Comparative study of acid functionization of carbon nanotube via ultrasonic and reflux mechanism

© 2018 Elsevier Ltd. Multi-walled carbon nanotubes (MWCNTs) have a great potential in wide applications due to their extraordinary physical, thermal and mechanical properties. However, the known shortcomings, such as hydrophobic nature, poor solubility and dispersibility in most solvents have impede...

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Main Authors: Jun, L., Mujawar, Mubarak, Yon, L., Bing, C., Khalid, M., Abdullah, E.
Format: Journal Article
Published: Elsevuer BV 2018
Online Access:http://hdl.handle.net/20.500.11937/72181
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author Jun, L.
Mujawar, Mubarak
Yon, L.
Bing, C.
Khalid, M.
Abdullah, E.
author_facet Jun, L.
Mujawar, Mubarak
Yon, L.
Bing, C.
Khalid, M.
Abdullah, E.
author_sort Jun, L.
building Curtin Institutional Repository
collection Online Access
description © 2018 Elsevier Ltd. Multi-walled carbon nanotubes (MWCNTs) have a great potential in wide applications due to their extraordinary physical, thermal and mechanical properties. However, the known shortcomings, such as hydrophobic nature, poor solubility and dispersibility in most solvents have impeded the technology to further develop. In the present study, various types of acid functionalized MWNCTs (f-MWCNTs) samples were prepared. The investigated process parameters include type of acids, acid concentrations, treatment methods, operating temperature and treatment duration. The f-MWCNTs were characterized using Fourier Transform Infrared Spectroscopy (FTIR), Energy dispersive X-ray (EDX), Field Emission Scanning Electron Microscopy (FESEM) and Zetasizer. The optimum conditions for acid functionalization of MWCNTs were achieved by dispersing MWCNTs in concentrated nitric and sulfuric acid mixture (1:3 v/v ratio), via ultrasonication treatment method at 40 °C for 2.5 h. EDX analysis also revealed that, 21.36 wt% of oxygenated functional groups, with no strong detection of inorganic and metal impurities. In addition, FESEM results also revealed that there is no any severe structural damage on the surface. Acid functionalization of MWCNTs via ultrasonic bath methods is more desirable than reflux method as it can result in high yields of MWCNTs with high density of oxygenated functional groups and minimum structural destruction on the surface of MWCNTs.
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spelling curtin-20.500.11937-721812018-12-13T09:31:55Z Comparative study of acid functionization of carbon nanotube via ultrasonic and reflux mechanism Jun, L. Mujawar, Mubarak Yon, L. Bing, C. Khalid, M. Abdullah, E. © 2018 Elsevier Ltd. Multi-walled carbon nanotubes (MWCNTs) have a great potential in wide applications due to their extraordinary physical, thermal and mechanical properties. However, the known shortcomings, such as hydrophobic nature, poor solubility and dispersibility in most solvents have impeded the technology to further develop. In the present study, various types of acid functionalized MWNCTs (f-MWCNTs) samples were prepared. The investigated process parameters include type of acids, acid concentrations, treatment methods, operating temperature and treatment duration. The f-MWCNTs were characterized using Fourier Transform Infrared Spectroscopy (FTIR), Energy dispersive X-ray (EDX), Field Emission Scanning Electron Microscopy (FESEM) and Zetasizer. The optimum conditions for acid functionalization of MWCNTs were achieved by dispersing MWCNTs in concentrated nitric and sulfuric acid mixture (1:3 v/v ratio), via ultrasonication treatment method at 40 °C for 2.5 h. EDX analysis also revealed that, 21.36 wt% of oxygenated functional groups, with no strong detection of inorganic and metal impurities. In addition, FESEM results also revealed that there is no any severe structural damage on the surface. Acid functionalization of MWCNTs via ultrasonic bath methods is more desirable than reflux method as it can result in high yields of MWCNTs with high density of oxygenated functional groups and minimum structural destruction on the surface of MWCNTs. 2018 Journal Article http://hdl.handle.net/20.500.11937/72181 10.1016/j.jece.2018.09.008 Elsevuer BV restricted
spellingShingle Jun, L.
Mujawar, Mubarak
Yon, L.
Bing, C.
Khalid, M.
Abdullah, E.
Comparative study of acid functionization of carbon nanotube via ultrasonic and reflux mechanism
title Comparative study of acid functionization of carbon nanotube via ultrasonic and reflux mechanism
title_full Comparative study of acid functionization of carbon nanotube via ultrasonic and reflux mechanism
title_fullStr Comparative study of acid functionization of carbon nanotube via ultrasonic and reflux mechanism
title_full_unstemmed Comparative study of acid functionization of carbon nanotube via ultrasonic and reflux mechanism
title_short Comparative study of acid functionization of carbon nanotube via ultrasonic and reflux mechanism
title_sort comparative study of acid functionization of carbon nanotube via ultrasonic and reflux mechanism
url http://hdl.handle.net/20.500.11937/72181