Fabrication of n-type CuInS2 modified TiO2 nanotube arrays heterostructure photoelectrode with enhanced photoelectrocatalytic properties

A novel n-type CuInS2 modified TiO2 nanotube arrays (NTs) heterostructure photoelectrode was successfully prepared via an ultrasonication-assisted cathodic electrodeposition strategy. CuInS2 particles were uniformly decorated on the inner and external walls of the TiO2 NTs electrode. The stoichiomet...

Full description

Bibliographic Details
Main Authors: Li, T., Li, Xin Yong, Zhao, Q., Shi, Y., Teng, W.
Format: Journal Article
Published: Elsevier 2014
Online Access:http://hdl.handle.net/20.500.11937/3523
_version_ 1848744255532564480
author Li, T.
Li, Xin Yong
Zhao, Q.
Shi, Y.
Teng, W.
author_facet Li, T.
Li, Xin Yong
Zhao, Q.
Shi, Y.
Teng, W.
author_sort Li, T.
building Curtin Institutional Repository
collection Online Access
description A novel n-type CuInS2 modified TiO2 nanotube arrays (NTs) heterostructure photoelectrode was successfully prepared via an ultrasonication-assisted cathodic electrodeposition strategy. CuInS2 particles were uniformly decorated on the inner and external walls of the TiO2 NTs electrode. The stoichiometry measured by XPS and ICP-OES clearly illustrated the excess indium. Mott–Schottky analysis further demonstrated CuInS2 possessed an n-type feature. Optical characterizations indicated that the introduced CuInS2 could extend the visible-light response range and enhance the visible light photoactivity. Moreover, the electrochemical measurements attested to a significant improvement of the interfacial electron-transfer properties. The photoelectrocatalytic (PEC) activity of CuInS2/TiO2 NTs electrode was evaluated by degradation of 2-chlorophenol (2-CP) under visible light irradiation (λ > 420 nm). The results indicated that the as-prepared CuInS2/TiO2 NTs electrode displayed much higher PEC performance than that of the pure TiO2 NTs electrode.
first_indexed 2025-11-14T05:58:34Z
format Journal Article
id curtin-20.500.11937-3523
institution Curtin University Malaysia
institution_category Local University
last_indexed 2025-11-14T05:58:34Z
publishDate 2014
publisher Elsevier
recordtype eprints
repository_type Digital Repository
spelling curtin-20.500.11937-35232017-09-13T14:43:26Z Fabrication of n-type CuInS2 modified TiO2 nanotube arrays heterostructure photoelectrode with enhanced photoelectrocatalytic properties Li, T. Li, Xin Yong Zhao, Q. Shi, Y. Teng, W. A novel n-type CuInS2 modified TiO2 nanotube arrays (NTs) heterostructure photoelectrode was successfully prepared via an ultrasonication-assisted cathodic electrodeposition strategy. CuInS2 particles were uniformly decorated on the inner and external walls of the TiO2 NTs electrode. The stoichiometry measured by XPS and ICP-OES clearly illustrated the excess indium. Mott–Schottky analysis further demonstrated CuInS2 possessed an n-type feature. Optical characterizations indicated that the introduced CuInS2 could extend the visible-light response range and enhance the visible light photoactivity. Moreover, the electrochemical measurements attested to a significant improvement of the interfacial electron-transfer properties. The photoelectrocatalytic (PEC) activity of CuInS2/TiO2 NTs electrode was evaluated by degradation of 2-chlorophenol (2-CP) under visible light irradiation (λ > 420 nm). The results indicated that the as-prepared CuInS2/TiO2 NTs electrode displayed much higher PEC performance than that of the pure TiO2 NTs electrode. 2014 Journal Article http://hdl.handle.net/20.500.11937/3523 10.1016/j.apcatb.2014.03.035 Elsevier restricted
spellingShingle Li, T.
Li, Xin Yong
Zhao, Q.
Shi, Y.
Teng, W.
Fabrication of n-type CuInS2 modified TiO2 nanotube arrays heterostructure photoelectrode with enhanced photoelectrocatalytic properties
title Fabrication of n-type CuInS2 modified TiO2 nanotube arrays heterostructure photoelectrode with enhanced photoelectrocatalytic properties
title_full Fabrication of n-type CuInS2 modified TiO2 nanotube arrays heterostructure photoelectrode with enhanced photoelectrocatalytic properties
title_fullStr Fabrication of n-type CuInS2 modified TiO2 nanotube arrays heterostructure photoelectrode with enhanced photoelectrocatalytic properties
title_full_unstemmed Fabrication of n-type CuInS2 modified TiO2 nanotube arrays heterostructure photoelectrode with enhanced photoelectrocatalytic properties
title_short Fabrication of n-type CuInS2 modified TiO2 nanotube arrays heterostructure photoelectrode with enhanced photoelectrocatalytic properties
title_sort fabrication of n-type cuins2 modified tio2 nanotube arrays heterostructure photoelectrode with enhanced photoelectrocatalytic properties
url http://hdl.handle.net/20.500.11937/3523