Determination of the new anthelmintic monepantel and its sulfone metabolite in milk and muscle using a UHPLC-MS/MS and QuEChERS method

This is the first paper to report a method for the detection of the new anthelmintic monepantel and its sulfone metabolite in goat's milk and ovine muscle. Samples were extracted and purified using a modified QuEChERS method. A concentration step was included when analyzing in the low μgkg -1...

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Main Authors: Kinsella, Brian, Byrne, P., Cantwell, H., McCormack, M., Furey, A., Danaher, M.
Format: Journal Article
Published: Elsevier BV 2011
Online Access:http://hdl.handle.net/20.500.11937/61682
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author Kinsella, Brian
Byrne, P.
Cantwell, H.
McCormack, M.
Furey, A.
Danaher, M.
author_facet Kinsella, Brian
Byrne, P.
Cantwell, H.
McCormack, M.
Furey, A.
Danaher, M.
author_sort Kinsella, Brian
building Curtin Institutional Repository
collection Online Access
description This is the first paper to report a method for the detection of the new anthelmintic monepantel and its sulfone metabolite in goat's milk and ovine muscle. Samples were extracted and purified using a modified QuEChERS method. A concentration step was included when analyzing in the low μgkg -1 range. Analysis was carried out by ultra high performance liquid chromatography-tandem mass spectrometry (UHPLC-MS/MS) in a 13min run time using atmospheric pressure electrospray ionisation in the negative mode (ESI - ) and multiple reaction monitoring (MRM) scanning. Monepantel (m/z 472) and monepantel-sulfone (m/z 504) both had product ions at m/z 186 and m/z 166. The method has been single-laboratory validated according to the 2002/657/EC guidelines. The mean recovery in milk was 108 and 106% for monepantel and monepantel-sulfone, respectively. The mean recovery in muscle was 109 and 108% for monepantel and monepantel-sulfone, respectively. The coefficients of variation for the within laboratory repeatability and reproducibility were ≤6.4% in milk and ≤14.2% in muscle. The decision limits (CCα) in milk were 2.20 and 2.08μgkg -1 for monepantel and monepantel-sulfone, respectively. The decision limits (CCα) in muscle were 771 and 746μgkg -1 for monepantel and monepantel-sulfone, respectively. © 2011 Elsevier B.V.
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spelling curtin-20.500.11937-616822018-02-01T05:57:06Z Determination of the new anthelmintic monepantel and its sulfone metabolite in milk and muscle using a UHPLC-MS/MS and QuEChERS method Kinsella, Brian Byrne, P. Cantwell, H. McCormack, M. Furey, A. Danaher, M. This is the first paper to report a method for the detection of the new anthelmintic monepantel and its sulfone metabolite in goat's milk and ovine muscle. Samples were extracted and purified using a modified QuEChERS method. A concentration step was included when analyzing in the low μgkg -1 range. Analysis was carried out by ultra high performance liquid chromatography-tandem mass spectrometry (UHPLC-MS/MS) in a 13min run time using atmospheric pressure electrospray ionisation in the negative mode (ESI - ) and multiple reaction monitoring (MRM) scanning. Monepantel (m/z 472) and monepantel-sulfone (m/z 504) both had product ions at m/z 186 and m/z 166. The method has been single-laboratory validated according to the 2002/657/EC guidelines. The mean recovery in milk was 108 and 106% for monepantel and monepantel-sulfone, respectively. The mean recovery in muscle was 109 and 108% for monepantel and monepantel-sulfone, respectively. The coefficients of variation for the within laboratory repeatability and reproducibility were ≤6.4% in milk and ≤14.2% in muscle. The decision limits (CCα) in milk were 2.20 and 2.08μgkg -1 for monepantel and monepantel-sulfone, respectively. The decision limits (CCα) in muscle were 771 and 746μgkg -1 for monepantel and monepantel-sulfone, respectively. © 2011 Elsevier B.V. 2011 Journal Article http://hdl.handle.net/20.500.11937/61682 10.1016/j.jchromb.2011.10.011 Elsevier BV restricted
spellingShingle Kinsella, Brian
Byrne, P.
Cantwell, H.
McCormack, M.
Furey, A.
Danaher, M.
Determination of the new anthelmintic monepantel and its sulfone metabolite in milk and muscle using a UHPLC-MS/MS and QuEChERS method
title Determination of the new anthelmintic monepantel and its sulfone metabolite in milk and muscle using a UHPLC-MS/MS and QuEChERS method
title_full Determination of the new anthelmintic monepantel and its sulfone metabolite in milk and muscle using a UHPLC-MS/MS and QuEChERS method
title_fullStr Determination of the new anthelmintic monepantel and its sulfone metabolite in milk and muscle using a UHPLC-MS/MS and QuEChERS method
title_full_unstemmed Determination of the new anthelmintic monepantel and its sulfone metabolite in milk and muscle using a UHPLC-MS/MS and QuEChERS method
title_short Determination of the new anthelmintic monepantel and its sulfone metabolite in milk and muscle using a UHPLC-MS/MS and QuEChERS method
title_sort determination of the new anthelmintic monepantel and its sulfone metabolite in milk and muscle using a uhplc-ms/ms and quechers method
url http://hdl.handle.net/20.500.11937/61682