Vapor-liquid phase equilibrium data of CO2 in some physical solvents from 285.19 K to 313.26 K

The solubility of CO 2 in polyethylene glycol dimethyl ether (NHD), octamethyl cyclotetrasiloxane (D4), and diethyl succinate (DS) was determined at the temperature variations from 285.19 K to 313.26 K up to 6 MPa by the constant-volume method. Then, Henry's law constant (H) based on mole frac...

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Main Authors: Gui, X., Wang, Wei, Wang, C., Zhang, L., Yun, Z., Tang, Z.
Format: Journal Article
Published: American Chemical Society 2014
Online Access:http://hdl.handle.net/20.500.11937/55349
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author Gui, X.
Wang, Wei
Wang, C.
Zhang, L.
Yun, Z.
Tang, Z.
author_facet Gui, X.
Wang, Wei
Wang, C.
Zhang, L.
Yun, Z.
Tang, Z.
author_sort Gui, X.
building Curtin Institutional Repository
collection Online Access
description The solubility of CO 2 in polyethylene glycol dimethyl ether (NHD), octamethyl cyclotetrasiloxane (D4), and diethyl succinate (DS) was determined at the temperature variations from 285.19 K to 313.26 K up to 6 MPa by the constant-volume method. Then, Henry's law constant (H) based on mole fraction was obtained by linear fitting of the vapor-liquid phase equilibrium data, and some thermodynamic properties of solutions were also calculated from the correlation of H. The values of H in NHD, D4, and DS vary from 2.5 MPa to 8 MPa and increase in the following order: DS < D4 < NHD, which is identical to the order of the solvents ability to dissolve CO 2 . Additionally, Henry's law constant increases with temperature increase to confirm the solubility of CO 2 decrease in the corresponding solvents for the pressure range studied. © 2014 American Chemical Society.
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spelling curtin-20.500.11937-553492023-08-02T06:39:09Z Vapor-liquid phase equilibrium data of CO2 in some physical solvents from 285.19 K to 313.26 K Gui, X. Wang, Wei Wang, C. Zhang, L. Yun, Z. Tang, Z. The solubility of CO 2 in polyethylene glycol dimethyl ether (NHD), octamethyl cyclotetrasiloxane (D4), and diethyl succinate (DS) was determined at the temperature variations from 285.19 K to 313.26 K up to 6 MPa by the constant-volume method. Then, Henry's law constant (H) based on mole fraction was obtained by linear fitting of the vapor-liquid phase equilibrium data, and some thermodynamic properties of solutions were also calculated from the correlation of H. The values of H in NHD, D4, and DS vary from 2.5 MPa to 8 MPa and increase in the following order: DS < D4 < NHD, which is identical to the order of the solvents ability to dissolve CO 2 . Additionally, Henry's law constant increases with temperature increase to confirm the solubility of CO 2 decrease in the corresponding solvents for the pressure range studied. © 2014 American Chemical Society. 2014 Journal Article http://hdl.handle.net/20.500.11937/55349 10.1021/je400985u American Chemical Society restricted
spellingShingle Gui, X.
Wang, Wei
Wang, C.
Zhang, L.
Yun, Z.
Tang, Z.
Vapor-liquid phase equilibrium data of CO2 in some physical solvents from 285.19 K to 313.26 K
title Vapor-liquid phase equilibrium data of CO2 in some physical solvents from 285.19 K to 313.26 K
title_full Vapor-liquid phase equilibrium data of CO2 in some physical solvents from 285.19 K to 313.26 K
title_fullStr Vapor-liquid phase equilibrium data of CO2 in some physical solvents from 285.19 K to 313.26 K
title_full_unstemmed Vapor-liquid phase equilibrium data of CO2 in some physical solvents from 285.19 K to 313.26 K
title_short Vapor-liquid phase equilibrium data of CO2 in some physical solvents from 285.19 K to 313.26 K
title_sort vapor-liquid phase equilibrium data of co2 in some physical solvents from 285.19 k to 313.26 k
url http://hdl.handle.net/20.500.11937/55349