X-Ray Diffraction Study on the In-Situ Crystallisation Kinetics in Electrospun PVP/TiO2 Nanofibers

Nanostructured TiO2 has received much attention recently owing to their promising physical properties for photocatalytic applications. The process of photocatalysis is closely related to the electronic band gap which is controlled by shape, surface area and particle size. Elongated structures such a...

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Main Authors: Albetran, Hani, Alsafwan, Asmahan, Haroosh, Hazim, Dong, Yu, Low, It Meng
Other Authors: Sanjay Mathur
Format: Conference Paper
Published: John Wiley & Sons 2014
Subjects:
Online Access:http://hdl.handle.net/20.500.11937/3045
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author Albetran, Hani
Alsafwan, Asmahan
Haroosh, Hazim
Dong, Yu
Low, It Meng
author2 Sanjay Mathur
author_facet Sanjay Mathur
Albetran, Hani
Alsafwan, Asmahan
Haroosh, Hazim
Dong, Yu
Low, It Meng
author_sort Albetran, Hani
building Curtin Institutional Repository
collection Online Access
description Nanostructured TiO2 has received much attention recently owing to their promising physical properties for photocatalytic applications. The process of photocatalysis is closely related to the electronic band gap which is controlled by shape, surface area and particle size. Elongated structures such as nanofibres are of particular importance because they can provide a high specific surface area for photocatalysis. In this paper, the effect of atmosphere and doping on the crystallisation kinetics of electrospun TiO2 nanofibers has been investigated using high-temperature synchrotron radiation diffraction. Electrospun TiO2 nanofibers were synthesized using titanium isopropoxide, poly (vinyl-pyrrolidone) as a polymer binder, and acetic acid and ethanol as a solvent. Diffraction results showed that the as-synthesized TiO2 nanofibres were amorphous initially but when heated in air they crystallized to form anatase and rutile at 600 °C and 700 °C respectively. However, in argon atmosphere, anatase and rutile formed simultaneously at 700 °C. In the presence of vanadium dopant, both anatase and rutile formed in concert at 500 °C. The effects of atmosphere and doping on the crystallisation kinetics and phase stability of TiO2 nanofibres at elevated temperature are discussed.
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institution Curtin University Malaysia
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publishDate 2014
publisher John Wiley & Sons
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spelling curtin-20.500.11937-30452023-02-13T08:01:36Z X-Ray Diffraction Study on the In-Situ Crystallisation Kinetics in Electrospun PVP/TiO2 Nanofibers Albetran, Hani Alsafwan, Asmahan Haroosh, Hazim Dong, Yu Low, It Meng Sanjay Mathur Francisco Hernandez-Ramirez TiO2 Electrospinning In-situ crystallisation X-ray diffraction analysis Nanostructured TiO2 has received much attention recently owing to their promising physical properties for photocatalytic applications. The process of photocatalysis is closely related to the electronic band gap which is controlled by shape, surface area and particle size. Elongated structures such as nanofibres are of particular importance because they can provide a high specific surface area for photocatalysis. In this paper, the effect of atmosphere and doping on the crystallisation kinetics of electrospun TiO2 nanofibers has been investigated using high-temperature synchrotron radiation diffraction. Electrospun TiO2 nanofibers were synthesized using titanium isopropoxide, poly (vinyl-pyrrolidone) as a polymer binder, and acetic acid and ethanol as a solvent. Diffraction results showed that the as-synthesized TiO2 nanofibres were amorphous initially but when heated in air they crystallized to form anatase and rutile at 600 °C and 700 °C respectively. However, in argon atmosphere, anatase and rutile formed simultaneously at 700 °C. In the presence of vanadium dopant, both anatase and rutile formed in concert at 500 °C. The effects of atmosphere and doping on the crystallisation kinetics and phase stability of TiO2 nanofibres at elevated temperature are discussed. 2014 Conference Paper http://hdl.handle.net/20.500.11937/3045 John Wiley & Sons restricted
spellingShingle TiO2
Electrospinning
In-situ crystallisation
X-ray diffraction analysis
Albetran, Hani
Alsafwan, Asmahan
Haroosh, Hazim
Dong, Yu
Low, It Meng
X-Ray Diffraction Study on the In-Situ Crystallisation Kinetics in Electrospun PVP/TiO2 Nanofibers
title X-Ray Diffraction Study on the In-Situ Crystallisation Kinetics in Electrospun PVP/TiO2 Nanofibers
title_full X-Ray Diffraction Study on the In-Situ Crystallisation Kinetics in Electrospun PVP/TiO2 Nanofibers
title_fullStr X-Ray Diffraction Study on the In-Situ Crystallisation Kinetics in Electrospun PVP/TiO2 Nanofibers
title_full_unstemmed X-Ray Diffraction Study on the In-Situ Crystallisation Kinetics in Electrospun PVP/TiO2 Nanofibers
title_short X-Ray Diffraction Study on the In-Situ Crystallisation Kinetics in Electrospun PVP/TiO2 Nanofibers
title_sort x-ray diffraction study on the in-situ crystallisation kinetics in electrospun pvp/tio2 nanofibers
topic TiO2
Electrospinning
In-situ crystallisation
X-ray diffraction analysis
url http://hdl.handle.net/20.500.11937/3045