Performance of layered double hydroxides intercalated with acetate as biodenitrification carbon source: The effects of metal ions and particle size

In situ synthesis of layered double hydroxides (LDHs) is an effective way to extract short chain fatty acids (SCFAs) from anaerobic fermentation liquid to be used as carbon source for biodenitrification, but the slow release performance need to be improved. Three layered double hydroxides with diffe...

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Main Authors: Jiang, L., Liu, Jian, Zuo, K., Zou, L., Li, Y., Qian, G., Xu, Z.
Format: Journal Article
Published: Elsevier BV 2018
Online Access:http://hdl.handle.net/20.500.11937/72462
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author Jiang, L.
Liu, Jian
Zuo, K.
Zou, L.
Li, Y.
Qian, G.
Xu, Z.
author_facet Jiang, L.
Liu, Jian
Zuo, K.
Zou, L.
Li, Y.
Qian, G.
Xu, Z.
author_sort Jiang, L.
building Curtin Institutional Repository
collection Online Access
description In situ synthesis of layered double hydroxides (LDHs) is an effective way to extract short chain fatty acids (SCFAs) from anaerobic fermentation liquid to be used as carbon source for biodenitrification, but the slow release performance need to be improved. Three layered double hydroxides with different metal cations (Mg-Al, Ni-Al, Ni-Fe) intercalated with acetate (Ac) were successfully prepared in the present study. The release rates decreased in the order of MgAl-LDH > NiAl-LDH > NiFe-LDH, meaning that NiFe-LDH-Ac showed the best slow release performance. The release rate of LDHs decreased greatly along with the increase of particle size. Batch denitrification tests showed that the carbon source utilization efficiency of NiFe-LDH-Ac was 79.9%, which was much higher than that of CH3COONa (48.8%) as control. These results indicate that NiFe-LDH-Ac could be successfully employed as slow release carbon source for biodenitrification.
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publishDate 2018
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spelling curtin-20.500.11937-724622019-01-31T03:22:39Z Performance of layered double hydroxides intercalated with acetate as biodenitrification carbon source: The effects of metal ions and particle size Jiang, L. Liu, Jian Zuo, K. Zou, L. Li, Y. Qian, G. Xu, Z. In situ synthesis of layered double hydroxides (LDHs) is an effective way to extract short chain fatty acids (SCFAs) from anaerobic fermentation liquid to be used as carbon source for biodenitrification, but the slow release performance need to be improved. Three layered double hydroxides with different metal cations (Mg-Al, Ni-Al, Ni-Fe) intercalated with acetate (Ac) were successfully prepared in the present study. The release rates decreased in the order of MgAl-LDH > NiAl-LDH > NiFe-LDH, meaning that NiFe-LDH-Ac showed the best slow release performance. The release rate of LDHs decreased greatly along with the increase of particle size. Batch denitrification tests showed that the carbon source utilization efficiency of NiFe-LDH-Ac was 79.9%, which was much higher than that of CH3COONa (48.8%) as control. These results indicate that NiFe-LDH-Ac could be successfully employed as slow release carbon source for biodenitrification. 2018 Journal Article http://hdl.handle.net/20.500.11937/72462 10.1016/j.biortech.2018.03.032 Elsevier BV restricted
spellingShingle Jiang, L.
Liu, Jian
Zuo, K.
Zou, L.
Li, Y.
Qian, G.
Xu, Z.
Performance of layered double hydroxides intercalated with acetate as biodenitrification carbon source: The effects of metal ions and particle size
title Performance of layered double hydroxides intercalated with acetate as biodenitrification carbon source: The effects of metal ions and particle size
title_full Performance of layered double hydroxides intercalated with acetate as biodenitrification carbon source: The effects of metal ions and particle size
title_fullStr Performance of layered double hydroxides intercalated with acetate as biodenitrification carbon source: The effects of metal ions and particle size
title_full_unstemmed Performance of layered double hydroxides intercalated with acetate as biodenitrification carbon source: The effects of metal ions and particle size
title_short Performance of layered double hydroxides intercalated with acetate as biodenitrification carbon source: The effects of metal ions and particle size
title_sort performance of layered double hydroxides intercalated with acetate as biodenitrification carbon source: the effects of metal ions and particle size
url http://hdl.handle.net/20.500.11937/72462