A novel way to improve performance of proton-conducting solid-oxide fuel cells through enhanced chemical interaction of anode components

We proposed a novel way to improve the cell performance of proton-conducting solid-oxide fuel cells by increasing the chemical interaction between the anode components using BaZr0.4Ce0.4Y 0.2O3-d (BZCY4) as the ionic conducting phase of anode for a fuel cell with a BaCe0.8Y0.2O 3-d (BCY) electrolyte...

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Main Authors: Guo, Y., Ran, R., Shao, Zongping
Format: Journal Article
Published: 2011
Online Access:http://hdl.handle.net/20.500.11937/6795
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author Guo, Y.
Ran, R.
Shao, Zongping
author_facet Guo, Y.
Ran, R.
Shao, Zongping
author_sort Guo, Y.
building Curtin Institutional Repository
collection Online Access
description We proposed a novel way to improve the cell performance of proton-conducting solid-oxide fuel cells by increasing the chemical interaction between the anode components using BaZr0.4Ce0.4Y 0.2O3-d (BZCY4) as the ionic conducting phase of anode for a fuel cell with a BaCe0.8Y0.2O 3-d (BCY) electrolyte. The strength of the chemical interaction between NiO and the ionic conducting phase (BZCY4 or BCY) was analyzed by the hydrogen temperature-programmed reduction (H2-TPR) technique. The effect of chemical interaction between NiO and the ionic conducting phase on the NiO diffusivity was investigated by SEM-EDX. The results demonstrated NiO had a much stronger interaction with BZCY4 than with BCY, thereby resulting in suppressed diffusivity of NiO into the BCY electrolyte. Using BZCY4 as the ionic conducting phase of the anode, a cell with an ohmic resistance of 0.65 O cm2 at 700 °C was obtained. In contrast, a cell with BCY as the ionic conducting phase of the anode had an ohmic resistance of 0.82 O cm2 at 700 °C. Therefore, the single cell with NiO + BZCY4 anode showed a peak power density higher than that of the cell with the NiO + BCY anode. © 2010 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved.
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spelling curtin-20.500.11937-67952017-09-13T14:37:01Z A novel way to improve performance of proton-conducting solid-oxide fuel cells through enhanced chemical interaction of anode components Guo, Y. Ran, R. Shao, Zongping We proposed a novel way to improve the cell performance of proton-conducting solid-oxide fuel cells by increasing the chemical interaction between the anode components using BaZr0.4Ce0.4Y 0.2O3-d (BZCY4) as the ionic conducting phase of anode for a fuel cell with a BaCe0.8Y0.2O 3-d (BCY) electrolyte. The strength of the chemical interaction between NiO and the ionic conducting phase (BZCY4 or BCY) was analyzed by the hydrogen temperature-programmed reduction (H2-TPR) technique. The effect of chemical interaction between NiO and the ionic conducting phase on the NiO diffusivity was investigated by SEM-EDX. The results demonstrated NiO had a much stronger interaction with BZCY4 than with BCY, thereby resulting in suppressed diffusivity of NiO into the BCY electrolyte. Using BZCY4 as the ionic conducting phase of the anode, a cell with an ohmic resistance of 0.65 O cm2 at 700 °C was obtained. In contrast, a cell with BCY as the ionic conducting phase of the anode had an ohmic resistance of 0.82 O cm2 at 700 °C. Therefore, the single cell with NiO + BZCY4 anode showed a peak power density higher than that of the cell with the NiO + BCY anode. © 2010 Professor T. Nejat Veziroglu. Published by Elsevier Ltd. All rights reserved. 2011 Journal Article http://hdl.handle.net/20.500.11937/6795 10.1016/j.ijhydene.2010.10.081 restricted
spellingShingle Guo, Y.
Ran, R.
Shao, Zongping
A novel way to improve performance of proton-conducting solid-oxide fuel cells through enhanced chemical interaction of anode components
title A novel way to improve performance of proton-conducting solid-oxide fuel cells through enhanced chemical interaction of anode components
title_full A novel way to improve performance of proton-conducting solid-oxide fuel cells through enhanced chemical interaction of anode components
title_fullStr A novel way to improve performance of proton-conducting solid-oxide fuel cells through enhanced chemical interaction of anode components
title_full_unstemmed A novel way to improve performance of proton-conducting solid-oxide fuel cells through enhanced chemical interaction of anode components
title_short A novel way to improve performance of proton-conducting solid-oxide fuel cells through enhanced chemical interaction of anode components
title_sort novel way to improve performance of proton-conducting solid-oxide fuel cells through enhanced chemical interaction of anode components
url http://hdl.handle.net/20.500.11937/6795