rapid economic development during the period from the late 1970s to the middle 1990s, the influence of human activity on Pb concentration remained weak in the Yangtze River Estuary. Since the early 2000s, however, sedimentary Pb has been significantly increasing in the coastal mud areas of the ECS due to the increasing influence of human activity, such as the increase in atmospheric emission of anthropogenic Pb in China, construction of the Three Gorges Dam (TGD), and the construction of smaller dams in the upper reaches of the Yangtze River. Coal combustion and the smelting of non-ferrous metals are possible anthropogenic sources for the sedimentary Pb in the Yangtze River Estuary. 2017 Journal Article http://hdl.handle.net/20.500.11937/72872 10.1016/j.scitotenv.2016.12.042 Elsevier restricted
spellingShingle Chen, B.
Liu, Jian
Hu, L.
Liu, M.
Wang, L.
Zhang, X.
Fan, D.
Spatio-temporal distribution and sources of Pb identified by stable isotopic ratios in sediments from the Yangtze River Estuary and adjacent areas
title Spatio-temporal distribution and sources of Pb identified by stable isotopic ratios in sediments from the Yangtze River Estuary and adjacent areas
title_full Spatio-temporal distribution and sources of Pb identified by stable isotopic ratios in sediments from the Yangtze River Estuary and adjacent areas
title_fullStr Spatio-temporal distribution and sources of Pb identified by stable isotopic ratios in sediments from the Yangtze River Estuary and adjacent areas
title_full_unstemmed Spatio-temporal distribution and sources of Pb identified by stable isotopic ratios in sediments from the Yangtze River Estuary and adjacent areas
title_short Spatio-temporal distribution and sources of Pb identified by stable isotopic ratios in sediments from the Yangtze River Estuary and adjacent areas
title_sort spatio-temporal distribution and sources of pb identified by stable isotopic ratios in sediments from the yangtze river estuary and adjacent areas
url http://hdl.handle.net/20.500.11937/72872