C3N4 anchored ZIF 8 composites: Photo-regenerable, high capacity sorbents as adsorptive photocatalysts for the effective removal of tetracycline from water

© 2017 The Royal Society of Chemistry. Materials combining the abilities of adsorption and photocatalysis provide a facile solution for pollutant disposal as secondary remediation processes are avoided. Herein, we report a simple strategy for the development of C 3 N 4 anchored ZIF-8 microcrystals...

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Main Authors: Panneri, S., Thomas, M., Ganguly, P., Nair, Balagopal, Mohamed, A., Warrier, K., Hareesh, U.
Format: Journal Article
Published: RSC Publications 2017
Online Access:http://hdl.handle.net/20.500.11937/55708
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author Panneri, S.
Thomas, M.
Ganguly, P.
Nair, Balagopal
Mohamed, A.
Warrier, K.
Hareesh, U.
author_facet Panneri, S.
Thomas, M.
Ganguly, P.
Nair, Balagopal
Mohamed, A.
Warrier, K.
Hareesh, U.
author_sort Panneri, S.
building Curtin Institutional Repository
collection Online Access
description © 2017 The Royal Society of Chemistry. Materials combining the abilities of adsorption and photocatalysis provide a facile solution for pollutant disposal as secondary remediation processes are avoided. Herein, we report a simple strategy for the development of C 3 N 4 anchored ZIF-8 microcrystals as sheathed architectures for the highly efficient adsorption and sunlight induced photocatalytic degradation of tetracycline from solution. An adsorption capacity as high as 420 mg g -1 of adsorbent was realized for a composition containing 60:40 wt% of C 3 N 4 and ZIF. Subsequently, the adsorbed tetracycline was degraded to over 96% in 1 h of sunlight exposure. The effects of pH and adsorbate concentration are studied and valid adsorption and degradation kinetic models are arrived at. The bifunctional composite thus developed offers a photo-regenerable adsorbent for the effective removal of an emerging hazardous contaminant.
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institution Curtin University Malaysia
institution_category Local University
last_indexed 2025-11-14T10:03:51Z
publishDate 2017
publisher RSC Publications
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spelling curtin-20.500.11937-557082023-08-02T06:39:09Z C3N4 anchored ZIF 8 composites: Photo-regenerable, high capacity sorbents as adsorptive photocatalysts for the effective removal of tetracycline from water Panneri, S. Thomas, M. Ganguly, P. Nair, Balagopal Mohamed, A. Warrier, K. Hareesh, U. © 2017 The Royal Society of Chemistry. Materials combining the abilities of adsorption and photocatalysis provide a facile solution for pollutant disposal as secondary remediation processes are avoided. Herein, we report a simple strategy for the development of C 3 N 4 anchored ZIF-8 microcrystals as sheathed architectures for the highly efficient adsorption and sunlight induced photocatalytic degradation of tetracycline from solution. An adsorption capacity as high as 420 mg g -1 of adsorbent was realized for a composition containing 60:40 wt% of C 3 N 4 and ZIF. Subsequently, the adsorbed tetracycline was degraded to over 96% in 1 h of sunlight exposure. The effects of pH and adsorbate concentration are studied and valid adsorption and degradation kinetic models are arrived at. The bifunctional composite thus developed offers a photo-regenerable adsorbent for the effective removal of an emerging hazardous contaminant. 2017 Journal Article http://hdl.handle.net/20.500.11937/55708 10.1039/c7cy00348j RSC Publications restricted
spellingShingle Panneri, S.
Thomas, M.
Ganguly, P.
Nair, Balagopal
Mohamed, A.
Warrier, K.
Hareesh, U.
C3N4 anchored ZIF 8 composites: Photo-regenerable, high capacity sorbents as adsorptive photocatalysts for the effective removal of tetracycline from water
title C3N4 anchored ZIF 8 composites: Photo-regenerable, high capacity sorbents as adsorptive photocatalysts for the effective removal of tetracycline from water
title_full C3N4 anchored ZIF 8 composites: Photo-regenerable, high capacity sorbents as adsorptive photocatalysts for the effective removal of tetracycline from water
title_fullStr C3N4 anchored ZIF 8 composites: Photo-regenerable, high capacity sorbents as adsorptive photocatalysts for the effective removal of tetracycline from water
title_full_unstemmed C3N4 anchored ZIF 8 composites: Photo-regenerable, high capacity sorbents as adsorptive photocatalysts for the effective removal of tetracycline from water
title_short C3N4 anchored ZIF 8 composites: Photo-regenerable, high capacity sorbents as adsorptive photocatalysts for the effective removal of tetracycline from water
title_sort c3n4 anchored zif 8 composites: photo-regenerable, high capacity sorbents as adsorptive photocatalysts for the effective removal of tetracycline from water
url http://hdl.handle.net/20.500.11937/55708