Activated alumina-based adsorption and recovery of excess fluoride ions subsequent to calcium and magnesium removal in base metal leach circuits

An effective electrowinning process in hydrometallurgical industry requires fluoride levels in the base metal solution to be less than 10 mg/l. Selective removal of the fluoride ions from base solution isthus desired, if fluoride was added to control calcium and magnesium in the circuit. Consequentl...

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Main Authors: Lorenzen, L., Eksteen, Jacques, Pelser, M., Aldrich, Chris, Georgalli, G.
Format: Journal Article
Published: Southern African Institute of Mining and Metallurgy 2009
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/6610
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author Lorenzen, L.
Eksteen, Jacques
Pelser, M.
Aldrich, Chris
Georgalli, G.
author_facet Lorenzen, L.
Eksteen, Jacques
Pelser, M.
Aldrich, Chris
Georgalli, G.
author_sort Lorenzen, L.
building Curtin Institutional Repository
collection Online Access
description An effective electrowinning process in hydrometallurgical industry requires fluoride levels in the base metal solution to be less than 10 mg/l. Selective removal of the fluoride ions from base solution isthus desired, if fluoride was added to control calcium and magnesium in the circuit. Consequently, adsorption of fluoride onto activated alumina was studied in a batch and a column set-up. Theeffects of base metal solution pH, temperature, initial concentration and flow rate on activated alumina performance were investigated in either a batch or column configuration. A two-level factorialexperimental design was implemented in studying column dynamics. Results demonstrate that activated alumina is an effective adsorbent for selective removal of fluoride from base solution. In the batch operation, fluoride was removed to values below the maximum allowable concentration (10 mg/l) when pH was = 8. In the column adsorption step at 55°C and 600mg/l initial concentration, up to 16 bed volumes were processed before breakthrough level was reached. Desorption step using 1% sodiumhydroxide solution achieved an elution of 8 bed volumes. The activated alumina (AA) had a capacity of 8.65 gF/l AA at the 10 mgF/l fluoride breakthrough level during the column adsorption test.
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spelling curtin-20.500.11937-66102017-02-28T01:30:59Z Activated alumina-based adsorption and recovery of excess fluoride ions subsequent to calcium and magnesium removal in base metal leach circuits Lorenzen, L. Eksteen, Jacques Pelser, M. Aldrich, Chris Georgalli, G. regeneration Fluoride activated alumina adsorption recovery An effective electrowinning process in hydrometallurgical industry requires fluoride levels in the base metal solution to be less than 10 mg/l. Selective removal of the fluoride ions from base solution isthus desired, if fluoride was added to control calcium and magnesium in the circuit. Consequently, adsorption of fluoride onto activated alumina was studied in a batch and a column set-up. Theeffects of base metal solution pH, temperature, initial concentration and flow rate on activated alumina performance were investigated in either a batch or column configuration. A two-level factorialexperimental design was implemented in studying column dynamics. Results demonstrate that activated alumina is an effective adsorbent for selective removal of fluoride from base solution. In the batch operation, fluoride was removed to values below the maximum allowable concentration (10 mg/l) when pH was = 8. In the column adsorption step at 55°C and 600mg/l initial concentration, up to 16 bed volumes were processed before breakthrough level was reached. Desorption step using 1% sodiumhydroxide solution achieved an elution of 8 bed volumes. The activated alumina (AA) had a capacity of 8.65 gF/l AA at the 10 mgF/l fluoride breakthrough level during the column adsorption test. 2009 Journal Article http://hdl.handle.net/20.500.11937/6610 Southern African Institute of Mining and Metallurgy restricted
spellingShingle regeneration
Fluoride
activated alumina
adsorption
recovery
Lorenzen, L.
Eksteen, Jacques
Pelser, M.
Aldrich, Chris
Georgalli, G.
Activated alumina-based adsorption and recovery of excess fluoride ions subsequent to calcium and magnesium removal in base metal leach circuits
title Activated alumina-based adsorption and recovery of excess fluoride ions subsequent to calcium and magnesium removal in base metal leach circuits
title_full Activated alumina-based adsorption and recovery of excess fluoride ions subsequent to calcium and magnesium removal in base metal leach circuits
title_fullStr Activated alumina-based adsorption and recovery of excess fluoride ions subsequent to calcium and magnesium removal in base metal leach circuits
title_full_unstemmed Activated alumina-based adsorption and recovery of excess fluoride ions subsequent to calcium and magnesium removal in base metal leach circuits
title_short Activated alumina-based adsorption and recovery of excess fluoride ions subsequent to calcium and magnesium removal in base metal leach circuits
title_sort activated alumina-based adsorption and recovery of excess fluoride ions subsequent to calcium and magnesium removal in base metal leach circuits
topic regeneration
Fluoride
activated alumina
adsorption
recovery
url http://hdl.handle.net/20.500.11937/6610