Influence of Temperature and Anisotropic Pressure on the Phase Transitions in α-Cristobalite

The role of temperature and anisotropy of the applied load in the pressure–induced transformations of α -cristobalite is investigated by means of first principles molecular dynamics combined with the metadynamics algorithm for the study of solid-solid phase transitions. We reproduce the transition t...

Full description

Bibliographic Details
Main Authors: Donadio, D., Martoňák, R., Raiteri, Paolo, Parrinello, M.
Format: Journal Article
Published: The American Physical Society 2008
Online Access:http://hdl.handle.net/20.500.11937/4233
_version_ 1848744457954918400
author Donadio, D.
Martoňák, R.
Raiteri, Paolo
Parrinello, M.
author_facet Donadio, D.
Martoňák, R.
Raiteri, Paolo
Parrinello, M.
author_sort Donadio, D.
building Curtin Institutional Repository
collection Online Access
description The role of temperature and anisotropy of the applied load in the pressure–induced transformations of α -cristobalite is investigated by means of first principles molecular dynamics combined with the metadynamics algorithm for the study of solid-solid phase transitions. We reproduce the transition to α-PbO2 as found in experiments and we observe that the transition paths are qualitatively different and yield different products when a nonhydrostatic load is applied, giving rise to a new class of metastable structures with mixed tetrahedral and octahedral coordination.
first_indexed 2025-11-14T06:01:47Z
format Journal Article
id curtin-20.500.11937-4233
institution Curtin University Malaysia
institution_category Local University
last_indexed 2025-11-14T06:01:47Z
publishDate 2008
publisher The American Physical Society
recordtype eprints
repository_type Digital Repository
spelling curtin-20.500.11937-42332017-09-13T14:47:34Z Influence of Temperature and Anisotropic Pressure on the Phase Transitions in α-Cristobalite Donadio, D. Martoňák, R. Raiteri, Paolo Parrinello, M. The role of temperature and anisotropy of the applied load in the pressure–induced transformations of α -cristobalite is investigated by means of first principles molecular dynamics combined with the metadynamics algorithm for the study of solid-solid phase transitions. We reproduce the transition to α-PbO2 as found in experiments and we observe that the transition paths are qualitatively different and yield different products when a nonhydrostatic load is applied, giving rise to a new class of metastable structures with mixed tetrahedral and octahedral coordination. 2008 Journal Article http://hdl.handle.net/20.500.11937/4233 10.1103/PhysRevLett.100.165502 The American Physical Society fulltext
spellingShingle Donadio, D.
Martoňák, R.
Raiteri, Paolo
Parrinello, M.
Influence of Temperature and Anisotropic Pressure on the Phase Transitions in α-Cristobalite
title Influence of Temperature and Anisotropic Pressure on the Phase Transitions in α-Cristobalite
title_full Influence of Temperature and Anisotropic Pressure on the Phase Transitions in α-Cristobalite
title_fullStr Influence of Temperature and Anisotropic Pressure on the Phase Transitions in α-Cristobalite
title_full_unstemmed Influence of Temperature and Anisotropic Pressure on the Phase Transitions in α-Cristobalite
title_short Influence of Temperature and Anisotropic Pressure on the Phase Transitions in α-Cristobalite
title_sort influence of temperature and anisotropic pressure on the phase transitions in α-cristobalite
url http://hdl.handle.net/20.500.11937/4233