Importance of the aromatic structures in volatiles to the in-situ destruction of nascent tar during the volatile-char interactions

This study aims to investigate the importance of aromatic structures in tar to the destruction of tar itself during the volatile-char interactions. The same nascent char was subjected to interactions with two distinctly different volatiles (e.g. coal volatiles and biomass volatiles) at 700-900 °C. T...

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Bibliographic Details
Main Authors: Song, Y., Xiang, J., Hu, S., Quyn, D., Zhao, Y., Hu, Xun, Wang, Y., Li, Chun-Zhu
Format: Journal Article
Published: Elsevier 2015
Online Access:http://hdl.handle.net/20.500.11937/4246
Description
Summary:This study aims to investigate the importance of aromatic structures in tar to the destruction of tar itself during the volatile-char interactions. The same nascent char was subjected to interactions with two distinctly different volatiles (e.g. coal volatiles and biomass volatiles) at 700-900 °C. The results indicate that the aromatic structures in tar are more reactive with char than the non-aromatic structures, especially at high temperature (e.g. 900 °C). At lower temperatures (< 800 °C), the more aromatic coal tar can form coke on the char surfaces more easily than the more aliphatic biomass tar. At higher temperatures (> 800 °C), the aromatic structures in tar are cracked and/or reformed into gases through interaction with the char; the aromatic structures from biomass can be reformed over char more easily than those from coal.