A new synthesis of 2,8-disubstituted pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidines

A practical synthesis of pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidines, which are key intermediates inthe preparation of adenosine receptor antagonists, is developed. The method allows introduction of avariety of aryl substituents at position 2 of the pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidi...

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Main Authors: Dolzhenko, Anton, Pastorin, G., Dolzhenko, A., Chui, W.
Format: Journal Article
Published: Elsevier Science Limted 2009
Online Access:http://hdl.handle.net/20.500.11937/35003
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author Dolzhenko, Anton
Pastorin, G.
Dolzhenko, A.
Chui, W.
author_facet Dolzhenko, Anton
Pastorin, G.
Dolzhenko, A.
Chui, W.
author_sort Dolzhenko, Anton
building Curtin Institutional Repository
collection Online Access
description A practical synthesis of pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidines, which are key intermediates inthe preparation of adenosine receptor antagonists, is developed. The method allows introduction of avariety of aryl substituents at position 2 of the pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidine systemvia cyclocondensation of 5-amino-4-iminopyrazolo[3,4-d]pyrimidine with benzaldehydes accompaniedwith oxidation by iodobenzene diacetate. Some unexpected reactions are observed and the structuresof the products are confirmed using NMR spectroscopy and X-ray crystallography.
first_indexed 2025-11-14T08:39:27Z
format Journal Article
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institution Curtin University Malaysia
institution_category Local University
last_indexed 2025-11-14T08:39:27Z
publishDate 2009
publisher Elsevier Science Limted
recordtype eprints
repository_type Digital Repository
spelling curtin-20.500.11937-350032017-09-13T16:07:33Z A new synthesis of 2,8-disubstituted pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidines Dolzhenko, Anton Pastorin, G. Dolzhenko, A. Chui, W. A practical synthesis of pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidines, which are key intermediates inthe preparation of adenosine receptor antagonists, is developed. The method allows introduction of avariety of aryl substituents at position 2 of the pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidine systemvia cyclocondensation of 5-amino-4-iminopyrazolo[3,4-d]pyrimidine with benzaldehydes accompaniedwith oxidation by iodobenzene diacetate. Some unexpected reactions are observed and the structuresof the products are confirmed using NMR spectroscopy and X-ray crystallography. 2009 Journal Article http://hdl.handle.net/20.500.11937/35003 10.1016/j.tetlet.2009.07.113 Elsevier Science Limted restricted
spellingShingle Dolzhenko, Anton
Pastorin, G.
Dolzhenko, A.
Chui, W.
A new synthesis of 2,8-disubstituted pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidines
title A new synthesis of 2,8-disubstituted pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidines
title_full A new synthesis of 2,8-disubstituted pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidines
title_fullStr A new synthesis of 2,8-disubstituted pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidines
title_full_unstemmed A new synthesis of 2,8-disubstituted pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidines
title_short A new synthesis of 2,8-disubstituted pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidines
title_sort new synthesis of 2,8-disubstituted pyrazolo[4,3-e][1,2,4]triazolo[1,5-c]pyrimidines
url http://hdl.handle.net/20.500.11937/35003