Effect of Monovalent and Divalent Salts on the Interfacial Tension of n-Heptane against Aqueous Anionic Surfactant Solutions

© 2017 American Chemical Society. A very low interfacial tension, γ, can be achieved between an oil phase and an aqueous solution containing anionic surfactant and salt at a very low concentration. This phenomenon can have potential applications in recovering residual oil from the reservoir through...

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Main Authors: Jha, N., Iglauer, Stefan, Sangwai, J.
Format: Journal Article
Published: American Chemical Society 2018
Online Access:http://hdl.handle.net/20.500.11937/71903
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author Jha, N.
Iglauer, Stefan
Sangwai, J.
author_facet Jha, N.
Iglauer, Stefan
Sangwai, J.
author_sort Jha, N.
building Curtin Institutional Repository
collection Online Access
description © 2017 American Chemical Society. A very low interfacial tension, γ, can be achieved between an oil phase and an aqueous solution containing anionic surfactant and salt at a very low concentration. This phenomenon can have potential applications in recovering residual oil from the reservoir through low salinity-low surfactant enhanced oil recovery flooding. Measurements of γ between n-heptane and aqueous solution of anionic surfactants in the concentration range of 0.141-2.167 mM and salts in the concentration range of 9.010-119.780 mM at 313.15 ± 0.1 K have been carried out. The experimental results show that the value of γ falls to a lowest value at a temperature above the Krafft point when the concentration of anionic surfactants [sodium dodecyl sulfate (SDS) and dioctyl sulfosuccinate sodium salt (AOT)] is increased up to a maximum surface excess concentration in an aqueous solution in the presence of monovalent [sodium chloride, (NaCl)] and divalent [calcium chloride, (CaCl2)] salts in the low concentration range. To understand and adequately capture the reduction of γ in such systems with n-heptane as an oil phase, a simplistic model is being proposed here. This model is an extension of the Petersen and Saykally model which was earlier developed to capture the Jones-Ray effect.
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spelling curtin-20.500.11937-719032019-04-02T05:21:52Z Effect of Monovalent and Divalent Salts on the Interfacial Tension of n-Heptane against Aqueous Anionic Surfactant Solutions Jha, N. Iglauer, Stefan Sangwai, J. © 2017 American Chemical Society. A very low interfacial tension, γ, can be achieved between an oil phase and an aqueous solution containing anionic surfactant and salt at a very low concentration. This phenomenon can have potential applications in recovering residual oil from the reservoir through low salinity-low surfactant enhanced oil recovery flooding. Measurements of γ between n-heptane and aqueous solution of anionic surfactants in the concentration range of 0.141-2.167 mM and salts in the concentration range of 9.010-119.780 mM at 313.15 ± 0.1 K have been carried out. The experimental results show that the value of γ falls to a lowest value at a temperature above the Krafft point when the concentration of anionic surfactants [sodium dodecyl sulfate (SDS) and dioctyl sulfosuccinate sodium salt (AOT)] is increased up to a maximum surface excess concentration in an aqueous solution in the presence of monovalent [sodium chloride, (NaCl)] and divalent [calcium chloride, (CaCl2)] salts in the low concentration range. To understand and adequately capture the reduction of γ in such systems with n-heptane as an oil phase, a simplistic model is being proposed here. This model is an extension of the Petersen and Saykally model which was earlier developed to capture the Jones-Ray effect. 2018 Journal Article http://hdl.handle.net/20.500.11937/71903 10.1021/acs.jced.7b00640 American Chemical Society restricted
spellingShingle Jha, N.
Iglauer, Stefan
Sangwai, J.
Effect of Monovalent and Divalent Salts on the Interfacial Tension of n-Heptane against Aqueous Anionic Surfactant Solutions
title Effect of Monovalent and Divalent Salts on the Interfacial Tension of n-Heptane against Aqueous Anionic Surfactant Solutions
title_full Effect of Monovalent and Divalent Salts on the Interfacial Tension of n-Heptane against Aqueous Anionic Surfactant Solutions
title_fullStr Effect of Monovalent and Divalent Salts on the Interfacial Tension of n-Heptane against Aqueous Anionic Surfactant Solutions
title_full_unstemmed Effect of Monovalent and Divalent Salts on the Interfacial Tension of n-Heptane against Aqueous Anionic Surfactant Solutions
title_short Effect of Monovalent and Divalent Salts on the Interfacial Tension of n-Heptane against Aqueous Anionic Surfactant Solutions
title_sort effect of monovalent and divalent salts on the interfacial tension of n-heptane against aqueous anionic surfactant solutions
url http://hdl.handle.net/20.500.11937/71903