Co-nanoencapsulated doxorubicin and Dz13 control osteosarcoma progression in a murine model

Objectives: Chitosan is a green (natural, abundant, biodegradable, biocompatible) biopolymer that can be formulated to encapsulate a variety of therapeutic compounds. This study aimed to investigate chitosan nanoparticles (NPs) as a means of improving delivery of the clinically used anti-cancer agen...

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Main Authors: Tan, M., Friedhuber, A., Dass, Crispin
Format: Journal Article
Published: John Wiley & Sons Ltd. 2013
Online Access:http://hdl.handle.net/20.500.11937/49673
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author Tan, M.
Friedhuber, A.
Dass, Crispin
author_facet Tan, M.
Friedhuber, A.
Dass, Crispin
author_sort Tan, M.
building Curtin Institutional Repository
collection Online Access
description Objectives: Chitosan is a green (natural, abundant, biodegradable, biocompatible) biopolymer that can be formulated to encapsulate a variety of therapeutic compounds. This study aimed to investigate chitosan nanoparticles (NPs) as a means of improving delivery of the clinically used anti-cancer agent doxorubicin (Dox) and the preclinical lead compound Dz13 oligonucleotide together. Methods: A novel chitosan NP system encapsulating Dox and Dz13 was designed, biophysically characterised and tested in a clinically relevant model of the metastasising bone tumour, osteosarcoma (OS). Key findings: By careful alteration of the concentration of the individual components, a final formulation of Dz13-Dox NPs (DDNPs) was achieved, with high (>91%) loading of both compounds, which consisted of individual 50-nm particles forming aggregates as large as 500 nm, with a large positive ζ-potential. The DDNPs could be stored at various temperatures for a week without loss in activity but were prone to degradation in serum. DDNPs successfully inhibited OS tumour growth more effectively than treatment with NPs of Dz13 and Dox-chitosan, as well as Dox administered intraperitoneally. Apart from inhibiting tumour growth, DDNPs protected the affected bone from substantial destruction by aggressive tumour growth and reduced the incidence of metastasis to the lungs without causing adverse effects in mice. Conclusion: This NP is a promising formulation that could be useful for clinical management of OS.
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spelling curtin-20.500.11937-496732017-09-13T15:48:32Z Co-nanoencapsulated doxorubicin and Dz13 control osteosarcoma progression in a murine model Tan, M. Friedhuber, A. Dass, Crispin Objectives: Chitosan is a green (natural, abundant, biodegradable, biocompatible) biopolymer that can be formulated to encapsulate a variety of therapeutic compounds. This study aimed to investigate chitosan nanoparticles (NPs) as a means of improving delivery of the clinically used anti-cancer agent doxorubicin (Dox) and the preclinical lead compound Dz13 oligonucleotide together. Methods: A novel chitosan NP system encapsulating Dox and Dz13 was designed, biophysically characterised and tested in a clinically relevant model of the metastasising bone tumour, osteosarcoma (OS). Key findings: By careful alteration of the concentration of the individual components, a final formulation of Dz13-Dox NPs (DDNPs) was achieved, with high (>91%) loading of both compounds, which consisted of individual 50-nm particles forming aggregates as large as 500 nm, with a large positive ζ-potential. The DDNPs could be stored at various temperatures for a week without loss in activity but were prone to degradation in serum. DDNPs successfully inhibited OS tumour growth more effectively than treatment with NPs of Dz13 and Dox-chitosan, as well as Dox administered intraperitoneally. Apart from inhibiting tumour growth, DDNPs protected the affected bone from substantial destruction by aggressive tumour growth and reduced the incidence of metastasis to the lungs without causing adverse effects in mice. Conclusion: This NP is a promising formulation that could be useful for clinical management of OS. 2013 Journal Article http://hdl.handle.net/20.500.11937/49673 10.1111/j.2042-7158.2012.01572.x John Wiley & Sons Ltd. restricted
spellingShingle Tan, M.
Friedhuber, A.
Dass, Crispin
Co-nanoencapsulated doxorubicin and Dz13 control osteosarcoma progression in a murine model
title Co-nanoencapsulated doxorubicin and Dz13 control osteosarcoma progression in a murine model
title_full Co-nanoencapsulated doxorubicin and Dz13 control osteosarcoma progression in a murine model
title_fullStr Co-nanoencapsulated doxorubicin and Dz13 control osteosarcoma progression in a murine model
title_full_unstemmed Co-nanoencapsulated doxorubicin and Dz13 control osteosarcoma progression in a murine model
title_short Co-nanoencapsulated doxorubicin and Dz13 control osteosarcoma progression in a murine model
title_sort co-nanoencapsulated doxorubicin and dz13 control osteosarcoma progression in a murine model
url http://hdl.handle.net/20.500.11937/49673