Assessment of drinking water quality at the tap using fluorescence spectroscopy

© 2017 The Authors Treated drinking water may become contaminated while travelling in the distribution system on the way to consumers. Elevated dissolved organic matter (DOM) at the tap relative to the water leaving the treatment plant is a potential indicator of contamination, and can be measured s...

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Main Authors: Heibati, Masoumeh, Stedmon, C., Stenroth, K., Rauch, S., Toljander, J., Säve-Söderbergh, M., Murphy, K.
Format: Journal Article
Published: IWA Publishing 2017
Online Access:http://hdl.handle.net/20.500.11937/71017
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author Heibati, Masoumeh
Stedmon, C.
Stenroth, K.
Rauch, S.
Toljander, J.
Säve-Söderbergh, M.
Murphy, K.
author_facet Heibati, Masoumeh
Stedmon, C.
Stenroth, K.
Rauch, S.
Toljander, J.
Säve-Söderbergh, M.
Murphy, K.
author_sort Heibati, Masoumeh
building Curtin Institutional Repository
collection Online Access
description © 2017 The Authors Treated drinking water may become contaminated while travelling in the distribution system on the way to consumers. Elevated dissolved organic matter (DOM) at the tap relative to the water leaving the treatment plant is a potential indicator of contamination, and can be measured sensitively, inexpensively and potentially on-line via fluorescence and absorbance spectroscopy. Detecting elevated DOM requires potential contamination events to be distinguished from natural fluctuations in the system, but how much natural variation to expect in a stable distribution system is unknown. In this study, relationships between DOM optical properties, microbial indicator organisms and trace elements were investigated for households connected to a biologically-stable drinking water distribution system. Across the network, humic-like fluorescence intensities showed limited variation (RSD = 3.5–4.4%), with half of measured variation explained by interactions with copper. After accounting for quenching by copper, fluorescence provided a very stable background signal (RSD < 2.2%) against which a ~2% infiltration of soil water would be detectable. Smaller infiltrations would be detectable in the case of contamination by sewage with a strong tryptophan-like fluorescence signal. These findings indicate that DOM fluorescence is a sensitive indicator of water quality changes in drinking water networks, as long as potential interferents are taken into account.
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institution Curtin University Malaysia
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publishDate 2017
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spelling curtin-20.500.11937-710172018-12-13T09:33:29Z Assessment of drinking water quality at the tap using fluorescence spectroscopy Heibati, Masoumeh Stedmon, C. Stenroth, K. Rauch, S. Toljander, J. Säve-Söderbergh, M. Murphy, K. © 2017 The Authors Treated drinking water may become contaminated while travelling in the distribution system on the way to consumers. Elevated dissolved organic matter (DOM) at the tap relative to the water leaving the treatment plant is a potential indicator of contamination, and can be measured sensitively, inexpensively and potentially on-line via fluorescence and absorbance spectroscopy. Detecting elevated DOM requires potential contamination events to be distinguished from natural fluctuations in the system, but how much natural variation to expect in a stable distribution system is unknown. In this study, relationships between DOM optical properties, microbial indicator organisms and trace elements were investigated for households connected to a biologically-stable drinking water distribution system. Across the network, humic-like fluorescence intensities showed limited variation (RSD = 3.5–4.4%), with half of measured variation explained by interactions with copper. After accounting for quenching by copper, fluorescence provided a very stable background signal (RSD < 2.2%) against which a ~2% infiltration of soil water would be detectable. Smaller infiltrations would be detectable in the case of contamination by sewage with a strong tryptophan-like fluorescence signal. These findings indicate that DOM fluorescence is a sensitive indicator of water quality changes in drinking water networks, as long as potential interferents are taken into account. 2017 Journal Article http://hdl.handle.net/20.500.11937/71017 10.1016/j.watres.2017.08.020 IWA Publishing restricted
spellingShingle Heibati, Masoumeh
Stedmon, C.
Stenroth, K.
Rauch, S.
Toljander, J.
Säve-Söderbergh, M.
Murphy, K.
Assessment of drinking water quality at the tap using fluorescence spectroscopy
title Assessment of drinking water quality at the tap using fluorescence spectroscopy
title_full Assessment of drinking water quality at the tap using fluorescence spectroscopy
title_fullStr Assessment of drinking water quality at the tap using fluorescence spectroscopy
title_full_unstemmed Assessment of drinking water quality at the tap using fluorescence spectroscopy
title_short Assessment of drinking water quality at the tap using fluorescence spectroscopy
title_sort assessment of drinking water quality at the tap using fluorescence spectroscopy
url http://hdl.handle.net/20.500.11937/71017