Preparation and characterisation of poly(vinyl) alcohol (PVA)/starch (ST)/halloysite nanotube (HNT) nanocomposite films as renewable materials

Poly(vinyl) alcohol (PVA)/starch (ST) films (weight ratio: 80/20) were prepared using a solution casting method, in the presence of 30 wt% glycerol (GL) as a plasticiser. Halloysite nanotubes (HNTs) were used as relatively new clay nanofillers to PVA/ST/GL blends for more economical material packagi...

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Main Authors: Abdullah, Zainab, Dong, Yu
Format: Journal Article
Published: Springer 2018
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/63440
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author Abdullah, Zainab
Dong, Yu
author_facet Abdullah, Zainab
Dong, Yu
author_sort Abdullah, Zainab
building Curtin Institutional Repository
collection Online Access
description Poly(vinyl) alcohol (PVA)/starch (ST) films (weight ratio: 80/20) were prepared using a solution casting method, in the presence of 30 wt% glycerol (GL) as a plasticiser. Halloysite nanotubes (HNTs) were used as relatively new clay nanofillers to PVA/ST/GL blends for more economical material packaging. HNTs at filler loadings of 0.25, 0.5, 1, 3 and 5 wt% were incorporated to enhance mechanical and thermal properties of resulting PVA/ST/HNT nanocomposites. The tensile strength of such nanocomposites was found to be improved by 20 and 3.4%, respectively, with the inclusion of 0.25 and 0.5 wt% HNTs as opposed to those of PVA/ST/GL blends. However, a decreasing strength trend was observed beyond the HNT loading of 0.5 wt% due to HNT agglomeration, as evidenced by relevant micrographs via scanning electron microscopy (SEM). However, Young’s modulus was enhanced by 148% with the addition of 1 wt% HNTs when compared with PVA/ST/GL blends. X-ray diffraction (XRD) analysis is indicative of slightly intercalated nanocomposite structures formed at low HNT loadings of 0.25–1 wt%. In general, the incorporation of HNTs improved the thermal stability of PVA/ST/GL blends by increasing melting and decomposition temperatures along with the reduction in weight loss.
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spelling curtin-20.500.11937-634402019-02-19T05:36:20Z Preparation and characterisation of poly(vinyl) alcohol (PVA)/starch (ST)/halloysite nanotube (HNT) nanocomposite films as renewable materials Abdullah, Zainab Dong, Yu Blends Nanocomposites Mechanical properties Poly(vinyl) alcohol (PVA)/starch (ST) films (weight ratio: 80/20) were prepared using a solution casting method, in the presence of 30 wt% glycerol (GL) as a plasticiser. Halloysite nanotubes (HNTs) were used as relatively new clay nanofillers to PVA/ST/GL blends for more economical material packaging. HNTs at filler loadings of 0.25, 0.5, 1, 3 and 5 wt% were incorporated to enhance mechanical and thermal properties of resulting PVA/ST/HNT nanocomposites. The tensile strength of such nanocomposites was found to be improved by 20 and 3.4%, respectively, with the inclusion of 0.25 and 0.5 wt% HNTs as opposed to those of PVA/ST/GL blends. However, a decreasing strength trend was observed beyond the HNT loading of 0.5 wt% due to HNT agglomeration, as evidenced by relevant micrographs via scanning electron microscopy (SEM). However, Young’s modulus was enhanced by 148% with the addition of 1 wt% HNTs when compared with PVA/ST/GL blends. X-ray diffraction (XRD) analysis is indicative of slightly intercalated nanocomposite structures formed at low HNT loadings of 0.25–1 wt%. In general, the incorporation of HNTs improved the thermal stability of PVA/ST/GL blends by increasing melting and decomposition temperatures along with the reduction in weight loss. 2018 Journal Article http://hdl.handle.net/20.500.11937/63440 10.1007/s10853-017-1812-0 Springer fulltext
spellingShingle Blends
Nanocomposites
Mechanical properties
Abdullah, Zainab
Dong, Yu
Preparation and characterisation of poly(vinyl) alcohol (PVA)/starch (ST)/halloysite nanotube (HNT) nanocomposite films as renewable materials
title Preparation and characterisation of poly(vinyl) alcohol (PVA)/starch (ST)/halloysite nanotube (HNT) nanocomposite films as renewable materials
title_full Preparation and characterisation of poly(vinyl) alcohol (PVA)/starch (ST)/halloysite nanotube (HNT) nanocomposite films as renewable materials
title_fullStr Preparation and characterisation of poly(vinyl) alcohol (PVA)/starch (ST)/halloysite nanotube (HNT) nanocomposite films as renewable materials
title_full_unstemmed Preparation and characterisation of poly(vinyl) alcohol (PVA)/starch (ST)/halloysite nanotube (HNT) nanocomposite films as renewable materials
title_short Preparation and characterisation of poly(vinyl) alcohol (PVA)/starch (ST)/halloysite nanotube (HNT) nanocomposite films as renewable materials
title_sort preparation and characterisation of poly(vinyl) alcohol (pva)/starch (st)/halloysite nanotube (hnt) nanocomposite films as renewable materials
topic Blends
Nanocomposites
Mechanical properties
url http://hdl.handle.net/20.500.11937/63440