Structural variations in metal complexes of a tertiary α-hydroxyoxime

Despite the long term interest in hydroxyoximes as metal ion extractants, there is a lack of information on the possible coordination modes these ligands can assume, particularly in concert with a co-ligand. This is pertinent to the use of these extractants in synergistic systems, where a combinatio...

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Main Authors: D'Alessio, D., Lombardo, D., Vaughan, J., Skelton, B., Barnard, K., Ogden, Mark
Format: Journal Article
Published: Royal Society of Chemistry 2015
Online Access:http://hdl.handle.net/20.500.11937/37410
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author D'Alessio, D.
Lombardo, D.
Vaughan, J.
Skelton, B.
Barnard, K.
Ogden, Mark
author_facet D'Alessio, D.
Lombardo, D.
Vaughan, J.
Skelton, B.
Barnard, K.
Ogden, Mark
author_sort D'Alessio, D.
building Curtin Institutional Repository
collection Online Access
description Despite the long term interest in hydroxyoximes as metal ion extractants, there is a lack of information on the possible coordination modes these ligands can assume, particularly in concert with a co-ligand. This is pertinent to the use of these extractants in synergistic systems, where a combination of extractants can achieve commercially useful results. We report here the structures of some metal complexes (M = Mn, Co, Ni, Cu, and Zn) with (1-hydroxycyclohexyl)-phenyl ketone oxime. The results demonstrate that this ligand can support complexes ranging from mononuclear to trinuclear, in association with anionic and neutral co-ligands in some cases. While these results have been obtained in the solid state, they illustrate a range of possible species that may be formed in extractant solutions.
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spelling curtin-20.500.11937-374102018-04-20T07:40:54Z Structural variations in metal complexes of a tertiary α-hydroxyoxime D'Alessio, D. Lombardo, D. Vaughan, J. Skelton, B. Barnard, K. Ogden, Mark Despite the long term interest in hydroxyoximes as metal ion extractants, there is a lack of information on the possible coordination modes these ligands can assume, particularly in concert with a co-ligand. This is pertinent to the use of these extractants in synergistic systems, where a combination of extractants can achieve commercially useful results. We report here the structures of some metal complexes (M = Mn, Co, Ni, Cu, and Zn) with (1-hydroxycyclohexyl)-phenyl ketone oxime. The results demonstrate that this ligand can support complexes ranging from mononuclear to trinuclear, in association with anionic and neutral co-ligands in some cases. While these results have been obtained in the solid state, they illustrate a range of possible species that may be formed in extractant solutions. 2015 Journal Article http://hdl.handle.net/20.500.11937/37410 10.1039/c4dt03393k Royal Society of Chemistry fulltext
spellingShingle D'Alessio, D.
Lombardo, D.
Vaughan, J.
Skelton, B.
Barnard, K.
Ogden, Mark
Structural variations in metal complexes of a tertiary α-hydroxyoxime
title Structural variations in metal complexes of a tertiary α-hydroxyoxime
title_full Structural variations in metal complexes of a tertiary α-hydroxyoxime
title_fullStr Structural variations in metal complexes of a tertiary α-hydroxyoxime
title_full_unstemmed Structural variations in metal complexes of a tertiary α-hydroxyoxime
title_short Structural variations in metal complexes of a tertiary α-hydroxyoxime
title_sort structural variations in metal complexes of a tertiary α-hydroxyoxime
url http://hdl.handle.net/20.500.11937/37410