RAFT polymerization and thiol chemistry: A complementary pairing for implementing modern macromolecular design

Reversible addition fragmentation chain transfer (RAFT) polymerization is one of the most extensively studied reversible deactivation radical polymerization methods for the production of well-defined polymers. After polymerization, the RAFT agent end-group can easily be converted into a thiol, openi...

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Main Authors: Roth, P., Boyer, C., Lowe, Andrew, Davis, T.
Format: Journal Article
Published: 2011
Online Access:http://hdl.handle.net/20.500.11937/22588
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author Roth, P.
Boyer, C.
Lowe, Andrew
Davis, T.
author_facet Roth, P.
Boyer, C.
Lowe, Andrew
Davis, T.
author_sort Roth, P.
building Curtin Institutional Repository
collection Online Access
description Reversible addition fragmentation chain transfer (RAFT) polymerization is one of the most extensively studied reversible deactivation radical polymerization methods for the production of well-defined polymers. After polymerization, the RAFT agent end-group can easily be converted into a thiol, opening manifold opportunities for thiol modification reactions. This review is focused both on the introduction of functional end-groups using well-established methods, such as thiol-ene chemistry, as well as on creating bio-cleavable disulfide linkages via disulfide exchange reactions. We demonstrate that thiol modification is a highly attractive and efficient chemistry for modifying RAFT polymers.
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spelling curtin-20.500.11937-225882017-09-13T13:55:44Z RAFT polymerization and thiol chemistry: A complementary pairing for implementing modern macromolecular design Roth, P. Boyer, C. Lowe, Andrew Davis, T. Reversible addition fragmentation chain transfer (RAFT) polymerization is one of the most extensively studied reversible deactivation radical polymerization methods for the production of well-defined polymers. After polymerization, the RAFT agent end-group can easily be converted into a thiol, opening manifold opportunities for thiol modification reactions. This review is focused both on the introduction of functional end-groups using well-established methods, such as thiol-ene chemistry, as well as on creating bio-cleavable disulfide linkages via disulfide exchange reactions. We demonstrate that thiol modification is a highly attractive and efficient chemistry for modifying RAFT polymers. 2011 Journal Article http://hdl.handle.net/20.500.11937/22588 10.1002/marc.201100127 restricted
spellingShingle Roth, P.
Boyer, C.
Lowe, Andrew
Davis, T.
RAFT polymerization and thiol chemistry: A complementary pairing for implementing modern macromolecular design
title RAFT polymerization and thiol chemistry: A complementary pairing for implementing modern macromolecular design
title_full RAFT polymerization and thiol chemistry: A complementary pairing for implementing modern macromolecular design
title_fullStr RAFT polymerization and thiol chemistry: A complementary pairing for implementing modern macromolecular design
title_full_unstemmed RAFT polymerization and thiol chemistry: A complementary pairing for implementing modern macromolecular design
title_short RAFT polymerization and thiol chemistry: A complementary pairing for implementing modern macromolecular design
title_sort raft polymerization and thiol chemistry: a complementary pairing for implementing modern macromolecular design
url http://hdl.handle.net/20.500.11937/22588