Solubility and solubility modeling of polycyclic aromatic hydrocarbons in subcritical ethanol and water mixtures

The solubilities of anthracene and p-terphenyl in subcritical ethanol and water mixtures were measured using a static analytical equilibrium method between 393 and 473 K and at 50 and 150 bar. Temperature and ethanol composition in the subcritical solvent mixtures were found to have significant effe...

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Main Authors: Teoh, W., Vieira De Melo, S., Mammucari, R., Foster, Neil
Format: Journal Article
Published: American Chemical Society 2014
Online Access:http://hdl.handle.net/20.500.11937/56207
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author Teoh, W.
Vieira De Melo, S.
Mammucari, R.
Foster, Neil
author_facet Teoh, W.
Vieira De Melo, S.
Mammucari, R.
Foster, Neil
author_sort Teoh, W.
building Curtin Institutional Repository
collection Online Access
description The solubilities of anthracene and p-terphenyl in subcritical ethanol and water mixtures were measured using a static analytical equilibrium method between 393 and 473 K and at 50 and 150 bar. Temperature and ethanol composition in the subcritical solvent mixtures were found to have significant effects on the solubility of polycyclic aromatic hydrocarbons (PAHs). The effect of pressure on solubility is negligible when the range of pressure considered is relatively small. An empirical model was proposed in the present study to correlate the solubility of PAHs to temperature and ethanol mole fraction. UNIQUAC, O-UNIFAC, and M-UNIFAC models were compared, with the UNIQUAC model found to be in good agreement with experimental data. © 2014 American Chemical Society.
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spelling curtin-20.500.11937-562072017-09-13T16:10:18Z Solubility and solubility modeling of polycyclic aromatic hydrocarbons in subcritical ethanol and water mixtures Teoh, W. Vieira De Melo, S. Mammucari, R. Foster, Neil The solubilities of anthracene and p-terphenyl in subcritical ethanol and water mixtures were measured using a static analytical equilibrium method between 393 and 473 K and at 50 and 150 bar. Temperature and ethanol composition in the subcritical solvent mixtures were found to have significant effects on the solubility of polycyclic aromatic hydrocarbons (PAHs). The effect of pressure on solubility is negligible when the range of pressure considered is relatively small. An empirical model was proposed in the present study to correlate the solubility of PAHs to temperature and ethanol mole fraction. UNIQUAC, O-UNIFAC, and M-UNIFAC models were compared, with the UNIQUAC model found to be in good agreement with experimental data. © 2014 American Chemical Society. 2014 Journal Article http://hdl.handle.net/20.500.11937/56207 10.1021/ie501276e American Chemical Society restricted
spellingShingle Teoh, W.
Vieira De Melo, S.
Mammucari, R.
Foster, Neil
Solubility and solubility modeling of polycyclic aromatic hydrocarbons in subcritical ethanol and water mixtures
title Solubility and solubility modeling of polycyclic aromatic hydrocarbons in subcritical ethanol and water mixtures
title_full Solubility and solubility modeling of polycyclic aromatic hydrocarbons in subcritical ethanol and water mixtures
title_fullStr Solubility and solubility modeling of polycyclic aromatic hydrocarbons in subcritical ethanol and water mixtures
title_full_unstemmed Solubility and solubility modeling of polycyclic aromatic hydrocarbons in subcritical ethanol and water mixtures
title_short Solubility and solubility modeling of polycyclic aromatic hydrocarbons in subcritical ethanol and water mixtures
title_sort solubility and solubility modeling of polycyclic aromatic hydrocarbons in subcritical ethanol and water mixtures
url http://hdl.handle.net/20.500.11937/56207