Biosorption of heavy metals from aqueous solutions with tobacco dust

A typical lignocellulosic agricultural residue, namely tobaccodust, was investigated for its heavymetal binding efficiency. The tobaccodust exhibited a strong capacity for heavymetals, such as Pb(II), Cu(II), Cd(II), Zn(II) and Ni(II), with respective equilibrium loadings of 39.6, 36.0, 29.6, 25.1 a...

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Main Authors: Qi, B., Aldrich, Chris
Format: Journal Article
Published: Elsevier BV 2008
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/31517
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author Qi, B.
Aldrich, Chris
author_facet Qi, B.
Aldrich, Chris
author_sort Qi, B.
building Curtin Institutional Repository
collection Online Access
description A typical lignocellulosic agricultural residue, namely tobaccodust, was investigated for its heavymetal binding efficiency. The tobaccodust exhibited a strong capacity for heavymetals, such as Pb(II), Cu(II), Cd(II), Zn(II) and Ni(II), with respective equilibrium loadings of 39.6, 36.0, 29.6, 25.1 and 24.5 mg of metal per g of sorbent. Moreover, the heavymetals loaded onto the biosorbent could be released easily with a dilute HCl solution. Zeta potential and surface acidity measurements showed that the tobaccodust was negatively charged over a wide pH range (pH > 2), with a strong surface acidity and a high OH- adsorption capacity. Changes in the surface morphology of the tobaccodust as visualized by atomic force microscopy suggested that the sorption of heavymetal ions on the tobacco could be associated with changes in the surface properties of the dust particles. These surface changes appeared to have resulted from a loss of some of the structures on the surface of the particles, owing to leaching in the acid metal ion solution. However, Fourier transform infrared spectroscopy (FTIR) showed no substantial change in the chemical structure of the tobaccodust subjected to biosorption. The heavymetal uptake by the tobaccodust may be interpreted as metal–H ion exchange or metal ion surface complexation adsorption or both.
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spelling curtin-20.500.11937-315172017-09-13T15:21:25Z Biosorption of heavy metals from aqueous solutions with tobacco dust Qi, B. Aldrich, Chris Heavymetals Biosorption Tobacco Lignocellulose A typical lignocellulosic agricultural residue, namely tobaccodust, was investigated for its heavymetal binding efficiency. The tobaccodust exhibited a strong capacity for heavymetals, such as Pb(II), Cu(II), Cd(II), Zn(II) and Ni(II), with respective equilibrium loadings of 39.6, 36.0, 29.6, 25.1 and 24.5 mg of metal per g of sorbent. Moreover, the heavymetals loaded onto the biosorbent could be released easily with a dilute HCl solution. Zeta potential and surface acidity measurements showed that the tobaccodust was negatively charged over a wide pH range (pH > 2), with a strong surface acidity and a high OH- adsorption capacity. Changes in the surface morphology of the tobaccodust as visualized by atomic force microscopy suggested that the sorption of heavymetal ions on the tobacco could be associated with changes in the surface properties of the dust particles. These surface changes appeared to have resulted from a loss of some of the structures on the surface of the particles, owing to leaching in the acid metal ion solution. However, Fourier transform infrared spectroscopy (FTIR) showed no substantial change in the chemical structure of the tobaccodust subjected to biosorption. The heavymetal uptake by the tobaccodust may be interpreted as metal–H ion exchange or metal ion surface complexation adsorption or both. 2008 Journal Article http://hdl.handle.net/20.500.11937/31517 10.1016/j.biortech.2007.10.042 Elsevier BV restricted
spellingShingle Heavymetals
Biosorption
Tobacco
Lignocellulose
Qi, B.
Aldrich, Chris
Biosorption of heavy metals from aqueous solutions with tobacco dust
title Biosorption of heavy metals from aqueous solutions with tobacco dust
title_full Biosorption of heavy metals from aqueous solutions with tobacco dust
title_fullStr Biosorption of heavy metals from aqueous solutions with tobacco dust
title_full_unstemmed Biosorption of heavy metals from aqueous solutions with tobacco dust
title_short Biosorption of heavy metals from aqueous solutions with tobacco dust
title_sort biosorption of heavy metals from aqueous solutions with tobacco dust
topic Heavymetals
Biosorption
Tobacco
Lignocellulose
url http://hdl.handle.net/20.500.11937/31517