Impact of Solid Surface Energy on Wettability of CO2-brine-Mineral Systems as a Function of Pressure, Temperature and Salinity

CO 2 storage refers to the methods employed to inject CO 2 in depleted oil and gas reservoirs and deep saline aquifers for long term storage of CO 2 with the objective to reduce the anthropogenic CO 2 emissions. Wettability and interfacial tension are two important multiphase parameters which ar...

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Main Authors: Arif, Muhammad, Barifcani, Ahmed, Lebedev, Maxim, Iglauer, Stefan
Format: Conference Paper
Published: 2017
Online Access:http://hdl.handle.net/20.500.11937/58044
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author Arif, Muhammad
Barifcani, Ahmed
Lebedev, Maxim
Iglauer, Stefan
author_facet Arif, Muhammad
Barifcani, Ahmed
Lebedev, Maxim
Iglauer, Stefan
author_sort Arif, Muhammad
building Curtin Institutional Repository
collection Online Access
description CO 2 storage refers to the methods employed to inject CO 2 in depleted oil and gas reservoirs and deep saline aquifers for long term storage of CO 2 with the objective to reduce the anthropogenic CO 2 emissions. Wettability and interfacial tension are two important multiphase parameters which are used to characterize the flow behavior of CO 2 in reservoirs. Numerous studies have reported wettability data of CO 2 -brine systems on various rock forming minerals as function of pressure, temperature and salinity. However, the associated trends have not been physically well-understood and require considerable attention which is objective of our present work. In this work, we apply Neumann's equation of state method to our measured contact angle data for CO 2 -brine-mica systems and contact angle data of CO 2 -brine-quartz from Sarmadivaleh et al., 2015. Our results indicate that for mica, solid-CO 2 interfacial tension decrease with pressure and salinity and increase with temperature. Moreover, solid-liquid interfacial tension decrease with temperature and decrease with salinity. For quartz, although the solid-CO 2 interfacial tension decrease with pressure and increase with temperature, yet solid-liquid interfacial tension increase with temperature which explains the increase in contact angle with temperature for quartz. Overall, we find that results are in accordance with wettability data as function of pressure, temperature and salinity. We thus conclude that hotter reservoirs with lower injection pressure and lower brine salinities exhibit relatively better water wetting state and hence better seal capacity leading to higher CO 2 storage potential. We also conclude that solid surface energy approach adequately explains the dependency of wettability on pressure, temperature and salinity.
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spelling curtin-20.500.11937-580442018-01-10T07:20:45Z Impact of Solid Surface Energy on Wettability of CO2-brine-Mineral Systems as a Function of Pressure, Temperature and Salinity Arif, Muhammad Barifcani, Ahmed Lebedev, Maxim Iglauer, Stefan CO 2 storage refers to the methods employed to inject CO 2 in depleted oil and gas reservoirs and deep saline aquifers for long term storage of CO 2 with the objective to reduce the anthropogenic CO 2 emissions. Wettability and interfacial tension are two important multiphase parameters which are used to characterize the flow behavior of CO 2 in reservoirs. Numerous studies have reported wettability data of CO 2 -brine systems on various rock forming minerals as function of pressure, temperature and salinity. However, the associated trends have not been physically well-understood and require considerable attention which is objective of our present work. In this work, we apply Neumann's equation of state method to our measured contact angle data for CO 2 -brine-mica systems and contact angle data of CO 2 -brine-quartz from Sarmadivaleh et al., 2015. Our results indicate that for mica, solid-CO 2 interfacial tension decrease with pressure and salinity and increase with temperature. Moreover, solid-liquid interfacial tension decrease with temperature and decrease with salinity. For quartz, although the solid-CO 2 interfacial tension decrease with pressure and increase with temperature, yet solid-liquid interfacial tension increase with temperature which explains the increase in contact angle with temperature for quartz. Overall, we find that results are in accordance with wettability data as function of pressure, temperature and salinity. We thus conclude that hotter reservoirs with lower injection pressure and lower brine salinities exhibit relatively better water wetting state and hence better seal capacity leading to higher CO 2 storage potential. We also conclude that solid surface energy approach adequately explains the dependency of wettability on pressure, temperature and salinity. 2017 Conference Paper http://hdl.handle.net/20.500.11937/58044 10.1016/j.egypro.2017.03.1623 http://creativecommons.org/licenses/by-nc-nd/4.0/ fulltext
spellingShingle Arif, Muhammad
Barifcani, Ahmed
Lebedev, Maxim
Iglauer, Stefan
Impact of Solid Surface Energy on Wettability of CO2-brine-Mineral Systems as a Function of Pressure, Temperature and Salinity
title Impact of Solid Surface Energy on Wettability of CO2-brine-Mineral Systems as a Function of Pressure, Temperature and Salinity
title_full Impact of Solid Surface Energy on Wettability of CO2-brine-Mineral Systems as a Function of Pressure, Temperature and Salinity
title_fullStr Impact of Solid Surface Energy on Wettability of CO2-brine-Mineral Systems as a Function of Pressure, Temperature and Salinity
title_full_unstemmed Impact of Solid Surface Energy on Wettability of CO2-brine-Mineral Systems as a Function of Pressure, Temperature and Salinity
title_short Impact of Solid Surface Energy on Wettability of CO2-brine-Mineral Systems as a Function of Pressure, Temperature and Salinity
title_sort impact of solid surface energy on wettability of co2-brine-mineral systems as a function of pressure, temperature and salinity
url http://hdl.handle.net/20.500.11937/58044