Characterization of the mechanisms controlling the permeability changes of fractured cements flowed through by CO2-rich brine

Experiments were conducted to assess the potential impact of fractured well-cement degradation on leakage rate. Permeability was monitored while CO2-enriched reservoir-equilibrated brine was flowed at constant rate through a single fracture in a class G cement core under conditions mimicking geologi...

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Main Authors: Abdoulghafour, Halidi, Luquot, L., Gouze, P.
Format: Journal Article
Published: 2013
Online Access:http://hdl.handle.net/20.500.11937/4222
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author Abdoulghafour, Halidi
Luquot, L.
Gouze, P.
author_facet Abdoulghafour, Halidi
Luquot, L.
Gouze, P.
author_sort Abdoulghafour, Halidi
building Curtin Institutional Repository
collection Online Access
description Experiments were conducted to assess the potential impact of fractured well-cement degradation on leakage rate. Permeability was monitored while CO2-enriched reservoir-equilibrated brine was flowed at constant rate through a single fracture in a class G cement core under conditions mimicking geologic sequestration environments (temperature 60 C, pressure 10 MPa). The results demonstrate that, at least for the conditions used in the experiment, an initial leakage in a 42 µm aperture fracture (permeability = 1.5 × 10-10 m2) can be self-mitigated due to the decrease of the fracture hydraulic aperture after about 15 h. This decrease results from the development of continuous highly hydrated amorphous Si-rich alteration products at the edge of the fracture and the dense carbonation of the bulk cement that mitigate the penetration of the alteration front. © 2013 American Chemical Society.
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spelling curtin-20.500.11937-42222017-09-13T14:44:36Z Characterization of the mechanisms controlling the permeability changes of fractured cements flowed through by CO2-rich brine Abdoulghafour, Halidi Luquot, L. Gouze, P. Experiments were conducted to assess the potential impact of fractured well-cement degradation on leakage rate. Permeability was monitored while CO2-enriched reservoir-equilibrated brine was flowed at constant rate through a single fracture in a class G cement core under conditions mimicking geologic sequestration environments (temperature 60 C, pressure 10 MPa). The results demonstrate that, at least for the conditions used in the experiment, an initial leakage in a 42 µm aperture fracture (permeability = 1.5 × 10-10 m2) can be self-mitigated due to the decrease of the fracture hydraulic aperture after about 15 h. This decrease results from the development of continuous highly hydrated amorphous Si-rich alteration products at the edge of the fracture and the dense carbonation of the bulk cement that mitigate the penetration of the alteration front. © 2013 American Chemical Society. 2013 Journal Article http://hdl.handle.net/20.500.11937/4222 10.1021/es401317c restricted
spellingShingle Abdoulghafour, Halidi
Luquot, L.
Gouze, P.
Characterization of the mechanisms controlling the permeability changes of fractured cements flowed through by CO2-rich brine
title Characterization of the mechanisms controlling the permeability changes of fractured cements flowed through by CO2-rich brine
title_full Characterization of the mechanisms controlling the permeability changes of fractured cements flowed through by CO2-rich brine
title_fullStr Characterization of the mechanisms controlling the permeability changes of fractured cements flowed through by CO2-rich brine
title_full_unstemmed Characterization of the mechanisms controlling the permeability changes of fractured cements flowed through by CO2-rich brine
title_short Characterization of the mechanisms controlling the permeability changes of fractured cements flowed through by CO2-rich brine
title_sort characterization of the mechanisms controlling the permeability changes of fractured cements flowed through by co2-rich brine
url http://hdl.handle.net/20.500.11937/4222