Vacuum-assisted electroless copper plating on Ni/(Sm,Ce)O2 anodes for intermediate temperature solid oxide fuel cells

Cu is incorporated by vacuum-assisted electroless plating into porous Ni/Sm0.2Ce0.8O1.9 (Ni/SDC) anodes as the active anodes for the oxidation reaction of hydrogen and methane of intermediate temperature solid oxide fuel cells (IT-SOFCs). The scanning electron microscopy (SEM) observation indicates...

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Main Authors: Ai, Na, Chen, Kongfa, Jiang, San Ping, Lu, Z., Su, W.
Format: Journal Article
Published: Pergamon-Elsevier Science Ltd 2011
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/4728
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author Ai, Na
Chen, Kongfa
Jiang, San Ping
Lu, Z.
Su, W.
author_facet Ai, Na
Chen, Kongfa
Jiang, San Ping
Lu, Z.
Su, W.
author_sort Ai, Na
building Curtin Institutional Repository
collection Online Access
description Cu is incorporated by vacuum-assisted electroless plating into porous Ni/Sm0.2Ce0.8O1.9 (Ni/SDC) anodes as the active anodes for the oxidation reaction of hydrogen and methane of intermediate temperature solid oxide fuel cells (IT-SOFCs). The scanning electron microscopy (SEM) observation indicates the formation of a uniformly distributed nanostructured Cu network within the porous Ni/SDC microstructure. The maximum power density of the cell with the Cu electroless-plated Ni/SDC anodes is 0.84 and 0.54 W cm2 in dry H2 and dry CH4 at 600 C, respectively, enhanced by w30% as compared to the cell with conventional Ni/SDC anodes. The increase in the performance of the cell with the Cu electroless-plated Ni/SDC anodes is most likely attributed to the enlarged effective threephaseboundaries (TPBs) by interconnecting the isolated Ni and/or SDC particles with the electroless-plated Cu network and the formation of TPBs at the Cu/SDC interface due to the activation of SDC surface by the Cu deposition. The stability test shows that cell degradation in dry methane due to carbon deposition is significantly reduced by the electroless copper plating.
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publishDate 2011
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spelling curtin-20.500.11937-47282017-09-13T14:45:48Z Vacuum-assisted electroless copper plating on Ni/(Sm,Ce)O2 anodes for intermediate temperature solid oxide fuel cells Ai, Na Chen, Kongfa Jiang, San Ping Lu, Z. Su, W. Carbon deposition Cu network Isolated TPBs Ni/SDC cermet anode Solid oxide fuel cells Electroless copper plating Cu is incorporated by vacuum-assisted electroless plating into porous Ni/Sm0.2Ce0.8O1.9 (Ni/SDC) anodes as the active anodes for the oxidation reaction of hydrogen and methane of intermediate temperature solid oxide fuel cells (IT-SOFCs). The scanning electron microscopy (SEM) observation indicates the formation of a uniformly distributed nanostructured Cu network within the porous Ni/SDC microstructure. The maximum power density of the cell with the Cu electroless-plated Ni/SDC anodes is 0.84 and 0.54 W cm2 in dry H2 and dry CH4 at 600 C, respectively, enhanced by w30% as compared to the cell with conventional Ni/SDC anodes. The increase in the performance of the cell with the Cu electroless-plated Ni/SDC anodes is most likely attributed to the enlarged effective threephaseboundaries (TPBs) by interconnecting the isolated Ni and/or SDC particles with the electroless-plated Cu network and the formation of TPBs at the Cu/SDC interface due to the activation of SDC surface by the Cu deposition. The stability test shows that cell degradation in dry methane due to carbon deposition is significantly reduced by the electroless copper plating. 2011 Journal Article http://hdl.handle.net/20.500.11937/4728 10.1016/j.ijhydene.2011.03.131 Pergamon-Elsevier Science Ltd restricted
spellingShingle Carbon deposition
Cu network
Isolated TPBs
Ni/SDC cermet anode
Solid oxide fuel cells
Electroless copper plating
Ai, Na
Chen, Kongfa
Jiang, San Ping
Lu, Z.
Su, W.
Vacuum-assisted electroless copper plating on Ni/(Sm,Ce)O2 anodes for intermediate temperature solid oxide fuel cells
title Vacuum-assisted electroless copper plating on Ni/(Sm,Ce)O2 anodes for intermediate temperature solid oxide fuel cells
title_full Vacuum-assisted electroless copper plating on Ni/(Sm,Ce)O2 anodes for intermediate temperature solid oxide fuel cells
title_fullStr Vacuum-assisted electroless copper plating on Ni/(Sm,Ce)O2 anodes for intermediate temperature solid oxide fuel cells
title_full_unstemmed Vacuum-assisted electroless copper plating on Ni/(Sm,Ce)O2 anodes for intermediate temperature solid oxide fuel cells
title_short Vacuum-assisted electroless copper plating on Ni/(Sm,Ce)O2 anodes for intermediate temperature solid oxide fuel cells
title_sort vacuum-assisted electroless copper plating on ni/(sm,ce)o2 anodes for intermediate temperature solid oxide fuel cells
topic Carbon deposition
Cu network
Isolated TPBs
Ni/SDC cermet anode
Solid oxide fuel cells
Electroless copper plating
url http://hdl.handle.net/20.500.11937/4728