Poly(furfuryl alcohol)-assisted pyrolysis synthesis of ceramic nanoparticles for solid oxide fuel cells

A pyrolysis synthesis method was developed to prepare ceramic nanoparticles for the fabrication of solid oxide fuel cells. Furfuryl alcohol was used as a polymerizable solvent to dissolve metal nitrates and then polymerized into poly(furfuryl alcohol) (PFA). During the pyrolysis at 600 °C, a mixture...

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Main Authors: Dong, Dehua, Yao, J., Li, Chun-Zhu, Wang, H.
Format: Journal Article
Published: Pergamon 2012
Online Access:http://hdl.handle.net/20.500.11937/23615
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author Dong, Dehua
Yao, J.
Li, Chun-Zhu
Wang, H.
author_facet Dong, Dehua
Yao, J.
Li, Chun-Zhu
Wang, H.
author_sort Dong, Dehua
building Curtin Institutional Repository
collection Online Access
description A pyrolysis synthesis method was developed to prepare ceramic nanoparticles for the fabrication of solid oxide fuel cells. Furfuryl alcohol was used as a polymerizable solvent to dissolve metal nitrates and then polymerized into poly(furfuryl alcohol) (PFA). During the pyrolysis at 600 °C, a mixture of nitrates/PFA was converted into ceramic nanoparticles/carbon networks nanocomposite, and the carbon networks act as a barrier to prevent the aggregation of newly formed nanoparticles during particle crystallization. Dispersible nanoparticles with particle sizes ranging from 40 nm to 200 nm were obtained after burning off carbon networks in air. As an example, Ce0.8Sm0.2O1.9 nanoparticles were synthesized to prepare solid oxide fuel cells, and the fuel cells achieved maximum power densities of 444.5, 625.5 and 684 mW cm−2 at 500 °C, 550 °C and 600 °C, respectively. Our study shows that the pyrolysis synthesis method described here is promising for the effective synthesis of high quality ceramic nanoparticles.
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institution Curtin University Malaysia
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publishDate 2012
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spelling curtin-20.500.11937-236152017-09-13T13:59:40Z Poly(furfuryl alcohol)-assisted pyrolysis synthesis of ceramic nanoparticles for solid oxide fuel cells Dong, Dehua Yao, J. Li, Chun-Zhu Wang, H. A pyrolysis synthesis method was developed to prepare ceramic nanoparticles for the fabrication of solid oxide fuel cells. Furfuryl alcohol was used as a polymerizable solvent to dissolve metal nitrates and then polymerized into poly(furfuryl alcohol) (PFA). During the pyrolysis at 600 °C, a mixture of nitrates/PFA was converted into ceramic nanoparticles/carbon networks nanocomposite, and the carbon networks act as a barrier to prevent the aggregation of newly formed nanoparticles during particle crystallization. Dispersible nanoparticles with particle sizes ranging from 40 nm to 200 nm were obtained after burning off carbon networks in air. As an example, Ce0.8Sm0.2O1.9 nanoparticles were synthesized to prepare solid oxide fuel cells, and the fuel cells achieved maximum power densities of 444.5, 625.5 and 684 mW cm−2 at 500 °C, 550 °C and 600 °C, respectively. Our study shows that the pyrolysis synthesis method described here is promising for the effective synthesis of high quality ceramic nanoparticles. 2012 Journal Article http://hdl.handle.net/20.500.11937/23615 10.1016/j.materresbull.2012.03.052 Pergamon restricted
spellingShingle Dong, Dehua
Yao, J.
Li, Chun-Zhu
Wang, H.
Poly(furfuryl alcohol)-assisted pyrolysis synthesis of ceramic nanoparticles for solid oxide fuel cells
title Poly(furfuryl alcohol)-assisted pyrolysis synthesis of ceramic nanoparticles for solid oxide fuel cells
title_full Poly(furfuryl alcohol)-assisted pyrolysis synthesis of ceramic nanoparticles for solid oxide fuel cells
title_fullStr Poly(furfuryl alcohol)-assisted pyrolysis synthesis of ceramic nanoparticles for solid oxide fuel cells
title_full_unstemmed Poly(furfuryl alcohol)-assisted pyrolysis synthesis of ceramic nanoparticles for solid oxide fuel cells
title_short Poly(furfuryl alcohol)-assisted pyrolysis synthesis of ceramic nanoparticles for solid oxide fuel cells
title_sort poly(furfuryl alcohol)-assisted pyrolysis synthesis of ceramic nanoparticles for solid oxide fuel cells
url http://hdl.handle.net/20.500.11937/23615