Energy transfer between Eu3+ and Nd3+ in near-infrared emitting β-triketonate coordination polymers

© The Royal Society of Chemistry. Isomorphous ß-triketonate-based lanthanoid polymers containing tris(4-methylbenzoyl)methanide (mtbm) and Rb+ with formula {[Ln(Rb)(mtbm)4]2}n (Ln = Eu3+ and Nd3+) have been synthesised and structurally characterised. The photophysical properties for the Nd3+ complex...

Full description

Bibliographic Details
Main Authors: Abad Galán, L., Sobolev, A., Skelton, B., Zysman-Colman, E., Ogden, Mark, Massi, Massimiliano
Format: Journal Article
Published: R S C Publications 2018
Online Access:http://hdl.handle.net/20.500.11937/72787
_version_ 1848762841871417344
author Abad Galán, L.
Sobolev, A.
Skelton, B.
Zysman-Colman, E.
Ogden, Mark
Massi, Massimiliano
author_facet Abad Galán, L.
Sobolev, A.
Skelton, B.
Zysman-Colman, E.
Ogden, Mark
Massi, Massimiliano
author_sort Abad Galán, L.
building Curtin Institutional Repository
collection Online Access
description © The Royal Society of Chemistry. Isomorphous ß-triketonate-based lanthanoid polymers containing tris(4-methylbenzoyl)methanide (mtbm) and Rb+ with formula {[Ln(Rb)(mtbm)4]2}n (Ln = Eu3+ and Nd3+) have been synthesised and structurally characterised. The photophysical properties for the Nd3+ complex presented relatively long lifetimes and high quantum yields in comparison with analogous ß-diketonate complexes. Mixed lanthanoid complexes were also formed and their luminescence properties studied, with effective sensitisation of the 4F3/2 of Nd3+via the 5D0 of Eu3+, which is to the best of our knowledge the first example of Eu3+ to Nd3+ sensitisation in a structurally defined coordination complex or polymer.
first_indexed 2025-11-14T10:53:59Z
format Journal Article
id curtin-20.500.11937-72787
institution Curtin University Malaysia
institution_category Local University
last_indexed 2025-11-14T10:53:59Z
publishDate 2018
publisher R S C Publications
recordtype eprints
repository_type Digital Repository
spelling curtin-20.500.11937-727872019-03-18T06:53:46Z Energy transfer between Eu3+ and Nd3+ in near-infrared emitting β-triketonate coordination polymers Abad Galán, L. Sobolev, A. Skelton, B. Zysman-Colman, E. Ogden, Mark Massi, Massimiliano © The Royal Society of Chemistry. Isomorphous ß-triketonate-based lanthanoid polymers containing tris(4-methylbenzoyl)methanide (mtbm) and Rb+ with formula {[Ln(Rb)(mtbm)4]2}n (Ln = Eu3+ and Nd3+) have been synthesised and structurally characterised. The photophysical properties for the Nd3+ complex presented relatively long lifetimes and high quantum yields in comparison with analogous ß-diketonate complexes. Mixed lanthanoid complexes were also formed and their luminescence properties studied, with effective sensitisation of the 4F3/2 of Nd3+via the 5D0 of Eu3+, which is to the best of our knowledge the first example of Eu3+ to Nd3+ sensitisation in a structurally defined coordination complex or polymer. 2018 Journal Article http://hdl.handle.net/20.500.11937/72787 10.1039/c8dt02499e R S C Publications restricted
spellingShingle Abad Galán, L.
Sobolev, A.
Skelton, B.
Zysman-Colman, E.
Ogden, Mark
Massi, Massimiliano
Energy transfer between Eu3+ and Nd3+ in near-infrared emitting β-triketonate coordination polymers
title Energy transfer between Eu3+ and Nd3+ in near-infrared emitting β-triketonate coordination polymers
title_full Energy transfer between Eu3+ and Nd3+ in near-infrared emitting β-triketonate coordination polymers
title_fullStr Energy transfer between Eu3+ and Nd3+ in near-infrared emitting β-triketonate coordination polymers
title_full_unstemmed Energy transfer between Eu3+ and Nd3+ in near-infrared emitting β-triketonate coordination polymers
title_short Energy transfer between Eu3+ and Nd3+ in near-infrared emitting β-triketonate coordination polymers
title_sort energy transfer between eu3+ and nd3+ in near-infrared emitting β-triketonate coordination polymers
url http://hdl.handle.net/20.500.11937/72787