Hydrothermal synthesis of ternary α-Fe2O3–ZnO–Au nano composites with high gas-sensing performance

This study reports facile hydrothermal strategies for the synthesis of novel ternary α-Fe2O3–ZnO–Au nanocomposites under mild conditions, through further surface coating of ZnO and Au nanoparticles (NPs) on α-Fe2O3 nanorods. The ternary α-Fe2O3–ZnO–Au nanocomposites are found to show (1) higher sens...

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Main Authors: Yusuf Valentino Kaneti, Julien Moriceau, Minsu Liu, Yuan Yuan, Quadir, Md Zakaria, Xuchuan Jiang, Aibing Yu
Format: Journal Article
Published: Elsevier 2014
Online Access:http://hdl.handle.net/20.500.11937/28299
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author Yusuf Valentino Kaneti
Julien Moriceau
Minsu Liu
Yuan Yuan
Quadir, Md Zakaria
Xuchuan Jiang
Aibing Yu
author_facet Yusuf Valentino Kaneti
Julien Moriceau
Minsu Liu
Yuan Yuan
Quadir, Md Zakaria
Xuchuan Jiang
Aibing Yu
author_sort Yusuf Valentino Kaneti
building Curtin Institutional Repository
collection Online Access
description This study reports facile hydrothermal strategies for the synthesis of novel ternary α-Fe2O3–ZnO–Au nanocomposites under mild conditions, through further surface coating of ZnO and Au nanoparticles (NPs) on α-Fe2O3 nanorods. The ternary α-Fe2O3–ZnO–Au nanocomposites are found to show (1) higher sensitivity/responses (S) of 113 and 57 toward 100-ppm n-butanol and acetone, respectively compared to single α-Fe2O3 (S = 11.7, 9.1 for n-butanol, acetone) and binary α-Fe2O3-ZnO (S = 54.4, 28 for n-butanol, acetone) sensing materials, and (2) lower optimum operating temperature, i.e., 225 °C. The enhanced sensitivity could be attributed to the chemical sensitization effect induced by the Au NPs, and the existence of conjugated depletion layers in the nanocomposites which promote a greater drop in resistance upon exposure to the gas. These results will be useful for future design of iron oxide-based ternary nanocomposites as gas-sensing materials with high sensitivity, selectivity and stability.
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format Journal Article
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institution Curtin University Malaysia
institution_category Local University
last_indexed 2025-11-14T08:09:35Z
publishDate 2014
publisher Elsevier
recordtype eprints
repository_type Digital Repository
spelling curtin-20.500.11937-282992017-01-30T13:04:15Z Hydrothermal synthesis of ternary α-Fe2O3–ZnO–Au nano composites with high gas-sensing performance Yusuf Valentino Kaneti Julien Moriceau Minsu Liu Yuan Yuan Quadir, Md Zakaria Xuchuan Jiang Aibing Yu This study reports facile hydrothermal strategies for the synthesis of novel ternary α-Fe2O3–ZnO–Au nanocomposites under mild conditions, through further surface coating of ZnO and Au nanoparticles (NPs) on α-Fe2O3 nanorods. The ternary α-Fe2O3–ZnO–Au nanocomposites are found to show (1) higher sensitivity/responses (S) of 113 and 57 toward 100-ppm n-butanol and acetone, respectively compared to single α-Fe2O3 (S = 11.7, 9.1 for n-butanol, acetone) and binary α-Fe2O3-ZnO (S = 54.4, 28 for n-butanol, acetone) sensing materials, and (2) lower optimum operating temperature, i.e., 225 °C. The enhanced sensitivity could be attributed to the chemical sensitization effect induced by the Au NPs, and the existence of conjugated depletion layers in the nanocomposites which promote a greater drop in resistance upon exposure to the gas. These results will be useful for future design of iron oxide-based ternary nanocomposites as gas-sensing materials with high sensitivity, selectivity and stability. 2014 Journal Article http://hdl.handle.net/20.500.11937/28299 Elsevier restricted
spellingShingle Yusuf Valentino Kaneti
Julien Moriceau
Minsu Liu
Yuan Yuan
Quadir, Md Zakaria
Xuchuan Jiang
Aibing Yu
Hydrothermal synthesis of ternary α-Fe2O3–ZnO–Au nano composites with high gas-sensing performance
title Hydrothermal synthesis of ternary α-Fe2O3–ZnO–Au nano composites with high gas-sensing performance
title_full Hydrothermal synthesis of ternary α-Fe2O3–ZnO–Au nano composites with high gas-sensing performance
title_fullStr Hydrothermal synthesis of ternary α-Fe2O3–ZnO–Au nano composites with high gas-sensing performance
title_full_unstemmed Hydrothermal synthesis of ternary α-Fe2O3–ZnO–Au nano composites with high gas-sensing performance
title_short Hydrothermal synthesis of ternary α-Fe2O3–ZnO–Au nano composites with high gas-sensing performance
title_sort hydrothermal synthesis of ternary α-fe2o3–zno–au nano composites with high gas-sensing performance
url http://hdl.handle.net/20.500.11937/28299