Macrocyclic alkanes in crude oils from the algaenan of Botryococcus braunii

New classes of biomarkers, macrocyclic alkanes, have been previously identified in high grade oil shales (torbanites, Late Carboniferous-Late Permian) containing remains of the freshwater alga Botryococcus braunii (B. braunii). In this study we report the occurrence of these compounds in two Indones...

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Main Authors: Audino, Michiele, Grice, Kliti, Alexander, Robert, Kagi, Robert
Format: Journal Article
Published: Pergamon-Elsevier 2002
Online Access:http://hdl.handle.net/20.500.11937/27096
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author Audino, Michiele
Grice, Kliti
Alexander, Robert
Kagi, Robert
author_facet Audino, Michiele
Grice, Kliti
Alexander, Robert
Kagi, Robert
author_sort Audino, Michiele
building Curtin Institutional Repository
collection Online Access
description New classes of biomarkers, macrocyclic alkanes, have been previously identified in high grade oil shales (torbanites, Late Carboniferous-Late Permian) containing remains of the freshwater alga Botryococcus braunii (B. braunii). In this study we report the occurrence of these compounds in two Indonesian crude oils (Minas and Duri, Tertiary) utilising metastable reaction monitoring GC?MS experiments. Based on 13C data and the distributions of the macrocyclic alkanes we suggest that the macrocyclic alkanes are likely formed by an olefin metathesis reaction of a structurallyspecificpolyunsaturated precursor i.e. the algaenan of B. braunii. The macrocyclic alkanes appear to be novel markers of B. braunii and add to the catalogue of the characteristic hydrocarbons derived from this alga. More importantly, these components could be original markers specific to the highly resistant algaenan of B. braunii in sediments and crude oils, unlike n-alkanes which can have multiple origins.
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spelling curtin-20.500.11937-270962017-09-13T16:08:11Z Macrocyclic alkanes in crude oils from the algaenan of Botryococcus braunii Audino, Michiele Grice, Kliti Alexander, Robert Kagi, Robert New classes of biomarkers, macrocyclic alkanes, have been previously identified in high grade oil shales (torbanites, Late Carboniferous-Late Permian) containing remains of the freshwater alga Botryococcus braunii (B. braunii). In this study we report the occurrence of these compounds in two Indonesian crude oils (Minas and Duri, Tertiary) utilising metastable reaction monitoring GC?MS experiments. Based on 13C data and the distributions of the macrocyclic alkanes we suggest that the macrocyclic alkanes are likely formed by an olefin metathesis reaction of a structurallyspecificpolyunsaturated precursor i.e. the algaenan of B. braunii. The macrocyclic alkanes appear to be novel markers of B. braunii and add to the catalogue of the characteristic hydrocarbons derived from this alga. More importantly, these components could be original markers specific to the highly resistant algaenan of B. braunii in sediments and crude oils, unlike n-alkanes which can have multiple origins. 2002 Journal Article http://hdl.handle.net/20.500.11937/27096 10.1016/S0146-6380(02)00061-X Pergamon-Elsevier restricted
spellingShingle Audino, Michiele
Grice, Kliti
Alexander, Robert
Kagi, Robert
Macrocyclic alkanes in crude oils from the algaenan of Botryococcus braunii
title Macrocyclic alkanes in crude oils from the algaenan of Botryococcus braunii
title_full Macrocyclic alkanes in crude oils from the algaenan of Botryococcus braunii
title_fullStr Macrocyclic alkanes in crude oils from the algaenan of Botryococcus braunii
title_full_unstemmed Macrocyclic alkanes in crude oils from the algaenan of Botryococcus braunii
title_short Macrocyclic alkanes in crude oils from the algaenan of Botryococcus braunii
title_sort macrocyclic alkanes in crude oils from the algaenan of botryococcus braunii
url http://hdl.handle.net/20.500.11937/27096