Phase transformations and crystallization kinetics in electrospun TiO2 nanofibers in air and argon atmospheres

The effects of atmospheric air and argon environments on thermal-induced phase transformations in electrospun TiO2 nanofibers have been investigated in situ using synchrotron radiation diffraction. Diffraction results showed that the as-synthesized TiO2 nanofibers were initially amorphous, but cryst...

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Main Authors: Albetran, Hani Manssor Mohammed, Haroosh, Hazim Jasim Mohammed, Dong, Yu, Prida, V., O'Connor, Brian, Low, It Meng
Format: Journal Article
Published: Springer 2014
Online Access:http://hdl.handle.net/20.500.11937/23519
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author Albetran, Hani Manssor Mohammed
Haroosh, Hazim Jasim Mohammed
Dong, Yu
Prida, V.
O'Connor, Brian
Low, It Meng
author_facet Albetran, Hani Manssor Mohammed
Haroosh, Hazim Jasim Mohammed
Dong, Yu
Prida, V.
O'Connor, Brian
Low, It Meng
author_sort Albetran, Hani Manssor Mohammed
building Curtin Institutional Repository
collection Online Access
description The effects of atmospheric air and argon environments on thermal-induced phase transformations in electrospun TiO2 nanofibers have been investigated in situ using synchrotron radiation diffraction. Diffraction results showed that the as-synthesized TiO2 nanofibers were initially amorphous, but crystallized to form anatase and rutile after thermal annealing in air or argon at elevated temperatures. The crystallization temperature of anatase was delayed by 100 °C in argon relative to in air, and the transformation of anatase into rutile occurs faster in argon atmosphere than in air due to the formation of oxygen vacancies. Non-linear strains formed in both polymorphs and the substantial elevation of rutile thermal expansion pointed to strain anisotropy in the rutile phase and the concomitant fibre breakage.
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institution Curtin University Malaysia
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last_indexed 2025-11-14T07:48:31Z
publishDate 2014
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spelling curtin-20.500.11937-235192019-02-19T05:35:05Z Phase transformations and crystallization kinetics in electrospun TiO2 nanofibers in air and argon atmospheres Albetran, Hani Manssor Mohammed Haroosh, Hazim Jasim Mohammed Dong, Yu Prida, V. O'Connor, Brian Low, It Meng The effects of atmospheric air and argon environments on thermal-induced phase transformations in electrospun TiO2 nanofibers have been investigated in situ using synchrotron radiation diffraction. Diffraction results showed that the as-synthesized TiO2 nanofibers were initially amorphous, but crystallized to form anatase and rutile after thermal annealing in air or argon at elevated temperatures. The crystallization temperature of anatase was delayed by 100 °C in argon relative to in air, and the transformation of anatase into rutile occurs faster in argon atmosphere than in air due to the formation of oxygen vacancies. Non-linear strains formed in both polymorphs and the substantial elevation of rutile thermal expansion pointed to strain anisotropy in the rutile phase and the concomitant fibre breakage. 2014 Journal Article http://hdl.handle.net/20.500.11937/23519 10.1007/s00339-014-8246-1 Springer fulltext
spellingShingle Albetran, Hani Manssor Mohammed
Haroosh, Hazim Jasim Mohammed
Dong, Yu
Prida, V.
O'Connor, Brian
Low, It Meng
Phase transformations and crystallization kinetics in electrospun TiO2 nanofibers in air and argon atmospheres
title Phase transformations and crystallization kinetics in electrospun TiO2 nanofibers in air and argon atmospheres
title_full Phase transformations and crystallization kinetics in electrospun TiO2 nanofibers in air and argon atmospheres
title_fullStr Phase transformations and crystallization kinetics in electrospun TiO2 nanofibers in air and argon atmospheres
title_full_unstemmed Phase transformations and crystallization kinetics in electrospun TiO2 nanofibers in air and argon atmospheres
title_short Phase transformations and crystallization kinetics in electrospun TiO2 nanofibers in air and argon atmospheres
title_sort phase transformations and crystallization kinetics in electrospun tio2 nanofibers in air and argon atmospheres
url http://hdl.handle.net/20.500.11937/23519