Seeing is believing: Visualization of He distribution in zircon and implications for thermal history reconstruction on single crystals

Zircon (U-Th)/He thermochronometry is an established radiometric dating technique used to place temporal constraints on a range of thermally sensitive geological events, such as crustal exhumation, volcanism, meteorite impact, and ore genesis. Isotopic, crystallographic, and/or mineralogical heterog...

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Main Authors: Danišík, Martin, McInnes, Brent, Kirkland, Chris, McDonald, Brad, Evans, Noreen, Becker, Thomas
Format: Journal Article
Published: 2017
Online Access:http://purl.org/au-research/grants/arc/DP160102427
http://hdl.handle.net/20.500.11937/51417
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author Danišík, Martin
McInnes, Brent
Kirkland, Chris
McDonald, Brad
Evans, Noreen
Becker, Thomas
author_facet Danišík, Martin
McInnes, Brent
Kirkland, Chris
McDonald, Brad
Evans, Noreen
Becker, Thomas
author_sort Danišík, Martin
building Curtin Institutional Repository
collection Online Access
description Zircon (U-Th)/He thermochronometry is an established radiometric dating technique used to place temporal constraints on a range of thermally sensitive geological events, such as crustal exhumation, volcanism, meteorite impact, and ore genesis. Isotopic, crystallographic, and/or mineralogical heterogeneities within analyzed grains can result in dispersed or anomalous (U-Th)/He ages. Understanding the effect of these grain-scale phenomena on the distribution of He in analyzed minerals should lead to improvements in data interpretation. We combine laser ablation microsampling and noble gas and trace element mass spectrometry to provide the first two-dimensional, grain-scale zircon He "maps" and quantify intragrain He distribution. These maps illustrate the complexity of intracrystalline He distribution in natural zircon and, combined with a correlated quantification of parent nuclide (U and Th) distribution, provide an opportunity to assess a number of crystal chemistry processes that can generate anomalous zircon (U-Th)/He ages. The technique provides new insights into fluid inclusions as potential traps of radiogenic He and confirms the effect of heterogeneity in parent-daughter isotope abundances and metamictization on (U-Th)/He systematics. Finally, we present a new inversion method where the He, U, and Th mapping data can be used to constrain the high- and low-temperature history of a single zircon crystal.
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spelling curtin-20.500.11937-514172022-10-27T04:25:48Z Seeing is believing: Visualization of He distribution in zircon and implications for thermal history reconstruction on single crystals Danišík, Martin McInnes, Brent Kirkland, Chris McDonald, Brad Evans, Noreen Becker, Thomas Zircon (U-Th)/He thermochronometry is an established radiometric dating technique used to place temporal constraints on a range of thermally sensitive geological events, such as crustal exhumation, volcanism, meteorite impact, and ore genesis. Isotopic, crystallographic, and/or mineralogical heterogeneities within analyzed grains can result in dispersed or anomalous (U-Th)/He ages. Understanding the effect of these grain-scale phenomena on the distribution of He in analyzed minerals should lead to improvements in data interpretation. We combine laser ablation microsampling and noble gas and trace element mass spectrometry to provide the first two-dimensional, grain-scale zircon He "maps" and quantify intragrain He distribution. These maps illustrate the complexity of intracrystalline He distribution in natural zircon and, combined with a correlated quantification of parent nuclide (U and Th) distribution, provide an opportunity to assess a number of crystal chemistry processes that can generate anomalous zircon (U-Th)/He ages. The technique provides new insights into fluid inclusions as potential traps of radiogenic He and confirms the effect of heterogeneity in parent-daughter isotope abundances and metamictization on (U-Th)/He systematics. Finally, we present a new inversion method where the He, U, and Th mapping data can be used to constrain the high- and low-temperature history of a single zircon crystal. 2017 Journal Article http://hdl.handle.net/20.500.11937/51417 10.1126/sciadv.1601121 http://purl.org/au-research/grants/arc/DP160102427 http://creativecommons.org/licenses/by-nc/4.0/ fulltext
spellingShingle Danišík, Martin
McInnes, Brent
Kirkland, Chris
McDonald, Brad
Evans, Noreen
Becker, Thomas
Seeing is believing: Visualization of He distribution in zircon and implications for thermal history reconstruction on single crystals
title Seeing is believing: Visualization of He distribution in zircon and implications for thermal history reconstruction on single crystals
title_full Seeing is believing: Visualization of He distribution in zircon and implications for thermal history reconstruction on single crystals
title_fullStr Seeing is believing: Visualization of He distribution in zircon and implications for thermal history reconstruction on single crystals
title_full_unstemmed Seeing is believing: Visualization of He distribution in zircon and implications for thermal history reconstruction on single crystals
title_short Seeing is believing: Visualization of He distribution in zircon and implications for thermal history reconstruction on single crystals
title_sort seeing is believing: visualization of he distribution in zircon and implications for thermal history reconstruction on single crystals
url http://purl.org/au-research/grants/arc/DP160102427
http://hdl.handle.net/20.500.11937/51417