A one-pot, three-component aminotriazine annulation onto 5-aminopyrazole-4-carbonitriles under microwave irradiation

A one-pot, three-component, microwave-assisted reaction of 5-aminopyrazole-4-carbonitriles, triethyl orthoformate and cyanamide afforded novel 7-arylamino-substituted 4-aminopyrazolo[1,5-a][1,3,5]triazine-8-carbonitriles. The reaction proceeded in a chemo- and regioselective manner resulting in the...

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Main Authors: Lim, Felicia Phei Lin, Luna, Giuseppe, Dolzhenko, Anton
Format: Journal Article
Published: Pergamon 2015
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/5411
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author Lim, Felicia Phei Lin
Luna, Giuseppe
Dolzhenko, Anton
author_facet Lim, Felicia Phei Lin
Luna, Giuseppe
Dolzhenko, Anton
author_sort Lim, Felicia Phei Lin
building Curtin Institutional Repository
collection Online Access
description A one-pot, three-component, microwave-assisted reaction of 5-aminopyrazole-4-carbonitriles, triethyl orthoformate and cyanamide afforded novel 7-arylamino-substituted 4-aminopyrazolo[1,5-a][1,3,5]triazine-8-carbonitriles. The reaction proceeded in a chemo- and regioselective manner resulting in the successful amino-1,3,5-triazine annulation onto 5-aminopyrazole-4-carbonitriles to give 4-aminopyrazolo[1,5-a][1,3,5]triazine-8-carbonitriles. The operational simplicity of the method and high purity of the products, which can be isolated via simple filtration, make this approach attractive for the preparation of a library of compounds for drug discovery processes.
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format Journal Article
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institution Curtin University Malaysia
institution_category Local University
last_indexed 2025-11-14T06:07:02Z
publishDate 2015
publisher Pergamon
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spelling curtin-20.500.11937-54112019-02-19T04:26:53Z A one-pot, three-component aminotriazine annulation onto 5-aminopyrazole-4-carbonitriles under microwave irradiation Lim, Felicia Phei Lin Luna, Giuseppe Dolzhenko, Anton Purine isostere Multicomponent reaction Microwave-assisted synthesis Triazine Pyrazole A one-pot, three-component, microwave-assisted reaction of 5-aminopyrazole-4-carbonitriles, triethyl orthoformate and cyanamide afforded novel 7-arylamino-substituted 4-aminopyrazolo[1,5-a][1,3,5]triazine-8-carbonitriles. The reaction proceeded in a chemo- and regioselective manner resulting in the successful amino-1,3,5-triazine annulation onto 5-aminopyrazole-4-carbonitriles to give 4-aminopyrazolo[1,5-a][1,3,5]triazine-8-carbonitriles. The operational simplicity of the method and high purity of the products, which can be isolated via simple filtration, make this approach attractive for the preparation of a library of compounds for drug discovery processes. 2015 Journal Article http://hdl.handle.net/20.500.11937/5411 10.1016/j.tetlet.2014.12.010 Pergamon fulltext
spellingShingle Purine isostere
Multicomponent reaction
Microwave-assisted synthesis
Triazine
Pyrazole
Lim, Felicia Phei Lin
Luna, Giuseppe
Dolzhenko, Anton
A one-pot, three-component aminotriazine annulation onto 5-aminopyrazole-4-carbonitriles under microwave irradiation
title A one-pot, three-component aminotriazine annulation onto 5-aminopyrazole-4-carbonitriles under microwave irradiation
title_full A one-pot, three-component aminotriazine annulation onto 5-aminopyrazole-4-carbonitriles under microwave irradiation
title_fullStr A one-pot, three-component aminotriazine annulation onto 5-aminopyrazole-4-carbonitriles under microwave irradiation
title_full_unstemmed A one-pot, three-component aminotriazine annulation onto 5-aminopyrazole-4-carbonitriles under microwave irradiation
title_short A one-pot, three-component aminotriazine annulation onto 5-aminopyrazole-4-carbonitriles under microwave irradiation
title_sort one-pot, three-component aminotriazine annulation onto 5-aminopyrazole-4-carbonitriles under microwave irradiation
topic Purine isostere
Multicomponent reaction
Microwave-assisted synthesis
Triazine
Pyrazole
url http://hdl.handle.net/20.500.11937/5411