A novel approach to formulate high flux multifunctional ultrafiltration membranes from photocatalytic titania composite precursors on multi-channel tubular substrates

© 2016 The Royal Society of Chemistry.Anatase rich titanium dioxide ultrafiltration membranes with high filtration rates have been successfully developed on multi-channel tubular alumina substrates via aqueous sol-gel method from titania-alumina composite precursors containing 30 wt% alumina. The co...

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Main Authors: Manjumol, K., Sankar, S., Nair, Balagopal, Midhun, M., Mohamed, P., Warrier, K.
Format: Journal Article
Published: Royal Society of Chemistry 2016
Online Access:http://hdl.handle.net/20.500.11937/31906
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author Manjumol, K.
Sankar, S.
Nair, Balagopal
Midhun, M.
Mohamed, P.
Warrier, K.
author_facet Manjumol, K.
Sankar, S.
Nair, Balagopal
Midhun, M.
Mohamed, P.
Warrier, K.
author_sort Manjumol, K.
building Curtin Institutional Repository
collection Online Access
description © 2016 The Royal Society of Chemistry.Anatase rich titanium dioxide ultrafiltration membranes with high filtration rates have been successfully developed on multi-channel tubular alumina substrates via aqueous sol-gel method from titania-alumina composite precursors containing 30 wt% alumina. The composite membrane material exhibited anatase phase stability above 800 °C and retained a BET surface area of 64 m2 g-1 even after calcination at 700 °C. Supported membranes on multi-channel substrates with an active layer thickness of 4 µm gave a water flux value of 215 L m-2 h-1 coupled with 80% rejection of Bovine Serum Albumin (BSA) with molecular weight 66 kD at 2 bar pressure. This is much higher compared to a flux of 27 L m-2 h-1 obtained for a single component titania membrane layer. The composite membrane materials showed excellent photocatalytic activity under UV irradiation such that a solution containing Methylene Blue (MB) dye showed 96% dye degradation within 2 h. Porous disc shaped substrates coated with the active titania composite layer showed methylene blue degradation of 44% under identical conditions. The present results point towards an excellent pathway for the development of multifunctional ultra-filtration membranes for water purification and also for other separation applications where separation together with photocatalysis will be of great importance.
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publishDate 2016
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spelling curtin-20.500.11937-319062017-09-13T15:15:33Z A novel approach to formulate high flux multifunctional ultrafiltration membranes from photocatalytic titania composite precursors on multi-channel tubular substrates Manjumol, K. Sankar, S. Nair, Balagopal Midhun, M. Mohamed, P. Warrier, K. © 2016 The Royal Society of Chemistry.Anatase rich titanium dioxide ultrafiltration membranes with high filtration rates have been successfully developed on multi-channel tubular alumina substrates via aqueous sol-gel method from titania-alumina composite precursors containing 30 wt% alumina. The composite membrane material exhibited anatase phase stability above 800 °C and retained a BET surface area of 64 m2 g-1 even after calcination at 700 °C. Supported membranes on multi-channel substrates with an active layer thickness of 4 µm gave a water flux value of 215 L m-2 h-1 coupled with 80% rejection of Bovine Serum Albumin (BSA) with molecular weight 66 kD at 2 bar pressure. This is much higher compared to a flux of 27 L m-2 h-1 obtained for a single component titania membrane layer. The composite membrane materials showed excellent photocatalytic activity under UV irradiation such that a solution containing Methylene Blue (MB) dye showed 96% dye degradation within 2 h. Porous disc shaped substrates coated with the active titania composite layer showed methylene blue degradation of 44% under identical conditions. The present results point towards an excellent pathway for the development of multifunctional ultra-filtration membranes for water purification and also for other separation applications where separation together with photocatalysis will be of great importance. 2016 Journal Article http://hdl.handle.net/20.500.11937/31906 10.1039/c6ra14117j Royal Society of Chemistry restricted
spellingShingle Manjumol, K.
Sankar, S.
Nair, Balagopal
Midhun, M.
Mohamed, P.
Warrier, K.
A novel approach to formulate high flux multifunctional ultrafiltration membranes from photocatalytic titania composite precursors on multi-channel tubular substrates
title A novel approach to formulate high flux multifunctional ultrafiltration membranes from photocatalytic titania composite precursors on multi-channel tubular substrates
title_full A novel approach to formulate high flux multifunctional ultrafiltration membranes from photocatalytic titania composite precursors on multi-channel tubular substrates
title_fullStr A novel approach to formulate high flux multifunctional ultrafiltration membranes from photocatalytic titania composite precursors on multi-channel tubular substrates
title_full_unstemmed A novel approach to formulate high flux multifunctional ultrafiltration membranes from photocatalytic titania composite precursors on multi-channel tubular substrates
title_short A novel approach to formulate high flux multifunctional ultrafiltration membranes from photocatalytic titania composite precursors on multi-channel tubular substrates
title_sort novel approach to formulate high flux multifunctional ultrafiltration membranes from photocatalytic titania composite precursors on multi-channel tubular substrates
url http://hdl.handle.net/20.500.11937/31906