Room-light-induced indoor air purification using an efficient Pt/N-TiO2 photocatalyst

A conceptual air purifier harvesting fluorescent room lights was tested in this study. Visible photocatalysis was applied to facilitate the degradation of volatile organic compounds (VOCs) on a highly efficient visible light photocatalyst, Pt/N-TiO2 synthesised via a sol–gel process. The as-prepared...

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Main Authors: Sun, Hongqi, Ullah, Ruh, Chong, Siewhui, Ang, Ha Ming, Tade, Moses, Wang, Shaobin
Format: Journal Article
Published: elsevier 2011
Online Access:http://hdl.handle.net/20.500.11937/24604
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author Sun, Hongqi
Ullah, Ruh
Chong, Siewhui
Ang, Ha Ming
Tade, Moses
Wang, Shaobin
author_facet Sun, Hongqi
Ullah, Ruh
Chong, Siewhui
Ang, Ha Ming
Tade, Moses
Wang, Shaobin
author_sort Sun, Hongqi
building Curtin Institutional Repository
collection Online Access
description A conceptual air purifier harvesting fluorescent room lights was tested in this study. Visible photocatalysis was applied to facilitate the degradation of volatile organic compounds (VOCs) on a highly efficient visible light photocatalyst, Pt/N-TiO2 synthesised via a sol–gel process. The as-prepared photocatalyst was characterised by many techniques, such as XRD, XPS, UV–vis DRS, N2 adsorption and SEM, etc. XPS spectra revealed that platinum was at a chemical state of 2+, while nitrogen existed as NOx species. The unique chemical compositions made the photocatalyst respond to visible light with a band gap of 2.69 eV, and present a broad absorption shoulder extended further into infrared region. The photocatalytic activities under irradiations of λ > 387, 430 and 490 nm were evaluated by photodegradation of phenol solutions. Under UV–vis light, the Pt/N-TiO2 exhibited 5.5 times higher activity than Degussa P25. Various gaseous pollutants were degraded by employing the Pt/N-TiO2 in a batch reactor. The capability of photodegradation of VOCs under room lights was also proven by the decomposition of gaseous toluene in a continuous reactor using fluorescent lamps (6 × 10 W). The mechanism of the enhanced activity in degradation of VOCs and potential application were discussed.
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publishDate 2011
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spelling curtin-20.500.11937-246042017-09-13T16:08:11Z Room-light-induced indoor air purification using an efficient Pt/N-TiO2 photocatalyst Sun, Hongqi Ullah, Ruh Chong, Siewhui Ang, Ha Ming Tade, Moses Wang, Shaobin A conceptual air purifier harvesting fluorescent room lights was tested in this study. Visible photocatalysis was applied to facilitate the degradation of volatile organic compounds (VOCs) on a highly efficient visible light photocatalyst, Pt/N-TiO2 synthesised via a sol–gel process. The as-prepared photocatalyst was characterised by many techniques, such as XRD, XPS, UV–vis DRS, N2 adsorption and SEM, etc. XPS spectra revealed that platinum was at a chemical state of 2+, while nitrogen existed as NOx species. The unique chemical compositions made the photocatalyst respond to visible light with a band gap of 2.69 eV, and present a broad absorption shoulder extended further into infrared region. The photocatalytic activities under irradiations of λ > 387, 430 and 490 nm were evaluated by photodegradation of phenol solutions. Under UV–vis light, the Pt/N-TiO2 exhibited 5.5 times higher activity than Degussa P25. Various gaseous pollutants were degraded by employing the Pt/N-TiO2 in a batch reactor. The capability of photodegradation of VOCs under room lights was also proven by the decomposition of gaseous toluene in a continuous reactor using fluorescent lamps (6 × 10 W). The mechanism of the enhanced activity in degradation of VOCs and potential application were discussed. 2011 Journal Article http://hdl.handle.net/20.500.11937/24604 10.1016/j.apcatb.2011.08.017 elsevier restricted
spellingShingle Sun, Hongqi
Ullah, Ruh
Chong, Siewhui
Ang, Ha Ming
Tade, Moses
Wang, Shaobin
Room-light-induced indoor air purification using an efficient Pt/N-TiO2 photocatalyst
title Room-light-induced indoor air purification using an efficient Pt/N-TiO2 photocatalyst
title_full Room-light-induced indoor air purification using an efficient Pt/N-TiO2 photocatalyst
title_fullStr Room-light-induced indoor air purification using an efficient Pt/N-TiO2 photocatalyst
title_full_unstemmed Room-light-induced indoor air purification using an efficient Pt/N-TiO2 photocatalyst
title_short Room-light-induced indoor air purification using an efficient Pt/N-TiO2 photocatalyst
title_sort room-light-induced indoor air purification using an efficient pt/n-tio2 photocatalyst
url http://hdl.handle.net/20.500.11937/24604