Development of a kinetic model for Fischer-Tropsch synthesis over a Ru promoted Co/Al2O3 catalyst in a slurry reactor

A detailed kinetic model for hydrocarbon formation rate over a wide range of operating conditions by using a stirred tank slurry reactor (STSR), which closely mimics the kinetics of the commercialized slurry process, is put forward. Kinetics of the Fischer-Tropsch (F-T) synthesis over 0.27% Ru 25% C...

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Main Authors: Bhatelia, Tejas, Ma, W., Jacobs, G., Davis, B., Bukur, D.
Format: Conference Paper
Published: 2011
Online Access:http://hdl.handle.net/20.500.11937/62363
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author Bhatelia, Tejas
Ma, W.
Jacobs, G.
Davis, B.
Bukur, D.
author_facet Bhatelia, Tejas
Ma, W.
Jacobs, G.
Davis, B.
Bukur, D.
author_sort Bhatelia, Tejas
building Curtin Institutional Repository
collection Online Access
description A detailed kinetic model for hydrocarbon formation rate over a wide range of operating conditions by using a stirred tank slurry reactor (STSR), which closely mimics the kinetics of the commercialized slurry process, is put forward. Kinetics of the Fischer-Tropsch (F-T) synthesis over 0.27% Ru 25% Co/Al 2 O 3 catalyst was studied using the STSR. Hydrogen-assisted dissociative adsorption of CO followed by hydrogenation of dissociatively adsorbed CO was the likely path for formation of the monomer (methylene) and was the likely rate controlling step in F-T synthesis. Rates obtained from the best kinetic model provided a satisfactory fit to the experimental data. This is an abstract of a paper presented at the 2011 AIChE Spring Meeting & 7th Global Congress on Process Safety (Chicago, IL 3/13-17/2011).
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institution Curtin University Malaysia
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spelling curtin-20.500.11937-623632018-12-14T01:02:02Z Development of a kinetic model for Fischer-Tropsch synthesis over a Ru promoted Co/Al2O3 catalyst in a slurry reactor Bhatelia, Tejas Ma, W. Jacobs, G. Davis, B. Bukur, D. A detailed kinetic model for hydrocarbon formation rate over a wide range of operating conditions by using a stirred tank slurry reactor (STSR), which closely mimics the kinetics of the commercialized slurry process, is put forward. Kinetics of the Fischer-Tropsch (F-T) synthesis over 0.27% Ru 25% Co/Al 2 O 3 catalyst was studied using the STSR. Hydrogen-assisted dissociative adsorption of CO followed by hydrogenation of dissociatively adsorbed CO was the likely path for formation of the monomer (methylene) and was the likely rate controlling step in F-T synthesis. Rates obtained from the best kinetic model provided a satisfactory fit to the experimental data. This is an abstract of a paper presented at the 2011 AIChE Spring Meeting & 7th Global Congress on Process Safety (Chicago, IL 3/13-17/2011). 2011 Conference Paper http://hdl.handle.net/20.500.11937/62363 restricted
spellingShingle Bhatelia, Tejas
Ma, W.
Jacobs, G.
Davis, B.
Bukur, D.
Development of a kinetic model for Fischer-Tropsch synthesis over a Ru promoted Co/Al2O3 catalyst in a slurry reactor
title Development of a kinetic model for Fischer-Tropsch synthesis over a Ru promoted Co/Al2O3 catalyst in a slurry reactor
title_full Development of a kinetic model for Fischer-Tropsch synthesis over a Ru promoted Co/Al2O3 catalyst in a slurry reactor
title_fullStr Development of a kinetic model for Fischer-Tropsch synthesis over a Ru promoted Co/Al2O3 catalyst in a slurry reactor
title_full_unstemmed Development of a kinetic model for Fischer-Tropsch synthesis over a Ru promoted Co/Al2O3 catalyst in a slurry reactor
title_short Development of a kinetic model for Fischer-Tropsch synthesis over a Ru promoted Co/Al2O3 catalyst in a slurry reactor
title_sort development of a kinetic model for fischer-tropsch synthesis over a ru promoted co/al2o3 catalyst in a slurry reactor
url http://hdl.handle.net/20.500.11937/62363