Structure and Hydrogenation Properties of a HfNbTiVZr High-Entropy Alloy

© 2018 American Chemical Society. A high-entropy alloy (HEA) of HfNbTiVZr was synthesized using an arc furnace followed by ball milling. The hydrogen absorption mechanism was studied by in situ X-ray diffraction at different temperatures and by in situ and ex situ neutron diffraction experiments. Th...

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Main Authors: Karlsson, D., Ek, G., Cedervall, J., Zlotea, C., Moller, Kasper, Hansen, T., Bednarcík, J., Paskevicius, M., Sørby, M., Jensen, T., Jansson, U., Sahlberg, M.
Format: Journal Article
Published: American Chemical Society 2018
Online Access:http://hdl.handle.net/20.500.11937/71372
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author Karlsson, D.
Ek, G.
Cedervall, J.
Zlotea, C.
Moller, Kasper
Hansen, T.
Bednarcík, J.
Paskevicius, M.
Sørby, M.
Jensen, T.
Jansson, U.
Sahlberg, M.
author_facet Karlsson, D.
Ek, G.
Cedervall, J.
Zlotea, C.
Moller, Kasper
Hansen, T.
Bednarcík, J.
Paskevicius, M.
Sørby, M.
Jensen, T.
Jansson, U.
Sahlberg, M.
author_sort Karlsson, D.
building Curtin Institutional Repository
collection Online Access
description © 2018 American Chemical Society. A high-entropy alloy (HEA) of HfNbTiVZr was synthesized using an arc furnace followed by ball milling. The hydrogen absorption mechanism was studied by in situ X-ray diffraction at different temperatures and by in situ and ex situ neutron diffraction experiments. The body centered cubic (BCC) metal phase undergoes a phase transformation to a body centered tetragonal (BCT) hydride phase with hydrogen occupying both tetrahedral and octahedral interstitial sites in the structure. Hydrogen cycling of the alloy at 500 °C is stable. The large lattice strain in the HEA seems favorable for absorption in both octahedral and tetrahedral sites. HEAs therefore have potential as hydrogen storage materials because of favorable absorption in all interstitial sites within the structure.
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institution Curtin University Malaysia
institution_category Local University
last_indexed 2025-11-14T10:47:57Z
publishDate 2018
publisher American Chemical Society
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spelling curtin-20.500.11937-713722018-12-13T09:33:40Z Structure and Hydrogenation Properties of a HfNbTiVZr High-Entropy Alloy Karlsson, D. Ek, G. Cedervall, J. Zlotea, C. Moller, Kasper Hansen, T. Bednarcík, J. Paskevicius, M. Sørby, M. Jensen, T. Jansson, U. Sahlberg, M. © 2018 American Chemical Society. A high-entropy alloy (HEA) of HfNbTiVZr was synthesized using an arc furnace followed by ball milling. The hydrogen absorption mechanism was studied by in situ X-ray diffraction at different temperatures and by in situ and ex situ neutron diffraction experiments. The body centered cubic (BCC) metal phase undergoes a phase transformation to a body centered tetragonal (BCT) hydride phase with hydrogen occupying both tetrahedral and octahedral interstitial sites in the structure. Hydrogen cycling of the alloy at 500 °C is stable. The large lattice strain in the HEA seems favorable for absorption in both octahedral and tetrahedral sites. HEAs therefore have potential as hydrogen storage materials because of favorable absorption in all interstitial sites within the structure. 2018 Journal Article http://hdl.handle.net/20.500.11937/71372 10.1021/acs.inorgchem.7b03004 American Chemical Society restricted
spellingShingle Karlsson, D.
Ek, G.
Cedervall, J.
Zlotea, C.
Moller, Kasper
Hansen, T.
Bednarcík, J.
Paskevicius, M.
Sørby, M.
Jensen, T.
Jansson, U.
Sahlberg, M.
Structure and Hydrogenation Properties of a HfNbTiVZr High-Entropy Alloy
title Structure and Hydrogenation Properties of a HfNbTiVZr High-Entropy Alloy
title_full Structure and Hydrogenation Properties of a HfNbTiVZr High-Entropy Alloy
title_fullStr Structure and Hydrogenation Properties of a HfNbTiVZr High-Entropy Alloy
title_full_unstemmed Structure and Hydrogenation Properties of a HfNbTiVZr High-Entropy Alloy
title_short Structure and Hydrogenation Properties of a HfNbTiVZr High-Entropy Alloy
title_sort structure and hydrogenation properties of a hfnbtivzr high-entropy alloy
url http://hdl.handle.net/20.500.11937/71372