A Comparative Study of the Performance of SrCo0.76Fe0.19Al0.1Ox and (SrCo0.8Fe0.2O3-deltda)0.95(SrAl2O4)0.05 Mixed-Conducting Membranes

Dense oxygen permeable ceramic membranes are promising materials for separating oxygen from air and for syngas production. The crystal structure, oxygen vacancy, microstructure, thermal expansion behavior, electrical conductivity, and oxygen permeability of two mixed-conducting ceramics: 5 mol% SrAl...

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Main Authors: Zhu, N., Zhang, G., Liu, Z., Dong, X., Jin, W., Liu, Shaomin
Format: Journal Article
Published: Wiley-Blackwell Publishing, Inc. 2013
Online Access:http://hdl.handle.net/20.500.11937/25462
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author Zhu, N.
Zhang, G.
Liu, Z.
Dong, X.
Jin, W.
Liu, Shaomin
author_facet Zhu, N.
Zhang, G.
Liu, Z.
Dong, X.
Jin, W.
Liu, Shaomin
author_sort Zhu, N.
building Curtin Institutional Repository
collection Online Access
description Dense oxygen permeable ceramic membranes are promising materials for separating oxygen from air and for syngas production. The crystal structure, oxygen vacancy, microstructure, thermal expansion behavior, electrical conductivity, and oxygen permeability of two mixed-conducting ceramics: 5 mol% SrAl2O4-doped SrCo0.8Fe0.2O3-delta (SCF-SA) and SrCo0.76 Fe0.19Al0.1Ox (SCFA), with the same overall cation composition, were systematically investigated in this work. The main phases of SCFA and SCF-SA are cubic perovskite and no orthorhombic brown millerite appears from 700°C to 900°C in air, while SCF-SA presents minor unidentified phases. SCF-SA shows lower electrical conductivity than SCFA. SCFA membranes exhibit lower oxygen permeation flux than SCF-SA. At 850°C, the oxygen permeation fluxes of SCFA and SCF-SA are 1.23 and 1.46 mL/cm2/min, respectively, under the oxygen partial pressure gradient of 0.21 x 10^5/1 3 10^2 Pa.
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institution Curtin University Malaysia
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publishDate 2013
publisher Wiley-Blackwell Publishing, Inc.
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spelling curtin-20.500.11937-254622017-09-13T15:18:09Z A Comparative Study of the Performance of SrCo0.76Fe0.19Al0.1Ox and (SrCo0.8Fe0.2O3-deltda)0.95(SrAl2O4)0.05 Mixed-Conducting Membranes Zhu, N. Zhang, G. Liu, Z. Dong, X. Jin, W. Liu, Shaomin Dense oxygen permeable ceramic membranes are promising materials for separating oxygen from air and for syngas production. The crystal structure, oxygen vacancy, microstructure, thermal expansion behavior, electrical conductivity, and oxygen permeability of two mixed-conducting ceramics: 5 mol% SrAl2O4-doped SrCo0.8Fe0.2O3-delta (SCF-SA) and SrCo0.76 Fe0.19Al0.1Ox (SCFA), with the same overall cation composition, were systematically investigated in this work. The main phases of SCFA and SCF-SA are cubic perovskite and no orthorhombic brown millerite appears from 700°C to 900°C in air, while SCF-SA presents minor unidentified phases. SCF-SA shows lower electrical conductivity than SCFA. SCFA membranes exhibit lower oxygen permeation flux than SCF-SA. At 850°C, the oxygen permeation fluxes of SCFA and SCF-SA are 1.23 and 1.46 mL/cm2/min, respectively, under the oxygen partial pressure gradient of 0.21 x 10^5/1 3 10^2 Pa. 2013 Journal Article http://hdl.handle.net/20.500.11937/25462 10.1111/jace.12248 Wiley-Blackwell Publishing, Inc. restricted
spellingShingle Zhu, N.
Zhang, G.
Liu, Z.
Dong, X.
Jin, W.
Liu, Shaomin
A Comparative Study of the Performance of SrCo0.76Fe0.19Al0.1Ox and (SrCo0.8Fe0.2O3-deltda)0.95(SrAl2O4)0.05 Mixed-Conducting Membranes
title A Comparative Study of the Performance of SrCo0.76Fe0.19Al0.1Ox and (SrCo0.8Fe0.2O3-deltda)0.95(SrAl2O4)0.05 Mixed-Conducting Membranes
title_full A Comparative Study of the Performance of SrCo0.76Fe0.19Al0.1Ox and (SrCo0.8Fe0.2O3-deltda)0.95(SrAl2O4)0.05 Mixed-Conducting Membranes
title_fullStr A Comparative Study of the Performance of SrCo0.76Fe0.19Al0.1Ox and (SrCo0.8Fe0.2O3-deltda)0.95(SrAl2O4)0.05 Mixed-Conducting Membranes
title_full_unstemmed A Comparative Study of the Performance of SrCo0.76Fe0.19Al0.1Ox and (SrCo0.8Fe0.2O3-deltda)0.95(SrAl2O4)0.05 Mixed-Conducting Membranes
title_short A Comparative Study of the Performance of SrCo0.76Fe0.19Al0.1Ox and (SrCo0.8Fe0.2O3-deltda)0.95(SrAl2O4)0.05 Mixed-Conducting Membranes
title_sort comparative study of the performance of srco0.76fe0.19al0.1ox and (srco0.8fe0.2o3-deltda)0.95(sral2o4)0.05 mixed-conducting membranes
url http://hdl.handle.net/20.500.11937/25462