Microfluidic extraction of copper from particle-laden solutions

Microfluidic solvent extraction (SX) of metal ions from particle-laden aqueous solutions is demonstrated as an alternative to conventional solvent extraction for a system of industrial interest: extraction of Cu2+ using 2-hydroxy-5-nonylacetophenone. In the presence of silica nanoparticles, bulk SX...

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Main Authors: Priest, C., Zhou, J., Sedev, Rossen, Ralston, J., Aota, A., Mawatari, K., Kitamori, T.
Format: Journal Article
Published: Elsevier 2011
Online Access:http://hdl.handle.net/20.500.11937/63363
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author Priest, C.
Zhou, J.
Sedev, Rossen
Ralston, J.
Aota, A.
Mawatari, K.
Kitamori, T.
author_facet Priest, C.
Zhou, J.
Sedev, Rossen
Ralston, J.
Aota, A.
Mawatari, K.
Kitamori, T.
author_sort Priest, C.
building Curtin Institutional Repository
collection Online Access
description Microfluidic solvent extraction (SX) of metal ions from particle-laden aqueous solutions is demonstrated as an alternative to conventional solvent extraction for a system of industrial interest: extraction of Cu2+ using 2-hydroxy-5-nonylacetophenone. In the presence of silica nanoparticles, bulk SX suffers from prolonged phase separation and, for hydrophobic particles, the formation of particle-stabilised emulsions, which can be indefinitely stable, leading to significant losses of valuable materials to the emulsion phase. In contrast, non-dispersive microfluidic SX can process fluids containing high particle concentrations (e.g. 61 g/L, 80 nm hydrophilic silica and 5 g/L, and 13 nm moderately hydrophobic silica). The SX was operated continuously for more than 7 h without blockage or failure of the microfluidic chip, in part due to the very short residence time of the silica nanoparticles in the aqueous phase. The microfluidic method is also able to access extraction kinetics for particle-laden systems, which cannot be obtained otherwise due to delayed phase separation. © 2010 Published by Elsevier B.V. All rights reserved.
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institution Curtin University Malaysia
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spelling curtin-20.500.11937-633632018-02-06T07:40:07Z Microfluidic extraction of copper from particle-laden solutions Priest, C. Zhou, J. Sedev, Rossen Ralston, J. Aota, A. Mawatari, K. Kitamori, T. Microfluidic solvent extraction (SX) of metal ions from particle-laden aqueous solutions is demonstrated as an alternative to conventional solvent extraction for a system of industrial interest: extraction of Cu2+ using 2-hydroxy-5-nonylacetophenone. In the presence of silica nanoparticles, bulk SX suffers from prolonged phase separation and, for hydrophobic particles, the formation of particle-stabilised emulsions, which can be indefinitely stable, leading to significant losses of valuable materials to the emulsion phase. In contrast, non-dispersive microfluidic SX can process fluids containing high particle concentrations (e.g. 61 g/L, 80 nm hydrophilic silica and 5 g/L, and 13 nm moderately hydrophobic silica). The SX was operated continuously for more than 7 h without blockage or failure of the microfluidic chip, in part due to the very short residence time of the silica nanoparticles in the aqueous phase. The microfluidic method is also able to access extraction kinetics for particle-laden systems, which cannot be obtained otherwise due to delayed phase separation. © 2010 Published by Elsevier B.V. All rights reserved. 2011 Journal Article http://hdl.handle.net/20.500.11937/63363 10.1016/j.minpro.2010.11.005 Elsevier restricted
spellingShingle Priest, C.
Zhou, J.
Sedev, Rossen
Ralston, J.
Aota, A.
Mawatari, K.
Kitamori, T.
Microfluidic extraction of copper from particle-laden solutions
title Microfluidic extraction of copper from particle-laden solutions
title_full Microfluidic extraction of copper from particle-laden solutions
title_fullStr Microfluidic extraction of copper from particle-laden solutions
title_full_unstemmed Microfluidic extraction of copper from particle-laden solutions
title_short Microfluidic extraction of copper from particle-laden solutions
title_sort microfluidic extraction of copper from particle-laden solutions
url http://hdl.handle.net/20.500.11937/63363