Micelle and Surface Tension of Double-Chain Cationic Surfactants

Since the early 20th century, the slightly disparate measurements of a surfactant's critical micelle concentration, via either surface tension or electrical conductivity, have been assumed one and the same. As a consequence, the possibility that micelles can adsorb at the air/water surface has...

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Main Authors: Phan, Chi, Yusa, S., Honda, T., Sharker, K., Hyde, A., Nguyen, C.
Format: Journal Article
Published: 2018
Online Access:http://hdl.handle.net/20.500.11937/71561
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author Phan, Chi
Yusa, S.
Honda, T.
Sharker, K.
Hyde, A.
Nguyen, C.
author_facet Phan, Chi
Yusa, S.
Honda, T.
Sharker, K.
Hyde, A.
Nguyen, C.
author_sort Phan, Chi
building Curtin Institutional Repository
collection Online Access
description Since the early 20th century, the slightly disparate measurements of a surfactant's critical micelle concentration, via either surface tension or electrical conductivity, have been assumed one and the same. As a consequence, the possibility that micelles can adsorb at the air/water surface has been disregarded and has led to some abnormalities in the literature that remain as yet unresolved. In this paper, we closely examined the two critical concentrations for a double-chain cationic surfactant. We confirmed that the two concentrations represent two different physical phenomena. Furthermore, the results verified the existence of surface micelles, which are different from the bulk micelles. The formation of the surface micelles can be explained by the structural changes of the adsorption layer, which was also corroborated by molecular simulations. The findings open new challenges to examine the surface adsorption, which offers new insights into the molecular levels.
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spelling curtin-20.500.11937-715612019-02-12T06:41:50Z Micelle and Surface Tension of Double-Chain Cationic Surfactants Phan, Chi Yusa, S. Honda, T. Sharker, K. Hyde, A. Nguyen, C. Since the early 20th century, the slightly disparate measurements of a surfactant's critical micelle concentration, via either surface tension or electrical conductivity, have been assumed one and the same. As a consequence, the possibility that micelles can adsorb at the air/water surface has been disregarded and has led to some abnormalities in the literature that remain as yet unresolved. In this paper, we closely examined the two critical concentrations for a double-chain cationic surfactant. We confirmed that the two concentrations represent two different physical phenomena. Furthermore, the results verified the existence of surface micelles, which are different from the bulk micelles. The formation of the surface micelles can be explained by the structural changes of the adsorption layer, which was also corroborated by molecular simulations. The findings open new challenges to examine the surface adsorption, which offers new insights into the molecular levels. 2018 Journal Article http://hdl.handle.net/20.500.11937/71561 10.1021/acsomega.8b01667 restricted
spellingShingle Phan, Chi
Yusa, S.
Honda, T.
Sharker, K.
Hyde, A.
Nguyen, C.
Micelle and Surface Tension of Double-Chain Cationic Surfactants
title Micelle and Surface Tension of Double-Chain Cationic Surfactants
title_full Micelle and Surface Tension of Double-Chain Cationic Surfactants
title_fullStr Micelle and Surface Tension of Double-Chain Cationic Surfactants
title_full_unstemmed Micelle and Surface Tension of Double-Chain Cationic Surfactants
title_short Micelle and Surface Tension of Double-Chain Cationic Surfactants
title_sort micelle and surface tension of double-chain cationic surfactants
url http://hdl.handle.net/20.500.11937/71561