Chromium deposition and poisoning at Ba0.5Sr0.5Co0.8Fe0.2O3 cathode of solid oxide fuel cells

Chromium deposition and poisoning at Ba0.5Sr0.5Co0.8Fe0.2O3-d (BSCF) cathodes of solid oxide fuel cells are investigated. BSCF cathode shows an excellent and stable performance in the absence of metallic interconnects. However, in the presence of a chromia-forming metallic interconnect performance o...

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Main Authors: Kim, Y., Chen, X., Jiang, San Ping, Bae, J.
Format: Journal Article
Published: Electrochemical Society 2011
Online Access:http://hdl.handle.net/20.500.11937/44841
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author Kim, Y.
Chen, X.
Jiang, San Ping
Bae, J.
author_facet Kim, Y.
Chen, X.
Jiang, San Ping
Bae, J.
author_sort Kim, Y.
building Curtin Institutional Repository
collection Online Access
description Chromium deposition and poisoning at Ba0.5Sr0.5Co0.8Fe0.2O3-d (BSCF) cathodes of solid oxide fuel cells are investigated. BSCF cathode shows an excellent and stable performance in the absence of metallic interconnects. However, in the presence of a chromia-forming metallic interconnect performance of the BSCF cathodes degrades quickly. Chromium deposition was observed on the BSCF cathode surface after 1200 min polarization at 900 and 800C. The Cr2O3/SrO and Cr2O3/BaCO3 oxide couple study indicates that SrCrO4, BaCrO4, and BaCr2O4 start to form at temperatures above 500C. The results indicate that BSCF cathode is not chromium-tolerant despite its superior activity for the O2 reduction reaction.
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institution Curtin University Malaysia
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publishDate 2011
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spelling curtin-20.500.11937-448412017-02-28T01:38:08Z Chromium deposition and poisoning at Ba0.5Sr0.5Co0.8Fe0.2O3 cathode of solid oxide fuel cells Kim, Y. Chen, X. Jiang, San Ping Bae, J. Chromium deposition and poisoning at Ba0.5Sr0.5Co0.8Fe0.2O3-d (BSCF) cathodes of solid oxide fuel cells are investigated. BSCF cathode shows an excellent and stable performance in the absence of metallic interconnects. However, in the presence of a chromia-forming metallic interconnect performance of the BSCF cathodes degrades quickly. Chromium deposition was observed on the BSCF cathode surface after 1200 min polarization at 900 and 800C. The Cr2O3/SrO and Cr2O3/BaCO3 oxide couple study indicates that SrCrO4, BaCrO4, and BaCr2O4 start to form at temperatures above 500C. The results indicate that BSCF cathode is not chromium-tolerant despite its superior activity for the O2 reduction reaction. 2011 Journal Article http://hdl.handle.net/20.500.11937/44841 Electrochemical Society restricted
spellingShingle Kim, Y.
Chen, X.
Jiang, San Ping
Bae, J.
Chromium deposition and poisoning at Ba0.5Sr0.5Co0.8Fe0.2O3 cathode of solid oxide fuel cells
title Chromium deposition and poisoning at Ba0.5Sr0.5Co0.8Fe0.2O3 cathode of solid oxide fuel cells
title_full Chromium deposition and poisoning at Ba0.5Sr0.5Co0.8Fe0.2O3 cathode of solid oxide fuel cells
title_fullStr Chromium deposition and poisoning at Ba0.5Sr0.5Co0.8Fe0.2O3 cathode of solid oxide fuel cells
title_full_unstemmed Chromium deposition and poisoning at Ba0.5Sr0.5Co0.8Fe0.2O3 cathode of solid oxide fuel cells
title_short Chromium deposition and poisoning at Ba0.5Sr0.5Co0.8Fe0.2O3 cathode of solid oxide fuel cells
title_sort chromium deposition and poisoning at ba0.5sr0.5co0.8fe0.2o3 cathode of solid oxide fuel cells
url http://hdl.handle.net/20.500.11937/44841