Synthesis, Chemistry and Structure of Some 1,1-Dimethylcyclopropazulenes

1,1-Dimethylcycloprop[e]azulene and 1,1-dimethylcyclo-prop[f]azulene derivatives were prepared through a short syn-thesis from thiophene-1,1-dioxides using a Houk-Leaver azu-lene synthesis. The strain caused by the fusion of thecyclopropane ring had no effect on electrophilic aromatic sub-stitution...

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Main Authors: Payne, Alan, Skelton, B., White, A., Wege, D.
Format: Journal Article
Published: 2016
Online Access:http://hdl.handle.net/20.500.11937/50398
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author Payne, Alan
Skelton, B.
White, A.
Wege, D.
author_facet Payne, Alan
Skelton, B.
White, A.
Wege, D.
author_sort Payne, Alan
building Curtin Institutional Repository
collection Online Access
description 1,1-Dimethylcycloprop[e]azulene and 1,1-dimethylcyclo-prop[f]azulene derivatives were prepared through a short syn-thesis from thiophene-1,1-dioxides using a Houk-Leaver azu-lene synthesis. The strain caused by the fusion of thecyclopropane ring had no effect on electrophilic aromatic sub-stitution reactions. X-ray structures of these compoundsshowed that cycloprop[e] azulenes have no or very small straininduced bond localisation, whereas cycloprop[f]azulene showssome minor localisation.
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spelling curtin-20.500.11937-503982017-09-13T15:34:03Z Synthesis, Chemistry and Structure of Some 1,1-Dimethylcyclopropazulenes Payne, Alan Skelton, B. White, A. Wege, D. 1,1-Dimethylcycloprop[e]azulene and 1,1-dimethylcyclo-prop[f]azulene derivatives were prepared through a short syn-thesis from thiophene-1,1-dioxides using a Houk-Leaver azu-lene synthesis. The strain caused by the fusion of thecyclopropane ring had no effect on electrophilic aromatic sub-stitution reactions. X-ray structures of these compoundsshowed that cycloprop[e] azulenes have no or very small straininduced bond localisation, whereas cycloprop[f]azulene showssome minor localisation. 2016 Journal Article http://hdl.handle.net/20.500.11937/50398 10.1002/slct.201601168 restricted
spellingShingle Payne, Alan
Skelton, B.
White, A.
Wege, D.
Synthesis, Chemistry and Structure of Some 1,1-Dimethylcyclopropazulenes
title Synthesis, Chemistry and Structure of Some 1,1-Dimethylcyclopropazulenes
title_full Synthesis, Chemistry and Structure of Some 1,1-Dimethylcyclopropazulenes
title_fullStr Synthesis, Chemistry and Structure of Some 1,1-Dimethylcyclopropazulenes
title_full_unstemmed Synthesis, Chemistry and Structure of Some 1,1-Dimethylcyclopropazulenes
title_short Synthesis, Chemistry and Structure of Some 1,1-Dimethylcyclopropazulenes
title_sort synthesis, chemistry and structure of some 1,1-dimethylcyclopropazulenes
url http://hdl.handle.net/20.500.11937/50398