Tracing bottom water oxygenation with sedimentary Mn/Fe ratios in Lake Zurich, Switzerland

Redox dynamics of manganese (Mn) were studied in the sediment of Lake Zurich using precise sediment core age models, monthly long-term oxygen (O2) monitoring data of the water column (1936–2010) and high-resolution XRF core scanning. The age models were based on bi-annual lamination and calcite prec...

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Main Authors: Naeher, Sebastian, Gilli, A., North, R., Hamann, Y., Schubert, C.
Format: Journal Article
Published: Elsevier Science BV 2013
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/6669
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author Naeher, Sebastian
Gilli, A.
North, R.
Hamann, Y.
Schubert, C.
author_facet Naeher, Sebastian
Gilli, A.
North, R.
Hamann, Y.
Schubert, C.
author_sort Naeher, Sebastian
building Curtin Institutional Repository
collection Online Access
description Redox dynamics of manganese (Mn) were studied in the sediment of Lake Zurich using precise sediment core age models, monthly long-term oxygen (O2) monitoring data of the water column (1936–2010) and high-resolution XRF core scanning. The age models were based on bi-annual lamination and calcite precipitation cycles. If present, Mn exhibits distinct maxima, which coincide with the annual maximum deep-water O2 concentrations in spring according to the monitoring data. In contrast, the iron (Fe) signal is mainly the result of calcite dilution, as indicated by a strong negative correlation between Fe and calcium (Ca) XRF data. The Mn/Fe ratio in the core from the maximum lake depth (ZH10-15, 137 m) revealed a moderate correlation with O2 measurements in the lake bottom water confirming the successful application of the Mn/Fe ratio to semi-quantitatively reconstruct bottom water oxygenation in the lake. Mostly low ratios were observed between 1895 and the mid-1960s as a result of eutrophication. However, geochemical focusing and sedimentological factors can reduce the applicability of the Mn/Fe ratio in reconstructing O2 concentrations in the bottom water of lakes.
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spelling curtin-20.500.11937-66692017-09-13T16:02:38Z Tracing bottom water oxygenation with sedimentary Mn/Fe ratios in Lake Zurich, Switzerland Naeher, Sebastian Gilli, A. North, R. Hamann, Y. Schubert, C. Oxygen Redox Mn/Fe ratio XRF core scanning Lake Zurich Manganese Redox dynamics of manganese (Mn) were studied in the sediment of Lake Zurich using precise sediment core age models, monthly long-term oxygen (O2) monitoring data of the water column (1936–2010) and high-resolution XRF core scanning. The age models were based on bi-annual lamination and calcite precipitation cycles. If present, Mn exhibits distinct maxima, which coincide with the annual maximum deep-water O2 concentrations in spring according to the monitoring data. In contrast, the iron (Fe) signal is mainly the result of calcite dilution, as indicated by a strong negative correlation between Fe and calcium (Ca) XRF data. The Mn/Fe ratio in the core from the maximum lake depth (ZH10-15, 137 m) revealed a moderate correlation with O2 measurements in the lake bottom water confirming the successful application of the Mn/Fe ratio to semi-quantitatively reconstruct bottom water oxygenation in the lake. Mostly low ratios were observed between 1895 and the mid-1960s as a result of eutrophication. However, geochemical focusing and sedimentological factors can reduce the applicability of the Mn/Fe ratio in reconstructing O2 concentrations in the bottom water of lakes. 2013 Journal Article http://hdl.handle.net/20.500.11937/6669 10.1016/j.chemgeo.2013.06.006 Elsevier Science BV restricted
spellingShingle Oxygen
Redox
Mn/Fe ratio
XRF core scanning
Lake Zurich
Manganese
Naeher, Sebastian
Gilli, A.
North, R.
Hamann, Y.
Schubert, C.
Tracing bottom water oxygenation with sedimentary Mn/Fe ratios in Lake Zurich, Switzerland
title Tracing bottom water oxygenation with sedimentary Mn/Fe ratios in Lake Zurich, Switzerland
title_full Tracing bottom water oxygenation with sedimentary Mn/Fe ratios in Lake Zurich, Switzerland
title_fullStr Tracing bottom water oxygenation with sedimentary Mn/Fe ratios in Lake Zurich, Switzerland
title_full_unstemmed Tracing bottom water oxygenation with sedimentary Mn/Fe ratios in Lake Zurich, Switzerland
title_short Tracing bottom water oxygenation with sedimentary Mn/Fe ratios in Lake Zurich, Switzerland
title_sort tracing bottom water oxygenation with sedimentary mn/fe ratios in lake zurich, switzerland
topic Oxygen
Redox
Mn/Fe ratio
XRF core scanning
Lake Zurich
Manganese
url http://hdl.handle.net/20.500.11937/6669