Surfactant-free self-assembly of reduced graphite oxide-MoO2 nanobelt composites used as electrode for lithium-ion batteries

Graphene/metal oxide nanocomposites are promising electrode materials for lithium-ion batteries (LIBs), in which synergistic effects between the two components may benefit the overall capacity, rate capability and cycling stability. Here, we report a simple and easy scale-up method for the preparati...

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Main Authors: Zhu, Y., Xu, X., Chen, G., Zhong, Y., Cai, R., Li, L., Shao, Zongping
Format: Journal Article
Published: Pergamon 2016
Online Access:http://hdl.handle.net/20.500.11937/42772
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author Zhu, Y.
Xu, X.
Chen, G.
Zhong, Y.
Cai, R.
Li, L.
Shao, Zongping
author_facet Zhu, Y.
Xu, X.
Chen, G.
Zhong, Y.
Cai, R.
Li, L.
Shao, Zongping
author_sort Zhu, Y.
building Curtin Institutional Repository
collection Online Access
description Graphene/metal oxide nanocomposites are promising electrode materials for lithium-ion batteries (LIBs), in which synergistic effects between the two components may benefit the overall capacity, rate capability and cycling stability. Here, we report a simple and easy scale-up method for the preparation of high-quality reduced graphite oxide-MoO2 (rGO-MoO2) nanobelt composites, which demonstrate attractive electrochemical performance as LIB anodes. MoO3 nanobelts are first prepared by a simple hydrothermal route and distributed homogeneously in water, and then graphite oxide (GO) is prepared by a modified Hummers method and introduced into the solution. Both materials slowly self-assemble to form GO-MoO3 nanocomposite in a surfactant-free manner. After thermal reduction, rGO-MoO2 nanobelt composites are obtained, as confirmed by FE-SEM and TEM. Using such composite as LIB electrodes, a reversible capacity of 754 mA h g-1 is obtained after 80 cycles at 0.2 A g-1, and the electrode also demonstrates superior rate capabilities. These results are comparable to or even higher than those of other reported graphene-MoO2 composites, which are fabricated in more complicated fashions, thus rendering the current product as highly promising electrode materials for practical use.
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spelling curtin-20.500.11937-427722017-09-13T15:15:02Z Surfactant-free self-assembly of reduced graphite oxide-MoO2 nanobelt composites used as electrode for lithium-ion batteries Zhu, Y. Xu, X. Chen, G. Zhong, Y. Cai, R. Li, L. Shao, Zongping Graphene/metal oxide nanocomposites are promising electrode materials for lithium-ion batteries (LIBs), in which synergistic effects between the two components may benefit the overall capacity, rate capability and cycling stability. Here, we report a simple and easy scale-up method for the preparation of high-quality reduced graphite oxide-MoO2 (rGO-MoO2) nanobelt composites, which demonstrate attractive electrochemical performance as LIB anodes. MoO3 nanobelts are first prepared by a simple hydrothermal route and distributed homogeneously in water, and then graphite oxide (GO) is prepared by a modified Hummers method and introduced into the solution. Both materials slowly self-assemble to form GO-MoO3 nanocomposite in a surfactant-free manner. After thermal reduction, rGO-MoO2 nanobelt composites are obtained, as confirmed by FE-SEM and TEM. Using such composite as LIB electrodes, a reversible capacity of 754 mA h g-1 is obtained after 80 cycles at 0.2 A g-1, and the electrode also demonstrates superior rate capabilities. These results are comparable to or even higher than those of other reported graphene-MoO2 composites, which are fabricated in more complicated fashions, thus rendering the current product as highly promising electrode materials for practical use. 2016 Journal Article http://hdl.handle.net/20.500.11937/42772 10.1016/j.electacta.2016.06.139 Pergamon restricted
spellingShingle Zhu, Y.
Xu, X.
Chen, G.
Zhong, Y.
Cai, R.
Li, L.
Shao, Zongping
Surfactant-free self-assembly of reduced graphite oxide-MoO2 nanobelt composites used as electrode for lithium-ion batteries
title Surfactant-free self-assembly of reduced graphite oxide-MoO2 nanobelt composites used as electrode for lithium-ion batteries
title_full Surfactant-free self-assembly of reduced graphite oxide-MoO2 nanobelt composites used as electrode for lithium-ion batteries
title_fullStr Surfactant-free self-assembly of reduced graphite oxide-MoO2 nanobelt composites used as electrode for lithium-ion batteries
title_full_unstemmed Surfactant-free self-assembly of reduced graphite oxide-MoO2 nanobelt composites used as electrode for lithium-ion batteries
title_short Surfactant-free self-assembly of reduced graphite oxide-MoO2 nanobelt composites used as electrode for lithium-ion batteries
title_sort surfactant-free self-assembly of reduced graphite oxide-moo2 nanobelt composites used as electrode for lithium-ion batteries
url http://hdl.handle.net/20.500.11937/42772