Effects of polymerization conditions on the properties of poly(furfuryl alcohol) composite membranes

Poly(furfuryl alcohol) (PFA) composite membranes were prepared by polymerization of furfuryl alcohol (FA) using sulfuric acid (H2SO4) as the catalyst and polysulfone ultrafiltration membrane as the substrate. The membrane samples were characterized by ATR-IR, TGA, SEM, and gas permeation technique....

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Main Authors: He, L., Li, D., Dong, Dehua, Yao, J., Huang, Y., Wang, H.
Format: Journal Article
Published: John Wiley and Sons Inc 2012
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/37748
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author He, L.
Li, D.
Dong, Dehua
Yao, J.
Huang, Y.
Wang, H.
author_facet He, L.
Li, D.
Dong, Dehua
Yao, J.
Huang, Y.
Wang, H.
author_sort He, L.
building Curtin Institutional Repository
collection Online Access
description Poly(furfuryl alcohol) (PFA) composite membranes were prepared by polymerization of furfuryl alcohol (FA) using sulfuric acid (H2SO4) as the catalyst and polysulfone ultrafiltration membrane as the substrate. The membrane samples were characterized by ATR-IR, TGA, SEM, and gas permeation technique. The effects of synthesis conditions including the FA/H2SO4 molar ratio, polymerization temperature, and the type of solvent on the chemical structure, surface morphology, and gas permeation properties of PFA composite membranes were studied. Our results showed that the suitable synthesis conditions for the preparation of PFA composite membranes with smooth surfaces and uniform structure include (1) FA/H2SO4 molar ratios: 74-300, (2) polymerization temperatures: 80–100°C, and (3) solvents: ethanol and acetone. The PFA composite membrane prepared with a FA/H2SO4 molar ratio of 250, a polymerization temperature of 80°C and ethanol as the solvent exhibited the highest H2/N2 ideal selectivity (xH2/N2 ), and a H2 permeability of 206 Barrers.
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institution Curtin University Malaysia
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spelling curtin-20.500.11937-377482017-09-13T16:08:34Z Effects of polymerization conditions on the properties of poly(furfuryl alcohol) composite membranes He, L. Li, D. Dong, Dehua Yao, J. Huang, Y. Wang, H. composite membrane poly(furfuryl alcohol) characterization gas permeation polymerization Poly(furfuryl alcohol) (PFA) composite membranes were prepared by polymerization of furfuryl alcohol (FA) using sulfuric acid (H2SO4) as the catalyst and polysulfone ultrafiltration membrane as the substrate. The membrane samples were characterized by ATR-IR, TGA, SEM, and gas permeation technique. The effects of synthesis conditions including the FA/H2SO4 molar ratio, polymerization temperature, and the type of solvent on the chemical structure, surface morphology, and gas permeation properties of PFA composite membranes were studied. Our results showed that the suitable synthesis conditions for the preparation of PFA composite membranes with smooth surfaces and uniform structure include (1) FA/H2SO4 molar ratios: 74-300, (2) polymerization temperatures: 80–100°C, and (3) solvents: ethanol and acetone. The PFA composite membrane prepared with a FA/H2SO4 molar ratio of 250, a polymerization temperature of 80°C and ethanol as the solvent exhibited the highest H2/N2 ideal selectivity (xH2/N2 ), and a H2 permeability of 206 Barrers. 2012 Journal Article http://hdl.handle.net/20.500.11937/37748 10.1002/app.35356 John Wiley and Sons Inc restricted
spellingShingle composite membrane
poly(furfuryl alcohol)
characterization
gas permeation
polymerization
He, L.
Li, D.
Dong, Dehua
Yao, J.
Huang, Y.
Wang, H.
Effects of polymerization conditions on the properties of poly(furfuryl alcohol) composite membranes
title Effects of polymerization conditions on the properties of poly(furfuryl alcohol) composite membranes
title_full Effects of polymerization conditions on the properties of poly(furfuryl alcohol) composite membranes
title_fullStr Effects of polymerization conditions on the properties of poly(furfuryl alcohol) composite membranes
title_full_unstemmed Effects of polymerization conditions on the properties of poly(furfuryl alcohol) composite membranes
title_short Effects of polymerization conditions on the properties of poly(furfuryl alcohol) composite membranes
title_sort effects of polymerization conditions on the properties of poly(furfuryl alcohol) composite membranes
topic composite membrane
poly(furfuryl alcohol)
characterization
gas permeation
polymerization
url http://hdl.handle.net/20.500.11937/37748