Mesoporous Nafion Membranes for Fuel Cell Applications

Ordered mesoporous structures were successfully introduced into Nafion membranes via a soft micelle templating method, using a nonionic block copolymer surfactant, PEO127-PPO48-PEO127 (Pluronic F108). The mesoporous Nafion or meso-Nafion membranes were characterized by the AFM, SAXS, TGA and conduct...

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Main Authors: Jiang, San Ping, Lu, J.
Other Authors: H. Gasteiger
Format: Journal Article
Published: The Electrochemical Society, Inc. 2011
Online Access:http://hdl.handle.net/20.500.11937/48367
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author Jiang, San Ping
Lu, J.
author2 H. Gasteiger
author_facet H. Gasteiger
Jiang, San Ping
Lu, J.
author_sort Jiang, San Ping
building Curtin Institutional Repository
collection Online Access
description Ordered mesoporous structures were successfully introduced into Nafion membranes via a soft micelle templating method, using a nonionic block copolymer surfactant, PEO127-PPO48-PEO127 (Pluronic F108). The mesoporous Nafion or meso-Nafion membranes were characterized by the AFM, SAXS, TGA and conductivity measurements. The results show that the meso-Nafion has a very high water retention capability. The proton conductivities of meso-Nafion are also much higher than that of Nafion 115 membranes particularly at reduced relative humidity (RH) and elevated temperatures. At 80˚C and 40%RH, the conductivity of meso-Nafion is 0.07 Scm-1, more than 3 times better than Nafion 115. At 60%RH and 80˚C, the cell with meso-Nafion reached a stable power output of 0.63 Wcm-2, more than 2 times higher than the cell with pristine Nafion 115 under identical experimental conditions. The cells with meso-Nafion membrane also demonstrate much better stability at elevated temperature of 120˚C and reduced humidities.
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spelling curtin-20.500.11937-483672023-02-02T07:57:34Z Mesoporous Nafion Membranes for Fuel Cell Applications Jiang, San Ping Lu, J. H. Gasteiger F.N. Buchi A.J. Davenport M. Edmundson T.F. Fuller Ordered mesoporous structures were successfully introduced into Nafion membranes via a soft micelle templating method, using a nonionic block copolymer surfactant, PEO127-PPO48-PEO127 (Pluronic F108). The mesoporous Nafion or meso-Nafion membranes were characterized by the AFM, SAXS, TGA and conductivity measurements. The results show that the meso-Nafion has a very high water retention capability. The proton conductivities of meso-Nafion are also much higher than that of Nafion 115 membranes particularly at reduced relative humidity (RH) and elevated temperatures. At 80˚C and 40%RH, the conductivity of meso-Nafion is 0.07 Scm-1, more than 3 times better than Nafion 115. At 60%RH and 80˚C, the cell with meso-Nafion reached a stable power output of 0.63 Wcm-2, more than 2 times higher than the cell with pristine Nafion 115 under identical experimental conditions. The cells with meso-Nafion membrane also demonstrate much better stability at elevated temperature of 120˚C and reduced humidities. 2011 Journal Article http://hdl.handle.net/20.500.11937/48367 10.1149/1.3635687 The Electrochemical Society, Inc. restricted
spellingShingle Jiang, San Ping
Lu, J.
Mesoporous Nafion Membranes for Fuel Cell Applications
title Mesoporous Nafion Membranes for Fuel Cell Applications
title_full Mesoporous Nafion Membranes for Fuel Cell Applications
title_fullStr Mesoporous Nafion Membranes for Fuel Cell Applications
title_full_unstemmed Mesoporous Nafion Membranes for Fuel Cell Applications
title_short Mesoporous Nafion Membranes for Fuel Cell Applications
title_sort mesoporous nafion membranes for fuel cell applications
url http://hdl.handle.net/20.500.11937/48367