Subgram-Scale Synthesis of Biomass Waste-Derived Fluorescent Carbon Dots in Subcritical Water for Bioimaging, Sensing, and Solid-State Patterning

Copyright © 2018 American Chemical Society. Fluorescent carbon dots (FCDs) have received considerable attention because of the great potential for a wide range of applications, from bioimaging to optoelectronic devices. In this work, we reported the synthesis of nitrogen-doped FCDs with an average s...

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Main Authors: Su, R., Wang, D., Liu, M., Yan, J., Wang, J., Zhan, Q., Pu, Y., Foster, Neil, Chen, J.
Format: Journal Article
Published: 2018
Online Access:http://hdl.handle.net/20.500.11937/71072
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author Su, R.
Wang, D.
Liu, M.
Yan, J.
Wang, J.
Zhan, Q.
Pu, Y.
Foster, Neil
Chen, J.
author_facet Su, R.
Wang, D.
Liu, M.
Yan, J.
Wang, J.
Zhan, Q.
Pu, Y.
Foster, Neil
Chen, J.
author_sort Su, R.
building Curtin Institutional Repository
collection Online Access
description Copyright © 2018 American Chemical Society. Fluorescent carbon dots (FCDs) have received considerable attention because of the great potential for a wide range of applications, from bioimaging to optoelectronic devices. In this work, we reported the synthesis of nitrogen-doped FCDs with an average size of 2 nm in a subcritical water apparatus by using biomass waste (i.e., expired milk) as the precursor. The obtained FCDs were highly dispersed in aqueous solution because of the presence of O-containing functional groups on their surfaces. Under the excitation of ultraviolet and blue light, the FCDs exhibited excitation wavelength-dependent fluorescence in the emission range of 400-550 nm. The FCDs could be easily taken up by HeLa cells without additional surface functionalization, serving as fluorescent nanoprobes for bioimaging. The applications of FCDs as sensing agents for the detection of Fe3+, solid-state fluorescent patterning, and transparent hybrid films were also performed, demonstrating their potential for solid-state fluorescent sensing, security labeling, and wearable optoelectronics.
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institution Curtin University Malaysia
institution_category Local University
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publishDate 2018
recordtype eprints
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spelling curtin-20.500.11937-710722018-12-13T09:32:38Z Subgram-Scale Synthesis of Biomass Waste-Derived Fluorescent Carbon Dots in Subcritical Water for Bioimaging, Sensing, and Solid-State Patterning Su, R. Wang, D. Liu, M. Yan, J. Wang, J. Zhan, Q. Pu, Y. Foster, Neil Chen, J. Copyright © 2018 American Chemical Society. Fluorescent carbon dots (FCDs) have received considerable attention because of the great potential for a wide range of applications, from bioimaging to optoelectronic devices. In this work, we reported the synthesis of nitrogen-doped FCDs with an average size of 2 nm in a subcritical water apparatus by using biomass waste (i.e., expired milk) as the precursor. The obtained FCDs were highly dispersed in aqueous solution because of the presence of O-containing functional groups on their surfaces. Under the excitation of ultraviolet and blue light, the FCDs exhibited excitation wavelength-dependent fluorescence in the emission range of 400-550 nm. The FCDs could be easily taken up by HeLa cells without additional surface functionalization, serving as fluorescent nanoprobes for bioimaging. The applications of FCDs as sensing agents for the detection of Fe3+, solid-state fluorescent patterning, and transparent hybrid films were also performed, demonstrating their potential for solid-state fluorescent sensing, security labeling, and wearable optoelectronics. 2018 Journal Article http://hdl.handle.net/20.500.11937/71072 10.1021/acsomega.8b01919 restricted
spellingShingle Su, R.
Wang, D.
Liu, M.
Yan, J.
Wang, J.
Zhan, Q.
Pu, Y.
Foster, Neil
Chen, J.
Subgram-Scale Synthesis of Biomass Waste-Derived Fluorescent Carbon Dots in Subcritical Water for Bioimaging, Sensing, and Solid-State Patterning
title Subgram-Scale Synthesis of Biomass Waste-Derived Fluorescent Carbon Dots in Subcritical Water for Bioimaging, Sensing, and Solid-State Patterning
title_full Subgram-Scale Synthesis of Biomass Waste-Derived Fluorescent Carbon Dots in Subcritical Water for Bioimaging, Sensing, and Solid-State Patterning
title_fullStr Subgram-Scale Synthesis of Biomass Waste-Derived Fluorescent Carbon Dots in Subcritical Water for Bioimaging, Sensing, and Solid-State Patterning
title_full_unstemmed Subgram-Scale Synthesis of Biomass Waste-Derived Fluorescent Carbon Dots in Subcritical Water for Bioimaging, Sensing, and Solid-State Patterning
title_short Subgram-Scale Synthesis of Biomass Waste-Derived Fluorescent Carbon Dots in Subcritical Water for Bioimaging, Sensing, and Solid-State Patterning
title_sort subgram-scale synthesis of biomass waste-derived fluorescent carbon dots in subcritical water for bioimaging, sensing, and solid-state patterning
url http://hdl.handle.net/20.500.11937/71072