Preparation of Magnetic Tubular Nanoreactors for Highly Efficient Catalysis

© 2016 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim We report an efficient and controllable route to prepare magnetic tubular nanoreactors composed of a mesoporous SiO2shell with iron-noble metal nanoparticles inside. The key of this method is to design and fabricate Fe nanoparticles encapsulate...

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Main Authors: Yang, S., Peng, L., Cao, C., Wei, F., Liu, Jian, Zhu, Y., Liu, C., Wang, X., Song, W.
Format: Journal Article
Published: Wiley - V C H Verlag GmbH & Co. KGaA 2016
Online Access:http://hdl.handle.net/20.500.11937/71643
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author Yang, S.
Peng, L.
Cao, C.
Wei, F.
Liu, Jian
Zhu, Y.
Liu, C.
Wang, X.
Song, W.
author_facet Yang, S.
Peng, L.
Cao, C.
Wei, F.
Liu, Jian
Zhu, Y.
Liu, C.
Wang, X.
Song, W.
author_sort Yang, S.
building Curtin Institutional Repository
collection Online Access
description © 2016 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim We report an efficient and controllable route to prepare magnetic tubular nanoreactors composed of a mesoporous SiO2shell with iron-noble metal nanoparticles inside. The key of this method is to design and fabricate Fe nanoparticles encapsulated in a mesoporous SiO2shell. Making use of a galvanic replacement reaction between Fe and noble metal ions, all of the noble metal nanoparticles are loaded inside the mesoporous SiO2shell, and thus nanoreactors are formed. Taking Pd as an example, the prepared Pd-Fe@meso-SiO2tubular nanoreactor exhibits a high catalytic activity and excellent reusability for styrene hydrogenation under mild conditions. This study provides a facile route to fabricate magnetic nanoreactors with enhanced catalytic properties.
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institution Curtin University Malaysia
institution_category Local University
last_indexed 2025-11-14T10:49:05Z
publishDate 2016
publisher Wiley - V C H Verlag GmbH & Co. KGaA
recordtype eprints
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spelling curtin-20.500.11937-716432018-12-13T09:35:02Z Preparation of Magnetic Tubular Nanoreactors for Highly Efficient Catalysis Yang, S. Peng, L. Cao, C. Wei, F. Liu, Jian Zhu, Y. Liu, C. Wang, X. Song, W. © 2016 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim We report an efficient and controllable route to prepare magnetic tubular nanoreactors composed of a mesoporous SiO2shell with iron-noble metal nanoparticles inside. The key of this method is to design and fabricate Fe nanoparticles encapsulated in a mesoporous SiO2shell. Making use of a galvanic replacement reaction between Fe and noble metal ions, all of the noble metal nanoparticles are loaded inside the mesoporous SiO2shell, and thus nanoreactors are formed. Taking Pd as an example, the prepared Pd-Fe@meso-SiO2tubular nanoreactor exhibits a high catalytic activity and excellent reusability for styrene hydrogenation under mild conditions. This study provides a facile route to fabricate magnetic nanoreactors with enhanced catalytic properties. 2016 Journal Article http://hdl.handle.net/20.500.11937/71643 10.1002/asia.201600454 Wiley - V C H Verlag GmbH & Co. KGaA restricted
spellingShingle Yang, S.
Peng, L.
Cao, C.
Wei, F.
Liu, Jian
Zhu, Y.
Liu, C.
Wang, X.
Song, W.
Preparation of Magnetic Tubular Nanoreactors for Highly Efficient Catalysis
title Preparation of Magnetic Tubular Nanoreactors for Highly Efficient Catalysis
title_full Preparation of Magnetic Tubular Nanoreactors for Highly Efficient Catalysis
title_fullStr Preparation of Magnetic Tubular Nanoreactors for Highly Efficient Catalysis
title_full_unstemmed Preparation of Magnetic Tubular Nanoreactors for Highly Efficient Catalysis
title_short Preparation of Magnetic Tubular Nanoreactors for Highly Efficient Catalysis
title_sort preparation of magnetic tubular nanoreactors for highly efficient catalysis
url http://hdl.handle.net/20.500.11937/71643