One-pot, microwave-assisted synthesis of polymethylene-bridged bis(1H-1,2,4-triazol-5(3)-amines) and their tautomerism

© 2018 Elsevier Ltd A highly selective and efficient method for the synthesis of 3,3'(5,5')-polymethylene-bis(1H-1,2,4-triazol-5(3)-amines) was developed using the reaction of dicarboxylic acids and aminoguanidine in an aqueous medium. This one-pot, microwave-promoted method was proved to...

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Main Authors: Lim, F., Hu, L., Tiekink, E., Dolzhenko, Anton
Format: Journal Article
Published: Pergamon 2018
Online Access:http://hdl.handle.net/20.500.11937/70971
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author Lim, F.
Hu, L.
Tiekink, E.
Dolzhenko, Anton
author_facet Lim, F.
Hu, L.
Tiekink, E.
Dolzhenko, Anton
author_sort Lim, F.
building Curtin Institutional Repository
collection Online Access
description © 2018 Elsevier Ltd A highly selective and efficient method for the synthesis of 3,3'(5,5')-polymethylene-bis(1H-1,2,4-triazol-5(3)-amines) was developed using the reaction of dicarboxylic acids and aminoguanidine in an aqueous medium. This one-pot, microwave-promoted method was proved to be scalable affording the desired products in good yields and purity. The scope of the method was successfully explored by the preparation of a small library of polymethylene-bis(1H-1,2,4-triazol-5(3)-amines) with different alkyl chain linkers. The annular prototropic tautomerism in the prepared compounds was studied using NMR spectroscopy and X-ray crystallography.
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institution Curtin University Malaysia
institution_category Local University
last_indexed 2025-11-14T10:46:14Z
publishDate 2018
publisher Pergamon
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spelling curtin-20.500.11937-709712018-12-13T09:32:50Z One-pot, microwave-assisted synthesis of polymethylene-bridged bis(1H-1,2,4-triazol-5(3)-amines) and their tautomerism Lim, F. Hu, L. Tiekink, E. Dolzhenko, Anton © 2018 Elsevier Ltd A highly selective and efficient method for the synthesis of 3,3'(5,5')-polymethylene-bis(1H-1,2,4-triazol-5(3)-amines) was developed using the reaction of dicarboxylic acids and aminoguanidine in an aqueous medium. This one-pot, microwave-promoted method was proved to be scalable affording the desired products in good yields and purity. The scope of the method was successfully explored by the preparation of a small library of polymethylene-bis(1H-1,2,4-triazol-5(3)-amines) with different alkyl chain linkers. The annular prototropic tautomerism in the prepared compounds was studied using NMR spectroscopy and X-ray crystallography. 2018 Journal Article http://hdl.handle.net/20.500.11937/70971 10.1016/j.tetlet.2018.09.018 Pergamon restricted
spellingShingle Lim, F.
Hu, L.
Tiekink, E.
Dolzhenko, Anton
One-pot, microwave-assisted synthesis of polymethylene-bridged bis(1H-1,2,4-triazol-5(3)-amines) and their tautomerism
title One-pot, microwave-assisted synthesis of polymethylene-bridged bis(1H-1,2,4-triazol-5(3)-amines) and their tautomerism
title_full One-pot, microwave-assisted synthesis of polymethylene-bridged bis(1H-1,2,4-triazol-5(3)-amines) and their tautomerism
title_fullStr One-pot, microwave-assisted synthesis of polymethylene-bridged bis(1H-1,2,4-triazol-5(3)-amines) and their tautomerism
title_full_unstemmed One-pot, microwave-assisted synthesis of polymethylene-bridged bis(1H-1,2,4-triazol-5(3)-amines) and their tautomerism
title_short One-pot, microwave-assisted synthesis of polymethylene-bridged bis(1H-1,2,4-triazol-5(3)-amines) and their tautomerism
title_sort one-pot, microwave-assisted synthesis of polymethylene-bridged bis(1h-1,2,4-triazol-5(3)-amines) and their tautomerism
url http://hdl.handle.net/20.500.11937/70971